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We analyze a single-level quantum system placed between metallic leads and strongly coupled to a localized vibrational mode, which models a singlemolecule junction or an STM setup. We consider a polaron model describing the interaction…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Pino D'Amico , Dmitry A. Ryndyk , Gianaurelio Cuniberti , Klaus Richter

The single-spin memory effect is considered within a minimal polaron model describing a single-level quantum dot interacting with a vibron and weakly coupled to ferromagnetic leads. We show that in the case of strong electron-vibron and…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Dmitry A. Ryndyk , Pino D'Amico , Klaus Richter

We investigate bistability and memory effects in a molecular junction weakly coupled to metallic leads with the latter being subject to an adiabatic periodic change of the bias voltage. The system is described by a simple Anderson-Holstein…

Mesoscale and Nanoscale Physics · Physics 2012-09-20 Andrea Donarini , Abdullah Yar , Milena Grifoni

We study theoretically the transport properties of a molecular two level system with large electron-vibron coupling in the Coulomb blockade regime. We show that when the electron-vibron coupling induces polaron states, the current-voltage…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Gregers A. Kaat , Karsten Flensberg

Consider a quantum dot coupled to two semi-infinite one-dimensional leads at thermal equilibrium. We turn on adiabatically a bias between the leads such that there exists exactly one discrete eigenvalue both at the beginning and at the end…

Mathematical Physics · Physics 2015-07-23 Horia D. Cornean , Arne Jensen , Gheorghe Nenciu

Theory of current hysteresis for tunneling through a molecular quantum dot (MQD) with strong electron-vibron interactions and attractive electron-electron correlations is developed. The dot is modeled as a d-fold degenerate energy level…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 A. S. Alexandrov , A. M. Bratkovsky

The interaction between electronic and vibrational degrees of freedom is an important mechanism in nonequilibrium charge transport through molecular nanojunctions. While adiabatic polaron-type coupling has been studied in great detail, new…

Mesoscale and Nanoscale Physics · Physics 2022-06-10 Christoph Kaspar , André Erpenbeck , Jakob Bätge , Christian Schinabeck , Michael Thoss

We study effects of electron-electron interactions on the steady-state characteristics of a hexagonal molecular ring in a magnetic field, as a model for a benzene molecular junction. The system is driven out of equilibrium by applying a…

Strongly Correlated Electrons · Physics 2014-05-07 Martin Nuss , Wolfgang von der Linden , Enrico Arrigoni

We study the model of a molecular switch comprised of a molecule with a soft vibrational degree of freedom coupled to metallic leads. In the presence of strong electron-ion interaction, different charge states of the molecule correspond to…

Mesoscale and Nanoscale Physics · Physics 2008-12-18 Fabio Pistolesi , Yaroslav M. Blanter , Ivar Martin

We investigate the transient nonequilibrium dynamics of a molecular junction biased by a finite voltage and strongly coupled to internal vibrational degrees of freedom. Using two different, numerical exact techniques, diagrammatic Monte…

Mesoscale and Nanoscale Physics · Physics 2012-10-05 Klaus Ferdinand Albrecht , Haobin Wang , Lothar Muehlbacher , Michael Thoss , Andreas Komnik

Quantum transport through single molecules is very sensitive to the strength of the molecule-electrode contact. Here, we investigate the behavior of a model molecular junction weakly coupled to external electrodes in the case where charging…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Bo Song , Dmitry A. Ryndyk , Gianaurelio Cuniberti

In many organic molecules the strong coupling of excess charges to vibrational modes leads to the formation of polarons, i.e., a localized state of a charge carrier and a molecular deformation. Incoherent hopping of polarons along the…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Benjamin B. Schmidt , Matthias H. Hettler , Gerd Schön

We observe large, reversible, bias driven changes in the vibrational energies of PCBM, based on simultaneous transport and surface-enhanced Raman spectroscopy (SERS) measurements on PCBM-gold junctions. A combination of linear and quadratic…

Mesoscale and Nanoscale Physics · Physics 2016-05-11 Yajing Li , Pavlo Zolotavin , Peter Doak , Leeor Kronik , Jeffrey B. Neaton , Douglas Natelson

Transport through molecular contacts with a sluggish intramolecular vibrational mode strongly coupled to excess charges is studied far from equilibrium. A Born-Oppenheimer approximation in steady state reveals voltage dependent energy…

Mesoscale and Nanoscale Physics · Physics 2012-06-27 Lars Kecke , Joachim Ankerhold

We investigate stationary charge imbalance effect in the system of coupled overdamped Josephson junctions. We show that coupling between junction and nonzero stationary charge imbalance in the resistive state bring to a decrease of the…

Superconductivity · Physics 2020-01-08 K. V. Kulikov , M. Nashaat , Yu. M. Shukrinov

A polaron model proposed as a possible mechanism for nonlinear conductance [Galperin M, Ratner M A, and Nitzan A 2005 Nano Lett. 5 125-30] is revisited with focus on the differences between the weak and strong molecule-lead coupling cases.…

Mesoscale and Nanoscale Physics · Physics 2008-08-26 Michael Galperin , Abraham Nitzan , Mark A. Ratner

We investigate single-electron transport through quantum dots with negative charging energy induced by a polaronic energy shift. For weak dot-lead tunnel couplings, we demonstrate a bipolaronic blockade effect at low biases which suppresses…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 Tie-Feng Fang , Shu-Feng Zhang , Chun-Jiang Niu , Qing-feng Sun

Phase-change memory (PCM), a promising candidate for next-generation non-volatile memories, exploits quenched glassy and thermodynamically stable crystalline states as reversibly switchable state variables. We demonstrate PCM functions…

Strongly Correlated Electrons · Physics 2015-01-15 H. Oike , F. Kagawa , N. Ogawa , A. Ueda , H. Mori , M. Kawasaki , Y. Tokura

Here we study the polaronic transport through molecules weakly connected to metallic electrodes in the nonlinear response regime. Molecule itself is treated as a quantum dot with discrete energy levels, its connection to the electrodes is…

Mesoscale and Nanoscale Physics · Physics 2007-07-22 Kamil Walczak

The role of exchange-correlation effects in non-equilibrium quantum transport through molecular junctions is assessed by analyzing the IV curve of a generic two-level model using self-consistent many-body perturbation theory (second Born…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Kristian S. Thygesen
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