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Quantum cascade laser (QCL) frequency combs are a promising candidate for chemical sensing and biomedical diagnostics, requiring only milliseconds of acquisition time to record absorption spectra without any moving parts. They are…
Optical frequency combs have had a remarkable impact on precision spectroscopy. Enabling this technology in the x-ray domain is expected to result in wide-ranging applications, such as stringent tests of astrophysical models and quantum…
A single photon prepared in a time-energy state described by a frequency comb combines the extreme precision of energy defined by a single tooth of the comb with a high sensitivity to small shifts in time defined by the narrowness of a…
We demonstrate for the first time coherent control of bond making, a milestone on the way to coherent control of photo-induced bimolecular chemical reactions. In strong-field multiphoton femtosecond photoassociation experiments, we find the…
Historically, there has been a trade-off in spectroscopic measurements between high spectral resolution, broadband coverage, and acquisition time. Optical frequency combs, initially envisioned for precision spectroscopy of the hydrogen atom…
Optical frequency combs based on mode-locked lasers have proven to be invaluable tools for a wide range of applications in precision spectroscopy and metrology. A novel principle of optical frequency comb generation in whispering-gallery…
The major development recently undergone by quantum cascade lasers has effectively extended frequency comb emission to longer-wavelength spectral regions, i.e. the mid and far infrared. Unlike classical pulsed frequency combs, their…
Reducing the pulse repetition rate of an optical frequency comb increases the pulse energy for a given average power. This enhances the efficiency of nonlinear frequency conversion and it facilitates extending the accessible wavelength…
We analyze several possibilities for precisely measuring electronic transitions in atomic helium by the direct use of phase-stabilized femtosecond frequency combs. Because the comb is self-calibrating and can be shifted into the ultraviolet…
Microresonator frequency combs harness the nonlinear Kerr effect in an integrated optical cavity to generate a multitude of phase-locked frequency lines. The line spacing can reach values in the order of 100 GHz, making it an attractive…
We developed an optical phased array using an optical frequency comb and demonstrated its proof-of-principle. Optical phased arrays have been actively developed in recent years as a technology that can control the wavefront of light without…
Coherent control of the resonant response in spatially extended optomechanical structures is complicated by the fact that the optical drive is affected by the back-action from the generated phonons. Here we report a new approach to coherent…
Optical frequency combs are key to optical precision measurements. While most frequency combs operate in the near-infrared regime, many applications require combs at mid-infrared, visible or even ultra-violet wavelengths. Frequency combs…
Coherent laser beams in the 3 to 20 {\mu}m region of the spectrum are most applicable for chemical sensing by addressing the strongest vibrational absorption resonances of the media. Broadband frequency combs in this spectral range are of…
Nanophotonic quantum devices can significantly boost light-matter interaction which is important for applications such as quantum networks. Reaching a high interaction strength between an optical transition of a spin system and a single…
Atoms are ideal quantum sensors and quantum light emitters. Interfacing atoms with nanophotonic devices promises novel nanoscale sensing and quantum optical functionalities. But precise optical control of atomic states in these devices is…
We describe optimized coherent control methods for two-photon transitions in atoms of a ladder-type three-state energy configuration. Our approach is based on the spatial coherent control scheme which utilizes counter-propagating ultrashort…
We have demonstrated that near complete coherence can be achieved in a four level double lambda-like systems using a train of ultra-short optical pulses. The effect of the Doppler broadening has been analyzed and a scheme has been proposed…
We present an experimental and theoretical investigation of two-photon direct frequency-comb spectroscopy performed through velocity-selective excitation. In particular, we explore the effect of repetition rate on the…
We propose a linear optical quantum computation scheme using time-frequency degree of freedom. In this scheme, a qubit is encoded in single-photon frequency combs, and manipulation of the qubits is performed using time-resolving detectors,…