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Nonlocal effects have been shown to be responsible for a variety of non-trivial optical effects in small-size plasmonic nanoparticles, beyond classical electrodynamics. However, it is not clear whether optical mode descriptions can be…

Many promising nanophotonics endeavours hinge upon the unique plasmonic properties of nanometallic structures with narrow non-metallic gaps, which support super-concentrated bonding modes that singularly redshift with decreasing…

The plasmon response of metallic nanostructures is anticipated to exhibit nonlocal dynamics of the electron gas when exploring the true nanoscale. We extend the local-response approximation (based on Ohm's law) to account for a general…

Mesoscale and Nanoscale Physics · Physics 2014-03-04 N. Asger Mortensen

We simulate the localized surface plasmon resonances of an Au nanoparticle within tunneling proximity of a Au substrate and demonstrate that the modes may be identified with those responsible for light emission from a scanning tunneling…

Mesoscale and Nanoscale Physics · Physics 2012-07-18 J. Mitra , Lei Feng , Michael G. Boyle , P. Dawson

Noble metal nanoparticles show specific optical properties due to the excitation of localized surface plasmons that make them attractive candidates for highly sensitive bionanosensors. The underlying physical principle is either an…

The nonclassical modification of plasmon-assisted fluorescence enhancement is theoretically explored by placing two-level dipole emitters at the narrow gaps encountered in canonical plasmonic architectures, namely dimers and trimers of…

Mesoscale and Nanoscale Physics · Physics 2017-08-09 Christos Tserkezis , N. Asger Mortensen , Martijn Wubs

Localized surface plasmons in metal nanoparticles are widely used in nano-optics to confine and enhance optical fields. It has been previously shown that, if the nanoparticles are distributed periodically, an additional enhancement can be…

Optics · Physics 2024-06-04 Xiaorun Zang , Andriy Shevchenko

Recent experiments have shown that spatial dispersion may have a conspicuous impact on the response of plasmonic structures. This suggests that in some cases the Drude model should be replaced by more advanced descriptions that take spatial…

Optical nonlocalities are elusive and hardly observable in traditional plasmonic materials like noble and alkali metals. Here we report experimental observation of viscoelastic nonlocalities in the infrared optical response of doped…

The electronic environment causes decoherence and dissipation of the collective surface plasmon excitation in metallic nanoparticles. We show that the coupling to the electronic environment influences the width and the position of the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Guillaume Weick , Gert-Ludwig Ingold , Rodolfo A. Jalabert , Dietmar Weinmann

Experiments have shown strong effects of some substrates on the localized plasmons of metallic nano particles but they are inconclusive on the affecting parameters. Here we have used Discrete Dipole Approximation in conjunction with…

Optics · Physics 2015-06-04 Murugesan Venkatapathi , Abhay K. Tiwari

In plasmonics, nonlocal effects arise when the material response to optical excitations is strongly dependent on the spatial correlations of the excitation. It is well known that a classical free electron gas system supports local Drude…

We analyze dispersion properties of metal-dielectric nanostructured metamaterials. We demonstrate that, in a sharp contrast to the results for the corresponding effective medium, the structure demonstrates strong optical nonlocality due to…

The near-field and far-field spectral response of plasmonic systems are often assumed to be identical, due to the lack of methods that can directly compare and correlate both responses under similar environmental conditions. We develop a…

We study the blueshift of the surface plasmon (SP) resonance energy of isolated Ag nanoparticles with decreasing particle diameter, which we recently measured using electron energy loss spectroscopy (EELS). As the particle diameter…

Optics · Physics 2013-11-05 Søren Raza , Wei Yan , Nicolas Stenger , Martijn Wubs , N. Asger Mortensen

We study the effect of nonlocal optical response on the optical properties of metallic nanowires, by numerically implementing the hydrodynamical Drude model for arbitrary nanowire geometries. We first demonstrate the accuracy of our…

Mesoscale and Nanoscale Physics · Physics 2012-02-07 Giuseppe Toscano , Søren Raza , Antti-Pekka Jauho , N. Asger Mortensen , Martijn Wubs

Polar dielectric nanoresonators can support hybrid photon-phonon modes termed surface phonon polaritons with lengthscales below the diffraction limit. In the deep sub-wavelength regime the optical response of these systems was recently…

Mesoscale and Nanoscale Physics · Physics 2020-06-11 C. R. Gubbin , S. De Liberato

In this work, the plasmonic properties of nanoparticle dimers with optical responses over a wide spectral range have been investigated by varying the inter-particle gap, dimer geometry, gap morphology, nanoparticle composition, and…

Theoretical description of oscillations of electron liquid in large metallic nanospheres (with radius of few tens nm) is formulated within random-phase-approximation semiclassical scheme. Spectrum of plasmons is determined including both…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 W. Jacak , J. Krasnyj , J. Jacak , R. Gonczarek , A. Chepok , L. Jacak , D. Z. Hu , D. Schaadt

Noble metal nanostructures are ubiquitous elements in nano-optics, supporting plasmon modes that can focus light down to length scales commensurate with nonlocal effects associated with quantum confinement and spatial dispersion in the…