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Ytterbium-based delafossites with effective S=1/2 moments are investigated intensively as candidates for quantum spin-liquid ground states. While the synthesis of related cerium compounds has also been reported,many important details…

Strongly Correlated Electrons · Physics 2020-12-25 M. S. Eldeeb , T. Petersen , L. Hozoi , V. Yushankhai , U. K. Rossler

Recently, several putative quantum spin liquid (QSL) states were discovered in ${\tilde S} = 1/2$ rare-earth based triangular-lattice antiferromagnets (TLAF) with the delafossite structure. A way to clarify the origin of the QSL state in…

A linear spin-wave approach, a variational method and exact diagonlization are used to investigate the magnetic long-range order (LRO) of the spin-1/2 Heisenberg antiferromagnet on a two-dimensional 1/7-depleted triangular (maple leaf)…

Strongly Correlated Electrons · Physics 2009-11-07 D. Schmalfuss , P. Tomczak , J. Schulenburg , J. Richter

CuFeO_2 is one of the multiferroic materials and is the first case that the electric polarization is not explained by the magnetostriction model or the spin-current model. We have studied this material using soft x-ray resonant diffraction…

{\it Ab-initio} studies of the stability of orbital ordering, its coupling to magnetic structure and its possible origins (electron-phonon and/or electron-electron interactions) are reported for two perovskite systems, LaMnO$_3$ and…

Strongly Correlated Electrons · Physics 2009-11-07 J. E. Medvedeva , M. A. Korotin , V. I. Anisimov , A. J. Freeman

First principles calculations were performed to study the ground state electronic properties of BaFeO3 (BFO) within the density functional theory (DFT). Adopting generalized gradient approximation (GGA) exchange and correlation functional…

Materials Science · Physics 2007-05-23 Hong-Jian Feng , Fa-Min Liu

The double-perovskite A$_2$BB'O$_6$ with heavy transition metal ions on the ordered B' sites is an important family of compounds to study the interplay between electron correlation and spin-orbit coupling (SOC). Here we prepared…

Strongly Correlated Electrons · Physics 2020-07-01 Shang Gao , Daigorou Hirai , Hajime Sagayama , Hiroyuki Ohsumi , Zenji Hiroi , Taka-hisa Arima

Using first principle calculations under the framework of density functional theory we have investigated the electronic structure, magnetism and ferroelectric polarization in the triangular lattice antiferromagnet AgFeO2, and its comparison…

Materials Science · Physics 2018-01-03 Jayita Chakraborty , Indra Dasgupta

Electronic structure calculations of the Verwey ground state of magnetite, Fe3O4, using density functional theory with treatment of on-site Coulomb interactions (DFT+U scheme) are reported. These calculations use the recently-published…

Strongly Correlated Electrons · Physics 2013-01-16 Mark Senn , Ingo Loa , Jon P. Wright , J. Paul Attfield

Yb- and Ce-based delafossites were recently identified as effective spin-1/2 antiferromagnets on the triangular lattice. Several Yb-based systems, such as NaYbO2, NaYbS2, and NaYbSe2, exhibit no long-range order down to the lowest measured…

We used single-crystal x-ray and neutron diffraction to investigate the crystal and magnetic structures of trigonal lattice iridate Ca2Sr2IrO6. The crystal structure is determined to be $R\bar3$ with two distinct Ir sites. The system…

Strongly Correlated Electrons · Physics 2018-06-14 Jieming Sheng , Feng Ye , Christina Hoffmann , Valentino R. Cooper , Satoshi Okamoto , Jasminka Terzic , Hao Zheng , Hengdi Zhao , G. Cao

We investigate the magnetic ground state of CuNdO$_2$, which is a delafossite with a triangular lattice of magnetic Nd$^{3+}$ ions that are well separated by non-magnetic Cu spacer layers. From inelastic neutron scattering measurements of…

Ground state and low-energy excitations of the quasi-one-dimensional antiferromagnet CuSe$_2$O$_5$ were experimentally studied using bulk magnetization, neutron diffraction, muon spin relaxation and antiferromagnetic resonance measurements.…

Strongly Correlated Electrons · Physics 2015-06-12 M. Herak , A. Zorko , M. Pregelj , O. Zaharko , G. Posnjak , Z. Jagličić , A. Potočnik , H. Luetkens , J. van Tol , A. Ozarowski , H. Berger , D. Arčon

Quasiperiodic structures possess long range positional order, but are freed of constraints imposed by translational invariance. For spins interacting via Heisenberg couplings, one may expect therefore to find novel magnetic configurations…

Strongly Correlated Electrons · Physics 2008-10-15 Anuradha Jagannathan , Attila Szallas

We predict that the anti-ferromagnetic (AFM) magnetic structure of delafossite PdCrO$_2$ has a staggered chirality with the double-layer periodicity along the $z$-axis with intriguing magnetic anisotropy. We study the electronic and…

Strongly Correlated Electrons · Physics 2020-01-22 Changhwi Park , Jaejun Yu

Multiferroic CuFe1-xAlxO2 (x=0.02) exhibits a ferroelectric ordering accompanied by a proper helical magnetic ordering below T=7K under zero magnetic field. By polarized neutron diffraction and pyroelectric measurements, we have revealed a…

Strongly Correlated Electrons · Physics 2008-03-31 T. Nakajima , S. Mitsuda , S. Kanetsuki , K. Tanaka , K. Fujii , N. Terada , M. Soda , M. Matsuura , K. Hirota

Magnetic and electronic structures in LaFeAsO in the single-stripe-type antiferromagnetic (AFM) phase are studied using first-principles density-functional calculations including the spin-orbit interaction. We show that the longitudinal…

Superconductivity · Physics 2016-12-28 Sehoon Oh , Jung-Hoon Lee , Hyun Myung Jang , Hyoung Joon Choi

We succeeded in observing pressure-suppressed magnetic long range ordering (LRO) in the triangular lattice antiferromagnet CuFeO$_{2}$, using neutron diffraction experiments under an isotropic pressure. The magnetic LRO of the…

Strongly Correlated Electrons · Physics 2015-03-17 Noriki Terada , Toyotaka Osakabe , Hideaki Kitazawa

We report the comprehensive experimental results identifying the magnetic spin ordering and the magnetization dynamics of a double perovskite Pr2CoFeO6 by employing the (dc and ac) magnetization, powder neutron diffraction (NPD) and X-ray…

Crystal and magnetic structures of the mineral centennialite CaCu$_3$(OH)$_6$Cl$_2\cdot0.6$H$_2$O are investigated by means of synchrotron x-ray diffraction and neutron diffraction measurements complemented by density functional theory…

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