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Related papers: Intersite 4p-3d hybridization in cobalt oxides: a …

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We analyze the recent experiment [W. Neubeck {\em et al.}, Phys. Rev. B \vol(60,1999,R9912)] for the resonant x-ray magnetic scattering (RXMS) around the K edge of Co in the antiferromagnet CoO. We propose a mechanism of the RXMS to make…

Strongly Correlated Electrons · Physics 2009-10-31 Jun-ichi Igarashi , Manabu Takahashi

We study noncentrosymmetric effects on resonant x-ray scattering (RXS) in magnetite. The noncentrosymmetry at A sites in spinel structure makes the 4p states strongly hybridize with the 3d states through neighboring oxygen 2p states, giving…

Strongly Correlated Electrons · Physics 2008-08-12 Jun-ichi Igarashi , Tatsuya Nagao

We investigate mixed-valence oxide Co$_3$O$_4$ using Co $2p3d$ resonant inelastic X-ray scattering (RIXS). By setting resonant edges at Co$^{2+}$ and Co$^{3+}$ ions, the $dd$ excitations on the two Co sites are probed selectively, providing…

X-ray absorption spectroscopy is a well established tool for obtaining information about orbital and spin degrees of freedom in transition metal- and rare earth-compounds. For this purpose usually the dipole transitions of the L- (2p to 3d)…

Strongly Correlated Electrons · Physics 2014-02-21 P. Hansmann , M. W. Haverkort , A. Toschi , G. Sangiovanni , F. Rodolakis , J. P. Rueff , M. Marsi , K. Held

Magnetism in transition metal compounds is usually considered starting from a description of isolated ions, as exact as possible, and treating their (exchange) interaction at a later stage. We show that this standard approach may break down…

Strongly Correlated Electrons · Physics 2016-10-24 S. V. Streltsov , D. I. Khomskii

Generic low-energy spectral features related to $d$-$d$ excitations in nearly cubic vanadium perovskites are predicted for the expected $L$-edge resonant inelastic X-ray scattering (RIXS) measurements. Model Hamiltonian describing local…

Strongly Correlated Electrons · Physics 2013-01-22 V. Yushankhai , L. Siurakshina

$Fe_3O_4$ is a mixed-valence strongly correlated transition metal oxide which displays the intriguing metal to insulator Verwey transition. Here we investigate the electronic and magnetic structure of $Fe_3O_4$ by a unique combination of…

Strongly Correlated Electrons · Physics 2018-11-13 H. Elnaggar , R. Wang , S. Lafuerza , E. Paris , A. C. Komarek , H. Guo , Y. Tseng , D. McNally , F. Frati , M. W. Haverkort , M. Sikora , T. Schmitt , F. M. F. de Groot

X-ray resonant scattering at the K-edge of transition metal oxides is shown to measure the orbital order parameter, supposed to accompany magnetic ordering in some cases. Virtual transitions to the 3d-orbitals are quadrupolar in general. In…

Strongly Correlated Electrons · Physics 2009-10-30 Michele Fabrizio , Massimo Altarelli , Maurizio Benfatto

Room temperature Co K- and La L-edges X-ray absorption studies have been carried out on LaCoO$_3$. Experimental near edge structures have been analysed by theoretical LDA+U density of states (DOS) and multiple scattering (MS) calculations.…

Strongly Correlated Electrons · Physics 2007-05-23 S. K. Pandey , Ashwani Kumar , S. Khalid , A. V. Pimpale

The 4p states in transition metals and their compounds usually play minor roles on their physical quantities. Recent development of resonant x-ray scattering (RXS) at the K-edge of transition metals, however, casts light on the 4p states,…

Materials Science · Physics 2015-06-25 Jun-ichi Igarashi , Manabu Takahashi

We report a comprehensive resonant inelastic x-ray scattering (RIXS) study of various iridate materials focusing on core-level excitations and transitions between crystal-field split d-levels. The 2p core hole created at the Ir $L_3$…

Strongly Correlated Electrons · Physics 2018-05-10 Young-June Kim , J. P. Clancy , H. Gretarsson , G. Cao , Yogesh Singh , Jungho Kim , M. H. Upton , D. Casa , T. Gog

The transition metal K-edge x-ray absorption near edge structure (XANES) studies have been carried on LaBO3 (B=Mn, Fe, Co, Ni), La2CuO4 and SrMnO3 compounds. The theoretical spectra have been calculated using transition metal (TM) 4p…

Strongly Correlated Electrons · Physics 2007-05-23 S. K. Pandey , S. Khalid , A. V. Pimpale

The application of modern layer-by-layer growth techniques to transition-metal oxide materials raises the possibility of creating new classes of materials with rationally designed correlated electron properties. An important step toward…

Materials Science · Physics 2010-10-07 Myung Joon Han , Chris A. Marianetti , Andrew J. Millis

We present a comparative analysis of 1$s$ and 2$p$ core-level hard X-ray photoelectron spectroscopy (HAXPES) spectra in metallic VO$_2$ and CrO$_2$. Even though the V 1$s$ and 2$p$ spectra in VO$_2$ display similar line shapes except the…

Current theoretical studies of electronic correlations in transition metal oxides typically only account for the local repulsion between d-electrons even if oxygen ligand p-states are an explicit part of the effective Hamiltonian.…

Strongly Correlated Electrons · Physics 2015-06-18 Philipp Hansmann , Nicolaus Parragh , Alessandro Toschi , Giorgio Sangiovanni , Karsten Held

2D heterostructures are more than a sum of the parent 2D materials, but are also a product of the interlayer coupling, which can induce new properties. In this paper we present a method to tune the interlayer coupling in Bi2Se3/MoS2 2D…

Soft-x-ray photoemission and absorption spectroscopies are employed to investigate the electronic structures of Sr_{1-x}Rh_{2}O_{4}. Similarly to the layered cobaltates such as Na_{1-x}CoO_{2}, a valence-band satellite feature (VBS) occurs…

Strongly Correlated Electrons · Physics 2009-08-13 Y. Ishida , T. Baba , R. Eguchi , M. Matsunami , M. Taguchi , A. Chainani , Y. Senba , H. Ohashi , Y. Okamoto , H. Takagi , S. Shin

In transition-metal compounds, the transition-metal d electrons play an important role in their physical properties; however, the effects of the electron correlation between the ligand p electrons have not been clear yet. In this Letter,…

The structural, magnetic and electronic properties of transition metal oxides reflect in atomic charge, spin and orbital degrees of freedom. Resonant x-ray scattering (RXS) allows us to perform an accurate investigation of all these…

Strongly Correlated Electrons · Physics 2015-05-14 G. Subías , Joaquín García , Blasco Javier , Javier Herrero-Martin , María Concepción Sanchez

We present a computational study of $L$-edge resonant inelastic x-ray scattering (RIXS) in correlated 3$d$ transition-metal oxides using an $ab$ $initio$ method based on local density approximation + dynamical mean-field theory (DMFT). The…

Strongly Correlated Electrons · Physics 2020-03-25 Atsushi Hariki , Mathias Winder , Takayuki Uozumi , Jan Kuneš
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