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We show that a combination of linear absorption spectroscopy, hyper-Rayleigh scattering, and a theoretical analysis using sum rules to reduce the size of the parameter space leads to a prediction of the two-photon absorption cross-section…

The emergent photoactive materials through photochemistry make it possible to directly convert photon energy to mechanical work. There is much recent work in developing appropriate materials and a promising new system is semi-crystalline…

Soft Condensed Matter · Physics 2021-03-24 Ruobing Bai , Eric Ocegueda , Kaushik Bhattacharya

We study the absorptive and dispersive properties of Doppler-broadened atomic media as a function of detuning. Beginning from the exact lineshape calculated for a two-level atom, a series of approximations to the electric susceptibility are…

Atomic Physics · Physics 2009-08-14 Paul Siddons , Charles S Adams , Ifan G Hughes

X-ray absorption by matter has long been described by the famous Beer-Lambert law. Here we show how this fundamental law needs to be modified for high-intensity coherent x-ray pulses, now available at x-ray free electron lasers, due to the…

Materials Science · Physics 2015-09-09 Joachim Stöhr , Andreas Scherz

We propose a methodology to detect weak Lorentz-violating (LV) backgrounds through the nonlinear shift photocurrent in noncentrosymmetric crystals. Using a spinful Rice--Mele model, we show that a LV background induces a momentum-odd…

Mesoscale and Nanoscale Physics · Physics 2026-04-24 Guilherme J. Inacio , Nathanael N. Batista , Wesley Spalenza , Humberto Belich , Juan José Palacios , Wendel S. Paz

Absorption imaging with quasi-resonant laser light is a commonly used technique to probe ultra-cold atomic gases in various geometries. Here we investigate some non-trivial aspects of this method when it is applied to in situ diagnosis of a…

Quantum Gases · Physics 2015-06-03 L. Chomaz , L. Corman , T. Yefsah , R. Desbuquois , J. Dalibard

Entanglement can modify light-matter interaction effects and, conversely, these interactions can change the non-classical correlations present in the system. We present an example where these mutual connections can be discussed in a simple…

Quantum Physics · Physics 2018-12-26 Pedro Sancho

We experimentally investigate a method of directly characterizing the photon number distribution of nonclassical light beams that is tolerant to losses and makes use only of standard binary detectors. This is achieved in a single…

Quantum Physics · Physics 2007-05-23 Daryl Achilles , Christine Silberhorn , Ian A. Walmsley

Theory of light absorption and circular photocurrent in Weyl semimetals is developed for arbitrary large light intensities with account for both elastic and inelastic relaxation processes of Weyl fermions. The direct optical transition rate…

Mesoscale and Nanoscale Physics · Physics 2019-10-21 N. V. Leppenen , E. L. Ivchenko , L. E. Golub

Recently, the photon absorption attracts lots of interest and plays an important role in a variety of applications. Here, we propose a valuable scheme to investigate the perfect photon absorption in a hybrid atom-optomechanical system both…

Quantum Physics · Physics 2017-04-19 Yang Zhang , Amjad Sohail , Chang-shui Yu

The photoisomerization of chromophores embedded in biological environments is of high importance for biomedical applications, but it is still challenging to define the photoisomerization mechanism both experimentally and computationally. We…

Soft Condensed Matter · Physics 2024-10-10 Silvio Osella , Giovanni Granucci , Maurizio Persico , Stefan Knippenberg

We consider the homogenization of a model of reactive flows through periodic porous media involving a single solute which can be absorbed and desorbed on the pore boundaries. This is a system of two convection-diffusion equations, one in…

Analysis of PDEs · Mathematics 2014-12-30 Grégoire Allaire , Harsha Hutridurga

Saturable absorption is a non-perturbative nonlinear optical phenomenon that plays a pivotal role in the generation of ultrafast light pulses. Here we show that this effect emerges in graphene at unprecedentedly low light intensities, thus…

Mesoscale and Nanoscale Physics · Physics 2017-03-15 A. Marini , J. D. Cox , F. J. Garcia de Abajo

Artificial neural networks have revolutionized fields from computer vision to natural language processing, yet their growing energy and computational demands threaten future progress. Optical neural networks promise greater speed,…

Optics · Physics 2025-08-18 Bofeng Liu , Xu Mei , Sadman Shafi , Tunan Xia , Iam-Choon Khoo , Zhiwen Liu , Xingjie Ni

When an electromagnetic wave is obliquely incident on an inhomogeneous high density plasma, it will be absorbed resonantly as long as it is polarized in the plane of incidence and has an electric field component along the plasma electron…

Plasma Physics · Physics 2009-01-27 S J Pestehe , M Mohammadnejad

We propose a new method to measure the absolute photon absorption cross section of neutral molecules in a molecular beam. It is independent of our knowledge of the particle beam density, nor does it rely on photo-induced fragmentation or…

Quantum Physics · Physics 2008-12-31 Stefan Nimmrichter , Klaus Hornberger , Hendrik Ulbricht , Markus Arndt

When the interaction between a molecular system and confined light modes in an optical or plasmonic cavity is strong enough to overcome the dissipative process, hybrid light-matter states (polaritons) become the fundamental excitations in…

Mesoscale and Nanoscale Physics · Physics 2020-01-08 Yu Zhang , Tammie Nelson , Sergei Tretiak

We present a self-consistent theory, as well as an illustrative application to a realistic system, of phase control of photoabsorption in an optically dense medium. We demonstrate that, when propagation effects are taken into consideration,…

Quantum Physics · Physics 2009-11-06 David Petrosyan , P. Lambropoulos

Light-induced chemical processes are ubiquitous in nature and have widespread technological applications. For example, photoisomerization can allow a drug with a photo-switchable scaffold such as azobenzene to be activated with light. In…

Chemical Physics · Physics 2022-10-12 Simon Axelrod , Eugene Shakhnovich , Rafael Gómez-Bombarelli

Specific features of nonlinear interference processes at quantum transitions in near- and fully-resonant optically-dense Doppler-broadened medium are studied. The feasibility of overcoming of the fundamental limitation on a…

Quantum Physics · Physics 2009-11-11 A. K. Popov , S. A. Myslivets , Thomas F. George