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Orbital degrees of freedom play a major role in the physics of many strongly correlated transition metal compounds. However, they are still very difficult to access experimentally, in particular by neutron scattering. We propose here how to…

Strongly Correlated Electrons · Physics 2015-04-28 Pasquale Marra

We develop a formalism to calculate the L-edge resonant x-ray scattering (RIXS) spectra from transition-metal compounds. Using a multi-orbital tight-binding model, we derive useful formulas to calculate the spectra by collecting up the…

Strongly Correlated Electrons · Physics 2015-06-16 Jun-ichi Igarashi , Tatsuya Nagao

Inelastic X-ray scattering (IXS) is an important tool for studies of equilibrium dynamics in condensed matter. A new spectrometer recently proposed for ultra-high-resolution IXS (UHRIX) has achieved 0.6~meV and 0.25~nm$^{-1}$ spectral and…

We investigate theoretically the resonant inelastic x-ray scattering (RIXS) at the $K$ edge of Si on the basis of an ab initio calculation. We calculate the RIXS spectra with systematically varying transfered-momenta, incident-photon energy…

Materials Science · Physics 2007-05-23 Yunori Nisikawa , Manabu Usuda , Jun-ichi Igarashi

The resonant inelastic x-ray scattering (RIXS) was measured in an insulating SrCuO$_{2}$ with changing the incident photon energy ($h\nu$) near the Cu $1s$ absorption edge (K-edge). Complex structures and their dependences on the momentum…

We explore the general phenomenology of resonant inelastic scattering (RIXS) using CuB2O4, a network of CuO4 plaquettes electronically isolated by B+3 ions. Spectra show a small number of well-separated features, and we exploit the simple…

Strongly Correlated Electrons · Physics 2013-05-29 J. N. Hancock , G. Chabot-Couture , Y. Li , G. Petrakovskii , K. Ishii , I. Jarrige , J. Mizuki , T. P. Devereaux , M. Greven

Young's archetypal double-slit experiment forms the basis for modern diffraction techniques: the elastic scattering of waves yields an interference pattern that captures the real-space structure. Here, we report on an inelastic incarnation…

Resonant inelastic x-ray scattering (RIXS) provides remarkable opportunities to interrogate ultrafast dynamics in liquids. Here we use RIXS to study the fundamentally and practically important hydroxyl radical in liquid water, OH(aq).…

We used high-resolution resonant inelastic x-ray scattering (RIXS) at the Ni $L_3$ edge to simultaneously investigate high-energy interband transitions characteristic of Ni-O bond ordering and low-energy collective excitations of the Ni…

Core hole resonance is used in X-ray spectroscopy to incisively probe the local electronic states of many-body systems. Here, resonant inelastic X-ray scattering (RIXS) is studied as a function of incident photon energy on Mott insulators…

Strongly Correlated Electrons · Physics 2016-12-14 L. Andrew Wray , Shih-Wen Huang , Yuqi Xia , M. Zahid Hasan , Charles Mathy , Hiroshi Eisaki , Zahid Hussain , Yi-De Chuang

Inelastic x-ray scattering (IXS) now a widely used technique for studying the dynamics of electrons in condensed matter. We previously posed a solution to the phase problem for IXS [P. Abbamonte, et. al., Phys. Rev. Lett. {\bf 92}, 237401…

Strongly Correlated Electrons · Physics 2013-05-29 P. Abbamonte , J. P. Reed , Y. I. Joe , Yu Gan , D. Casa

The capability to probe the dispersion of elementary spin, charge, orbital, and lattice excitations has positioned resonant inelastic x-ray scattering (RIXS) at the forefront of photon science. Here we develop the scattering theory for RIXS…

Superconductivity · Physics 2015-04-10 Pasquale Marra , Steffen Sykora , Krzysztof Wohlfeld , Jeroen van den Brink

Recent improvements in instrumentation have established resonant inelastic x-ray scattering (RIXS) as a valuable new probe of the magnetic excitations in the cuprates. This article introduces RIXS, focusing on the Cu $L_3$ resonance, and…

Superconductivity · Physics 2015-02-17 M. P. M. Dean

In the study of dynamic charge order correlations in the cuprates, most high energy-resolution resonant inelastic x-ray scattering (RIXS) measurements have focused on momenta along the high-symmetry directions of the copper oxide plane.…

We present a theory of the resonant inelastic x-ray scattering (RIXS) to study electronic excitations in orbital ordered manganites. The charge and orbital excitations of the Mn 3d electron are caused by the Coulomb interactions in the…

Strongly Correlated Electrons · Physics 2009-10-31 H. Kondo , S. Ishihara , S. Maekawa

We have developed x-ray diffraction measurements with high energy-resolution and accuracy to study water structure at three different temperatures (7, 25 and 66 C) under normal pressure. Using a spherically curved Ge crystal an energy…

Soft Condensed Matter · Physics 2017-09-13 Congcong Huang , K. T. Wikfeldt , D. Nordlund , U. Bergmann , T. McQueen , J. Sellberg , L. G. M. Pettersson , A. Nilsson

The orbital distribution of the spin fluctuation in the iron-based superconductors(IBSs) is the key information needed to understand the magnetism, superconductivity and electronic nematicity in these multi-orbital systems. In this work, we…

Superconductivity · Physics 2021-07-28 Da-Wei Yao , Tao Li

We develop a formalism for calculating resonant inelastic x-ray scattering (RIXS) spectra in systems of itinerant electrons with arbitrary band structures, accounting for the effect of the positively-charged core hole exactly. We apply this…

Superconductivity · Physics 2013-12-24 David Benjamin , Israel Klich , Eugene Demler

Resonant-magnetic x-ray scattering (RMXS) near the vanadium $L_{2,3}$-absorption edges has been used to investigate the low temperature magnetic structure of high quality \bvs\ single crystals. Below $T_N$ = 31 K, the strong resonance…

Strongly Correlated Electrons · Physics 2011-04-27 Ph. Leininger , V. Ilakovac , Y. Joly , E. Schierle , E. Weschke , O. Bunau , H. Berger , J. -P. Pouget , P. Foury-Leylekian

Single crystals of ice Ih, extracted from the subglacial Lake Vostok accretion ice layer (3621 m depth) were investigated by means of diffuse x-ray scattering and inelastic x-ray scattering. The diffuse scattering was identified as mainly…

Materials Science · Physics 2015-09-22 Björn Wehinger , Dmitry Chernyshov , Michael Krisch , Sergey Bulat , Victor Ezhov , Alexeï Bosak