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Single-molecule electronics has been envisioned as the ultimate goal in the miniaturisation of electronic circuits. While the aim of incorporating single-molecule junctions into modern technology still proves elusive, recent developments in…

Mesoscale and Nanoscale Physics · Physics 2017-11-22 Jakub K. Sowa , Jan A. Mol , G. Andrew D. Briggs , Erik M. Gauger

In the present work we theoretically analyze electroluminescence occurring in a biased single-molecule junction with a chiral bridge imitated by a helical chain. We show that optical transitions between electron states of the chiral linker…

Mesoscale and Nanoscale Physics · Physics 2025-07-22 Natalya A Zimbovskaya

We study the behavior of shot noise in resonant tunneling junctions far from equilibrium. Quantum-coherent elastic charge transport can be characterized by a transmission function, that is the probability for an incoming electron at a given…

Mesoscale and Nanoscale Physics · Physics 2019-02-19 Anqi Mu , Dvira Segal

We show how one can measure the signal from slow jumps of a single molecule between metastable positions using a setup where the molecule is fixed to one lead, and one of the coupling strengths is controlled externally. Such a measurement…

Mesoscale and Nanoscale Physics · Physics 2013-04-04 Tero T. Heikkila , Wolfgang Belzig

An experimental protocol which allows to perform conductance spectroscopy on organic molecules at low temperatures (T~30 K) has been developed. This extends the method of mechanically controlled break junctions which has recently…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 J. Reichert , H. B. Weber , M. Mayor , H. v. Löhneysen

We present a device architecture of hybrid-edge and dual-gated quantum point contact. We demonstrate improved electrostatic control over the separation, position, and coupling of each broken-symmetry compressible strip in graphene. Via…

Mesoscale and Nanoscale Physics · Physics 2023-11-27 Wei Ren , Xi Zhang , Jaden Ma , Xihe Han , Kenji Watanabe , Takashi Taniguchi , Ke Wang

We have combined ab initio quantum chemistry calculations with a rate-equation formalism to analyze electroluminescence spectra in single-molecule junctions, measured recently by several groups in Scanning Tunneling Microscope setups. In…

Mesoscale and Nanoscale Physics · Physics 2010-05-20 Johannes S. Seldenthuis , Herre S. J. van der Zant , Mark A. Ratner , Joseph M. Thijssen

We calculate the tunneling density of states (TDOS) in a three wire junction of interacting spin-1/2 electrons, and find an anomalous enhancement of the TDOS in the zero bias limit, even for repulsive interactions for several bosonic fixed…

Mesoscale and Nanoscale Physics · Physics 2015-08-05 Sougata Mardanya , Amit Agarwal

Here we present theoretical studies of the effect of vibronic coupling on nonlinear transport characteristics (current-voltage and conductance-voltage) in molecular electronic devices. Considered device is composed of molecular quantum dot…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Kamil Walczak

The low-temperature transport properties of a molecule are studied in the field-effect transitor geometry. The molecule has an internal mechanical mode that modulates its electronic levels and renormalizes both the interactions and the…

Strongly Correlated Electrons · Physics 2008-01-23 P. S. Cornaglia , Gonzalo Usaj , C. A. Balseiro

Vibrational-excitation cross sections of ground electronic state of carbon dioxide molecule by electron-impact through the CO2-(2\Pi) shape resonance is considered in the separation of the normal modes approximation. Resonance curves and…

Chemical Physics · Physics 2016-11-01 V. Laporta , J. Tennyson , R. Celiberto

We develop a microscopic model to investigate current-induced light emission in single-molecule tunnel junctions, where a two-level system interacts with a plasmonic field. Using the quantum master equation, we explore the transition from…

Mesoscale and Nanoscale Physics · Physics 2025-07-08 Andrés Bejarano , Moritz Frankerl , Rémi Avriller , Thomas Frederiksen , Fabio Pistolesi

Motivated by a recent experiment on nonlinear tunneling in a suspended Carbon nanotube connected to two normal electrodes [S. Sapmaz, {\it et al}., Phys. Rev. Lett. {\bf 96}, 26801 (2006)], we investigate nonequilibrium vibration-mediated…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 X. Y. Shen , Bing Dong , X. L. Lei , N. J. M. Horing

We consider the interaction between electrons and molecular vibrations in the context of electronic transport in nanoscale devices. We present a method based on non-equilibrium Green's functions to calculate both equilibrium and…

Mesoscale and Nanoscale Physics · Physics 2010-03-16 L. K. Dash , H. Ness , R. W. Godby

We have computed the probability distribution of the conductance of a ballistic and chaotic cavity which is connected to two electron reservoirs by leads with a single propagating mode, for arbitrary values of the transmission probability…

Condensed Matter · Physics 2007-05-23 P. W. Brouwer , C. W. J. Beenakker

Transition voltage spectroscopy (TVS) has recently been introduced as a spectroscopic tool for molecular junctions where it offers the possibility to probe molecular level energies at relatively low bias voltages. In this work we perform…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 Jingzhe Chen , Troels Markussen , Kristian S. Thygesen

A single electron shared between two levels threaded by a magnetic flux is an irreducibly simple quantum system in which interference is predicted to occur. We demonstrate tuning of the tunnel coupling between two such electronic levels…

Mesoscale and Nanoscale Physics · Physics 2024-09-12 Christian G. Prosko , Ivan Kulesh , Michael Chan , Lin Han , Di Xiao , Candice Thomas , Michael J. Manfra , Srijit Goswami , Filip K. Malinowski

We present a theory of single-electron tunneling transport through a ferromagnetic nanoparticle in which particle-hole excitations are coupled to spin collective modes. The model employed to describe the interaction between quasiparticles…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 L. Michalak , C. M. Canali , V. G. Benza

We theoretically analyzed inelastic effects in the electron transport through molecular junctions originating from electron-vibron interactions. The molecular bridge was simulated by a periodic chain of identical interacting hydrogen-like…

Materials Science · Physics 2010-01-03 Natalya A. Zimbovskaya , Maija M. Kuklja

We investigate electronic transport through two types of conjugated molecules. Mechanically controlled break-junctions are used to couple thiol endgroups of single molecules to two gold electrodes. Current-voltage characteristics (IVs) of…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 J. Reichert , R. Ochs , D. Beckmann , H. B. Weber , M. Mayor , H. v. Loehneysen