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The order of high harmonics emitted by an atom in an intense laser field is limited by the so-called cutoff frequency. Solving the time-dependent Schr\"odinger equation, we show that this frequency can be increased considerably by a…

Atomic Physics · Physics 2016-09-08 Carla Figueira de Morisson Faria , Jan-Michael Rost

We studied the high-order harmonic generation (HHG) from 2D solid materials in circularly and bichromatic circularly polarized laser fields numerically by simulating the dynamics of single-active-electron processes in 2D periodic…

High harmonic generation (HHG) in solids has recently emerged as a powerful all-optical approach for probing material properties and ultrafast electron dynamics in quantum systems. It has been widely applied for studying two-dimensional and…

Optics · Physics 2026-04-28 Eyal Uzner , Ofer Neufeld

Isotropic gases irradiated by long pulses of intense IR light can generate very high harmonics of the incident field. It is generally accepted that, due to the symmetry of the generating medium, be it an atomic or an isotropic molecular…

Atomic Physics · Physics 2016-09-28 R. E. F. Silva , P. Rivière , F. Morales , O. Smirnova , M. Ivanov , F. Martín

High-order harmonic generation (HHG) is combined with resonant x-ray excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process. To describe this setting, I develop a…

Atomic Physics · Physics 2015-10-15 Christian Buth

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

Atomic Physics · Physics 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

We study theoretically and experimentally High Harmonic Generation (HHG) using two non collinear driving fields focused in gases. We show that these two fields form a non stationary blazed active grating in the generation medium. The…

Optics · Physics 2019-03-13 C. Chappuis , D. Bresteau , T. Auguste , O. Gobert , T. Ruchon

The alignment- and internuclear-distance dependent ionization of H$_2$ exposed to intense, ultrashort laser fields is studied by solving the time-dependent two-electron Schr\"odinger equation. In the regime of perturbative few-photon…

Atomic Physics · Physics 2015-06-23 Johann Förster , Yulian V. Vanne , Alejandro Saenz

We make a systematic study of high-order harmonic generation (HHG) in a He$^+$-like model ion when the initial states are prepared as a coherent superposition of the ground state and an excited state. It is found that, according to the…

Atomic Physics · Physics 2009-11-11 Bingbing Wang , Taiwang Cheng , Xiaofeng Li , Panming Fu , Shigang Chen , Jie Liu

In a recent experiment (N. Wagner et al., PNAS v103, p13279) on SF$_{6}$, a high-harmonic generating laser pulse is preceded by a pump pulse which stimulates Raman-active modes in the molecule. Varying the time delay between the two pulses…

Atomic Physics · Physics 2009-11-13 Zachary B. Walters , Stefano Tonzani , Chris H. Greene

High-order harmonic generation from atomic systems is considered in the crossed fields of a relativistically strong infrared laser and a weak attosecond-pulse train of soft x-rays. Due to one-photon ionization by the x-ray pulse, the…

Atomic Physics · Physics 2009-11-13 Michael Klaiber , Karen Z. Hatsagortsyan , Carsten Müller , Christoph H. Keitel

High-order harmonic generation (HHG) in gases leads to short-pulse extreme ultraviolet (XUV) radiation useful in a number of applications, for example, attosecond science and nanoscale imaging. However, this process depends on many…

We theoretically investigate the interference effect of high-order harmonics generated from molecules at different alignment angles. It is shown that the interference of the harmonic emissions from molecules aligned at different angles can…

Optics · Physics 2015-02-27 Meiyan Qin , Xiaosong Zhu , Yang Li , Qingbin Zhang , Pengfei Lan , Peixiang Lu

The magnetic dressing phenomenon occurs when spins precessing in a static field (holding field) are subject to an additional, strong, alternating field. It is usually studied when such extra field is homogeneous and oscillates in one…

Atomic Physics · Physics 2021-04-16 Giuseppe Bevilacqua , Valerio Biancalana , Yordanka Dancheva , Antonio Vigilante

We present an experimental technique using orbital angular momentum (OAM) in a fundamental laser field to drive High Harmonic Generation (HHG). The mixing of beams with different OAM allows to generate two laser foci tightly spaced to study…

Chemical Physics · Physics 2019-07-24 Jan Troßand Carlos A. Trallero-Herrero

Increase of the cut-off value in the high order harmonics generation process is demonstrated for a special case of the driving field composed of several harmonics of a given frequency. It is shown that a moderate, of the order of 20%,…

Atomic Physics · Physics 2015-05-13 I. A. Ivanov , A. S. Kheifets

We make a detailed assessment of which form of the dipole operator to use in calculating high order harmonic generation within the framework of the strong field approximation, and look specifically at the role the form plays in the…

Atomic Physics · Physics 2015-05-19 B. B. Augstein , C. Figueira de Morisson Faria

High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to…

We consider several aspects of high-order harmonic generation in solids: the effects of elastic and inelastic scattering; varying pulse characteristics; and inclusion of material-specific parameters through a realistic band structure. We…

Other Condensed Matter · Physics 2013-02-07 A. F. Kemper , B. Moritz , J. K. Freericks , T. P. Devereaux

High-harmonic generation from hydrogenlike muonic atoms exposed to ultraintense high-frequency laser fields is calculated. Systems of low nuclear charge number Z are considered where a nonrelativistic description applies. By comparing the…

Atomic Physics · Physics 2015-05-18 Atif Shahbaz , Thomas J. Buervenich , Carsten Müller