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We use extreme-ultraviolet interferometry to measure the phase of high-order harmonic generation from transiently aligned CO2 molecules. We unambiguously observe a reversal in phase of the high order harmonic emission for higher harmonic…

Atomic Physics · Physics 2009-11-13 Xibin Zhou , Robynne Lock , Wen Li , Nick Wagner , Margaret. M. Murnane , Henry C. Kapteyn

We present ab initio calculations using the $R$-matrix with time dependence (RMT) method for high-order harmonic generation (HHG) in argon in a short, intense pulse regime. The calculations employ a $6$-cycle $\sin^2$ pulse at $850$ nm with…

Atomic Physics · Physics 2026-04-23 Aaron T. Bondy , Klaus Bartschat

We study high-order harmonic generation (HHG) resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneities of the local electric field and the confinement of the electron motion…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , Srdjan S. Acimovic , T. Shaaran , J. Biegert , R. Quidant , M. Lewenstein

We theoretically study high-order harmonic generation (HHG) from solid-phase systems in spatially inhomogeneous strong laser fields originated by resonant plasmons within a metallic nanostructure. The intensity of the second plateau in HHG…

Optics · Physics 2016-09-12 Tao-Yuan Du , Zhong Guan , Xiao-Xin Zhou , Xue-Bin Bian

We present Floquet calculations of high harmonic generation (HHG) for the lowest two electronic states of the $\mbox{H}_2^+$ ion by strong continuous-wave laser fields. We solve the non-Hermitian matrix problem to get accurate solutions to…

Atomic Physics · Physics 2015-06-18 Ts Tsogbayar , M Horbatsch

We present a study of the possibility to significantly enhance the efficiency of high-order harmonic generation (HHG) using few-cycle optical waveforms obtained by superposing two laser pulses of different color delayed optimally relative…

Optics · Physics 2024-12-11 O. V. Meshkov , M. Yu. Emelin , M. Yu. Ryabikin

We investigate the effect of dynamic electron correlation on high-harmonic generation in helium atoms using intense visible light (\lambda=390nm). Two complementary approaches are used which account for correlation in an approximate manner:…

Quantum Physics · Physics 2009-05-21 G. A. McKenna , R. Nepstad , J. F. McCann , D. Dundas

High order harmonic (HOH) generation by interacting extremely intense electromagnetic waves in the quantum vacuum is investigated within the framework of the Heisenberg-Euler formalism. We consider here the process in the lowest order of a…

Plasma Physics · Physics 2026-01-13 Pavel Sasorov , Sergei Bulanov

We investigate ultrafast harmonic generation (HG) in Si:B, driven by intense pump pulses with fields reaching ~100 kV/cm and a carrier frequency of 300 GHz, at 4 K and 300 K, both experimentally and theoretically. We report several novel…

We investigate the generation of higher-order harmonics from a quantum optics perspective via the interaction of a semiconductor with a coherent pump field focusing on the regime where strong-field intraband excitations dominate. The…

The sub-cycle dynamics of electrons driven by strong laser fields is central to the emerging field of attosecond science. We demonstrate how the dynamics can be probed through high-order harmonic generation, where different trajectories…

The generation of high harmonics (HHG) in atomic systems by the highly non-linear response to an intense laser field is a prominent pathway to the synthesis of ever shorter laser pulses at increasingly higher photon energies. Extensions of…

Atomic Physics · Physics 2022-11-23 Mohammad Monfared , Elnaz Irani , Christoph Lemell , Joachim Burgdörfer

The strong-field approximation for high-harmonic generation in near-infrared and infrared laser pulses is formulated in the accelerated Kramers-Henneberger frame. The accompanying physical picture is discussed and the nature of the…

Quantum Physics · Physics 2021-10-04 Lars Bojer Madsen

We compare the enhancement of high-order harmonic generation in argon using 800--400 and 800--266~nm laser fields with their optimized single-color counterparts. We observe that the two-color fields generally outperform the single-color…

We experimentally observe longer than long trajectory influence in high order harmonic generation (HHG) by varying the peak intensity of the driving laser field through either direct attenuation, or by chirping the laser pulse. Using a…

We report the first experimental observation of frequency shift in high order harmonic generation (HHG) from isotopic molecules H2 and D2 . It is found that harmonics generated from the isotopic molecules exhibit obvious spectral red shift…

Atomic Physics · Physics 2016-04-25 Lixin He , Pengfei Lan , Chunyang Zhai , Feng Wang , Wenjing Shi , Qingbin Zhang , Xiaosong Zhu , Peixiang Lu

We present an analytic, and fully quantum theory of high harmonic generation by low frequency laser fields for a two-state hydrogenlike atom model. The model is valid for an arbitrary atomic potential role of dipole matrix elements and can…

Optics · Physics 2011-04-19 S Batebi , M Mohebbi

We present the theoretical treatment of laser-assisted $(e,2e)$ ionizing collisions in hydrogen for fast electrons, in the framework of the first-order Born approximation at moderate laser intensities and photon energies beyond the…

Atomic Physics · Physics 2023-06-19 Gabriela Buică

We investigated the high-order harmonic generation (HHG) process of diatomic molecular ion $\mathrm{H}_2^+$ in non-Born-Oppenheimer approximations. The corresponding three-dimensional time-dependent Schr\"odinger equation is solved with…

Atomic Physics · Physics 2017-02-28 Mu-Zi Li , Guang-Rui Jia , Xue-Bin Bian

The generation of harmonics by atoms or ions in a two-color, coplanar field configuration with commensurate frequencies is investigated through both, an analytical calculation based on the Lewenstein model and the numerical ab initio…

Atomic Physics · Physics 2009-11-07 F. Ceccherini , D. Bauer , F. Cornolti