Related papers: Non-linear dynamics of absorption and photo-bleach…
We show that a combination of linear absorption spectroscopy, hyper-Rayleigh scattering, and a theoretical analysis using sum rules to reduce the size of the parameter space leads to a prediction of the two-photon absorption cross-section…
The emergent photoactive materials through photochemistry make it possible to directly convert photon energy to mechanical work. There is much recent work in developing appropriate materials and a promising new system is semi-crystalline…
We study the absorptive and dispersive properties of Doppler-broadened atomic media as a function of detuning. Beginning from the exact lineshape calculated for a two-level atom, a series of approximations to the electric susceptibility are…
X-ray absorption by matter has long been described by the famous Beer-Lambert law. Here we show how this fundamental law needs to be modified for high-intensity coherent x-ray pulses, now available at x-ray free electron lasers, due to the…
We propose a methodology to detect weak Lorentz-violating (LV) backgrounds through the nonlinear shift photocurrent in noncentrosymmetric crystals. Using a spinful Rice--Mele model, we show that a LV background induces a momentum-odd…
Absorption imaging with quasi-resonant laser light is a commonly used technique to probe ultra-cold atomic gases in various geometries. Here we investigate some non-trivial aspects of this method when it is applied to in situ diagnosis of a…
Entanglement can modify light-matter interaction effects and, conversely, these interactions can change the non-classical correlations present in the system. We present an example where these mutual connections can be discussed in a simple…
We experimentally investigate a method of directly characterizing the photon number distribution of nonclassical light beams that is tolerant to losses and makes use only of standard binary detectors. This is achieved in a single…
Theory of light absorption and circular photocurrent in Weyl semimetals is developed for arbitrary large light intensities with account for both elastic and inelastic relaxation processes of Weyl fermions. The direct optical transition rate…
Recently, the photon absorption attracts lots of interest and plays an important role in a variety of applications. Here, we propose a valuable scheme to investigate the perfect photon absorption in a hybrid atom-optomechanical system both…
The photoisomerization of chromophores embedded in biological environments is of high importance for biomedical applications, but it is still challenging to define the photoisomerization mechanism both experimentally and computationally. We…
We consider the homogenization of a model of reactive flows through periodic porous media involving a single solute which can be absorbed and desorbed on the pore boundaries. This is a system of two convection-diffusion equations, one in…
Saturable absorption is a non-perturbative nonlinear optical phenomenon that plays a pivotal role in the generation of ultrafast light pulses. Here we show that this effect emerges in graphene at unprecedentedly low light intensities, thus…
Artificial neural networks have revolutionized fields from computer vision to natural language processing, yet their growing energy and computational demands threaten future progress. Optical neural networks promise greater speed,…
When an electromagnetic wave is obliquely incident on an inhomogeneous high density plasma, it will be absorbed resonantly as long as it is polarized in the plane of incidence and has an electric field component along the plasma electron…
We propose a new method to measure the absolute photon absorption cross section of neutral molecules in a molecular beam. It is independent of our knowledge of the particle beam density, nor does it rely on photo-induced fragmentation or…
When the interaction between a molecular system and confined light modes in an optical or plasmonic cavity is strong enough to overcome the dissipative process, hybrid light-matter states (polaritons) become the fundamental excitations in…
We present a self-consistent theory, as well as an illustrative application to a realistic system, of phase control of photoabsorption in an optically dense medium. We demonstrate that, when propagation effects are taken into consideration,…
Light-induced chemical processes are ubiquitous in nature and have widespread technological applications. For example, photoisomerization can allow a drug with a photo-switchable scaffold such as azobenzene to be activated with light. In…
Specific features of nonlinear interference processes at quantum transitions in near- and fully-resonant optically-dense Doppler-broadened medium are studied. The feasibility of overcoming of the fundamental limitation on a…