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We analytically study the linear propagation of arbitrarily shaped light-pulses through an absorbing medium with a narrow transparency-window or through a resonant amplifying medium. We point out that, under certain general conditions, the…
We use state- and time-resolved coherent Raman spectroscopy to study the rotational dynamics of oxygen molecules in ultra-high rotational states. While it is possible to reach rotational quantum numbers up to $N \approx 50$ by increasing…
Four-wave mixing can be stimulated or occur spontaneously. The first process is intrinsically much stronger, and well understood through classical nonlinear optics. The latter, also known as parametric fluorescence, can be explained only in…
Resonant nonlinear-optical interference processes in four-level Doppler-broadened media are studied. Specific features of amplification and optical switching of short-wavelength radiation in a strongly-absorbing resonant gas under coherent…
Quantum entanglement has emerged as a great resource for interactions between molecules and radiation. We propose a new paradigm of stimulated Raman scattering with entangled photons. A quantum ultrafast Raman spectroscopy is developed for…
We develop an ultrafast frequency-resolved Raman spectroscopy with entangled photons for polyatomic molecules in condensed phases, to probe the electronic and vibrational coherences. Using quantum correlation between the photons, the signal…
Slow-light media are of interest in the context of quantum computing and enhanced measurement of quantum effects, with particular emphasis on using slow-light with single photons. We use light-in-flight imaging with a single photon…
Non-Hermitian optical systems with parity-time (PT) symmetry have recently revealed many intriguing prospects that outperform conservative structures. The prevous works are mostly rooted in complex arrangements with controlled gain-loss…
We show that arrival times for electromagnetic pulses measured through the rate of absorption in an ideal impedance matched detector are equivalent to the arrival times using the average flow of optical energy as proposed by Peatross {\it…
Raman spectroscopy uses light scattering to extract information on low-energy excitations of solids. The Raman process is described by diagrams which are fourth order in the light-matter interaction, and in particular the resonant…
We report the demonstration of phase coherence and control for the recently developed "light storage" technique. Specifically, we use a pulsed magnetic field to vary the phase of atomic spin excitations which result from the deceleration…
We report observations of novel dynamic behavior in resonantly-enhanced stimulated Raman scattering in Rb vapor. In particular, we demonstrate a dynamic hysteresis of the Raman scattered optical field in response to changes of the drive…
The development of optical metamaterials has resulted in the demonstration of remarkable physical properties, including cloaking, optical magnetism, and negative refraction. The latter has attracted particular interest, mainly because of…
We present results of a study of four-wave mixing in Rb vapour with highly nonlinear susceptibility, using both homodyne and heterodyne detection. We demonstrate that the spectra have different appearances for media possessing…
Nonstationary pump-probe interaction between short laser pulses propagating in a resonant optically dense coherent medium is considered. A special attention is paid to the case, where the density of two-level particles is high enough that a…
Single photon, emitted in a transition between two states, has a frequency distribution of intensity, which is given by Lorentzian if the transition is only naturally broadened and the period of observation $T$ is long compared to the…
For future quantum technologies the combination of a long quantum state lifetime and an efficient interface with external optical excitation are required. In solids, the former is for example achieved by individual spins, while the latter…
In recent years, photon drag has attracted enormous attention owing to both fundamental and practical interests. In this paper, by presenting a density-matrix approach, we have theoretically demonstrated an enhanced photon drag in a moving…
We describe possibilities of spontaneous, degenerate four-wave mixing (FWM) processes in spin-orbit coupled Bose-Einstein condensates. Phase matching conditions (i.e., energy and momentum conservation laws) in such systems allow one to…
By identifying the similarities between the coupled-wave equations and the parametrically driven nonlinear Schr\"odinger equation, we unveil the existence condition of the quadratic soliton mode-locked degenerate optical parametric…