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We present a neutron and x-ray scattering investigation of Ca$_3$LiOsO$_6$, a material predicted to host magnetic ordering solely through an extended superexchange pathway involving two anions, an interaction mechanism that has undergone…

Strongly Correlated Electrons · Physics 2012-08-13 S. Calder , M. D. Lumsden , V. O. Garlea , J. -W. Kim , Y. G. Shi , H. L. Feng , K. Yamaura , A. D. Christianson

Low dimensionality, broken symmetry and easily-modulated carrier concentrations provoke novel electronic phase emergence at oxide interfaces. However, the spatial extent of such reconstructions - i.e. the interfacial "depth" - remains…

Strongly Correlated Electrons · Physics 2014-06-23 A. P. Petrović , A. Paré , T. R. Paudel , K. Lee , S. Holmes , C. H. W. Barnes , A. David , T. Wu , E. Y. Tsymbal , C. Panagopoulos

The electronic and magnetic properties of NdNiO$_3$ (NNO) thin films are very sensitive to epitaxial strain and to the proximity to ferromagnetic oxides. In this work, we investigate the structural, electronic, and magnetic properties of…

Materials Science · Physics 2024-09-20 Henrique M. M. Cardoso , Maria C. O. Aguiar , Cinthia Piamonteze , Walber H. Brito

Performing an analysis within density functional theory, we develop insight into the structural and electronic properties of the oxide heterostructure LaAlO3/SrTiO3. Electrostatic surface effects are decomposed from the internal lattice…

Materials Science · Physics 2015-05-13 U. Schwingenschloegl , C. Schuster

We present calculations of the charge density profile, subband occupancy and ellipsometry spectra of the electron gas at the LaAlO3/SrTiO3 interface. The calculations employ self-consistent Hartree and random phase approximations, a tight…

Strongly Correlated Electrons · Physics 2015-06-15 Se Young Park , Andrew J. Millis

The $t_{2g}$ band-structure of SrTiO$_3$-based two-dimensional electron gasses (2DEGs), have been found to play a role in features such as the superconducting dome, high-mobility transport, and the magnitude of spin-orbit coupling. This…

A detailed analysis of the crystal structure in RETiO3 with RE = La, Nd, Sm, Gd, and Y reveals an intrinsic coupling between orbital degrees of freedom and the lattice which cannot be fully attributed to the structural deformation arising…

Strongly Correlated Electrons · Physics 2009-09-29 A. C. Komarek , H. Roth , M. Cwik , W. -D. Stein , J. Baier , M. Kriener , F. Bouree , T. Lorenz , M. Braden

We investigate the effect of the experimentally observed Jahn-Teller distortion of the oxygen octahedra in LaTiO3 on the magnetic exchange. We present a localized model for the effective hopping between nearest-neighbor Ti ions and the…

Strongly Correlated Electrons · Physics 2009-11-10 Robert Schmitz , Ora Entin-Wohlman , Amnon Aharony , A. Brooks Harris , Erwin Mueller-Hartmann

The emerging field of complex oxide interfaces is generically built on one of the most celebrated substrates - strontium titanate (SrTiO3). This material hosts a range of phenomena, including ferroelasticity, incipient ferroelectricity, and…

Mesoscale and Nanoscale Physics · Physics 2013-12-13 Maayan Honig , Joseph A. Sulpizio , Jonathan Drori , Arjun Joshua , Eli Zeldov , Shahal Ilani

Polar discontinuities occurring at interfaces between two different materials constitute both a challenge and an opportunity in the study and application of a variety of devices. In order to cure the large electric field occurring in such…

Recent experiments have found new magnetic behaviors, which are different from the parent bulk materials, at the interfaces between 3$d$ and 5$d$ oxides such as SrMnO$_3$ (SMO) and SrIrO$_3$ (SIO). The system is of considerable interest due…

Strongly Correlated Electrons · Physics 2018-08-29 Sayantika Bhowal , Sashi Satpathy

The electronic and magnetic properties of the delafossite CuFeO2 are investigated by means of electronic structure calculations. They are performed using density functional theory in the generalized gradient approximation as well as the new…

Strongly Correlated Electrons · Physics 2008-08-24 Volker Eyert , Raymond Fresard , Antoine Maignan

We show that oxygen vacancies at titanate interfaces induce a complex multiorbital reconstruction which involves a lowering of the local symmetry and an inversion of t2g and eg orbitals resulting in the occupation of the eg orbitals of Ti…

Strongly Correlated Electrons · Physics 2012-08-27 N. Pavlenko , T. Kopp , E. Y. Tsymbal , J. Mannhart , G. A. Sawatzky

The interface between the band gap insulators LaAlO3 and SrTiO3 is known to host a highly mobile two-dimensional electron gas. Here we report on the fabrication and characterization of the NdGaO3/SrTiO3 interface, that shares with…

Recently a metallic state was discovered at the interface between insulating oxides, most notably LaAlO3 and SrTiO3. Properties of this two-dimensional electron gas (2DEG) have attracted significant interest due to its potential…

After more than a decade of extensive research on the magnetic order triggered by lattice defects in a wide range of nominally non-magnetic materials, we report its application in a spintronic device. This device is based on a spin-filter…

Mesoscale and Nanoscale Physics · Physics 2017-07-10 L. Botsch , I. Lorite , Y. Kumar , P. Esquinazi , T. Michalsky , J. Zajadacz , K. Zimmer

Understanding the nature of charge carriers at the LaAlO3/SrTiO3 interface is one of the major open issues in the full comprehension of the charge confinement phenomenon in oxide heterostructures. Here, we investigate thermopower to study…

Strongly Correlated Electrons · Physics 2015-04-09 I. Pallecchi , F. Telesio , D. Li , A. Fête , S. Gariglio , J. -M. Triscone , A. Filippetti , P. Delugas , V. Fiorentini , D. Marré

We have measured the electronic structure of the two-dimensional electron system (2DES) found at the Al/SrTiO3 (Al/STO) and LaAlO3/SrTiO3 (LAO/STO) interfaces by means of laser angle resolved photoemission spectroscopy, taking advantage of…

First principles calculations reveal that adding a metallic overlayer on LaAlO3/SrTiO3(001) eliminates the electric field within the polar LaAlO3 film and thus suppresses the thickness-dependent insulator-to-metal transition observed in…

Materials Science · Physics 2012-03-23 V. G. Ruiz López , R. Arras , W. E. Pickett , R. Pentcheva

We present a study of modulation of spin-orbit interaction (SOI) at the interface of LaTiO$_3$/SrTiO$_3$ by $\delta$-doping with an iso-structural ferromagnetic perovskite LaCoO$_3$. The sheet carrier density at the interface decreases…

Strongly Correlated Electrons · Physics 2016-10-18 Shubhankar Das , Z. Hossain , R. C. Budhani