Related papers: Non-linear dynamics of absorption and photo-bleach…
We present a general analysis of the influence of nonlinear optical absorption on terahertz generation via optical difference frequency generation, when reaching for the quantum conversion efficiency limit. By casting the equations…
In acoustics, ultrasonics and in electromagnetic wave propagation, the crossed medium can be often modelled by a linear invariant filter (LIF) which acts on a wide-sense stationary process. Its complex gain follows the Beer-Lambert law i.e…
Accurate knowledge of absorption coefficient of a sample is a prerequisite for measuring the third order optical nonlinearity of materials, which can be a serious limitation for unknown samples. We introduce a method, which measures both…
In a seminal article, Fano predicts that absorption of light occurs preferably with increase of angular momentum. Here we generalize Fano's propensity rule to laser-assisted photoionization, consisting of absorption of an…
The propagation of light in nonlinear media is well described by a $2$D nonlinear Schr\"odinger equation (NLSE) within the paraxial approximation, which is equivalent to the Gross-Pitaesvskii equation (GPE), the mean-field description for…
In a joint theoretical and experimental work the optical properties of azobenzene-functionalized self-assembled monolayers (SAMs) are studied at different molecular packing densities. Our results, based on density-functional and many-body…
The macroscopic shape of liquid crystalline elastomers strongly depends on the order parameter of the mesogenic groups. This order can be manipulated if photoisomerisable groups, e.g. containing N=N bonds, are introduced into the material.…
We theoretically show how slow light in an optofluidic environment facilitates enhanced light-matter interactions, by orders of magnitude. The proposed concept provides strong opportunities for improving existing miniaturized chemical…
We explore the diffusion dynamics of a Brownian microparticle in a lyotropic chromonic liquid crystal (LCLC). In the planarly oriented nematic phase, the microparticle exhibits levitation and anisotropic two-dimensional diffusion. Upon…
Magnetic-free nonreciprocal optical devices that can prevent backscattering of signals are essential for integrated optical information processing. The achieved nonreciprocal behaviors mostly rely on various dispersive effects in optical…
Thermal radiation is strictly governed by Kirchhoff s law to reach thermal equilibrium. The violation of Kirchhoff s law decouples nonreciprocally the equity between absorptivity and emissivity, enabling exotic thermal engineering…
In capillary electrophoresis, sample ions migrate along a micro-capillary filled with a background electrolyte under the influence of an applied electric field. If the sample concentration is sufficiently high, the electrical conductivity…
We present an experimental and computational study of the nonlinear optical response of conduction electrons to intense terahertz (THz) electric field. Our observations (saturable absorption and an amplitude-dependent group refractive…
The absorption of light by materials is one of the most fundamental processes in optics and condensed-matter physics. Here we investigate whether laser light is absorbed by a crystalline material as an electromagnetic wave or as localized…
The dynamics of thin, non-circular droplets evaporating in the diffusion-limited regime are examined. The challenging non-rectilinear mixed-boundary problem this poses is solved using a novel asymptotic approach and an asymptotic expansion…
We provide the first demonstration of nonlinear self-trapping of light in solutions of food coloring dyes, leading to dirt cheap soliton waveguides. The optical self-focusing nonlinearity observed in such solutions is attributed to the…
The photoisomerization reaction of the retinal chromophore in rhodopsin was computationally studied using a two-state two-mode model coupled to thermal baths. Reaction quantum yields at the steady state (10 ps and beyond) were found to be…
Experimental and numerical investigation of single-beam and pump-probe interaction with a resonantly absorbing dense extended medium under strong and weak field-matter coupling is presented. Significant probe beam amplification and conical…
We study coherent perfect absorption (CPA) of light in a Kerr nonlinear metal-dielectric composite medium, illuminated from the opposite ends. Elementary symmetry considerations reveal that equality of the incident light intensities is a…
We use molecular dynamics simulations to unravel the physics underpinning the light-induced density changes caused by the dynamic trans-cis-trans isomerization cycles of azo-mesogens embedded in a liquid crystal polymer network, an…