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The recently proposed center-focused post-processing procedure [Phys. Rev. Research 2, 033476 (2020)] of cellular dynamical mean-field theory suggests that central sites of large impurity clusters are closer to the exact solution of the…

Strongly Correlated Electrons · Physics 2024-02-28 Michael Meixner , Henri Menke , Marcel Klett , Sarah Heinzelmann , Sabine Andergassen , Philipp Hansmann , Thomas Schäfer

DFT is used throughout nanoscience, especially when modeling spin-dependent properties that are important in spintronics. But standard quantum chemical methods (both CCSD(T) and self-consistent semilocal density functional calculations)…

Chemical Physics · Physics 2017-08-29 Suhwan Song , Min-Cheol Kim , Eunji Sim , Anouar Benali , Olle Heinonen , Kieron Burke

In this work we present a multi-orbital form of the Two-Particle Self-Consistent approach (TPSC), here the effective local and static irreducible interaction vertices are determined by means of the Dynamical Mean-Field Theory (DMFT). This…

Strongly Correlated Electrons · Physics 2023-06-16 Karim Zantout , Steffen Backes , Aleksandar Razpopov , Dominik Lessnich , Roser Valenti

Quantitative descriptions of strongly correlated materials pose a considerable challenge in condensed matter physics and chemistry. A promising approach to address this problem is quantum embedding methods. In particular, the dynamical…

Quantum Physics · Physics 2024-05-07 Rihito Sakurai , Wataru Mizukami , Hiroshi Shinaoka

We applied a mean-field approach associated to Monte Carlo simulations in order to study the spin-1 ferromagnetic Blume-Capel model in the square and the linear lattice. This new technique, which we call MFT-MC, determines the molecular…

Statistical Mechanics · Physics 2016-07-06 J. Roberto Viana , Octavio D. Rodriguez Salmon , Minos A. Neto

Near-term quantum processors are limited in terms of the number of qubits and gates they can afford. They nevertheless give unprecedented access to programmable quantum systems that can efficiently, although imperfectly, simulate quantum…

Strongly Correlated Electrons · Physics 2025-11-25 Thomas Ayral

In the pursuit of accurate descriptions of strongly correlated quantum many-body systems, dynamical mean-field theory (DMFT) has been an invaluable tool for elucidating the spectral properties and quantum phases of both phenomenological…

Strongly Correlated Electrons · Physics 2019-10-07 Carlos Mejuto-Zaera , Norm M. Tubman , K. Birgitta Whaley

Strongly correlated quantum impurity problems appear in a wide variety of contexts ranging from nanoscience and surface physics to material science and the theory of strongly correlated lattice models, where they appear as auxiliary systems…

Strongly Correlated Electrons · Physics 2013-02-19 Hartmut Hafermann , Philipp Werner , Emanuel Gull

Theoretical methods that are accurate for both short-distance observables and long-wavelength collective modes are still being developed for the Hubbard model. Here, we benchmark an approach that combines dynamical mean-field theory (DMFT)…

Strongly Correlated Electrons · Physics 2023-03-09 N. Martin , C. Gauvin-Ndiaye , A. -M. S. Tremblay

An acceleration of continuous time quantum Monte Carlo (CTQMC) methods is a potentially interesting branch of work as they are matchless as impurity solvers of a density functional theory in combination with a dynamical mean field theory…

Strongly Correlated Electrons · Physics 2019-08-07 Taegeun Song , Hunpyo Lee

Classical density functional theory (DFT) of fluids is a valuable tool to analyze inhomogeneous fluids. However, few numerical solution algorithms for three-dimensional systems exist. Here we present an efficient numerical scheme for fluids…

In this paper, we investigate the use of multilevel Monte Carlo (MLMC) methods for estimating the expectation of discretized random fields. Specifically, we consider a setting in which the input and output vectors of numerical simulators…

We develop a nanoscale dynamical mean-field theory (nano-DMFT) to deal with strong Coulomb interaction effects in physical systems that are intermediate in size between atoms and bulk materials, taking into account the tunneling into nearby…

Strongly Correlated Electrons · Physics 2009-11-13 Serge Florens

We present a detailed study of the energetics of water clusters (H$_2$O)$_n$ with $n \le 6$, comparing diffusion Monte Carlo (DMC) and approximate density functional theory (DFT) with well converged coupled-cluster benchmarks. We use the…

Materials Science · Physics 2015-06-04 M. J. Gillan , F. R. Manby , M. D. Towler , D. Alfè

Quantum computers open up new avenues for modelling the physical properties of materials and molecules. Density Functional Theory (DFT) is the gold standard classical algorithm for predicting these properties, but relies on approximations…

Quantum Physics · Physics 2024-02-29 Evan Sheridan , Lana Mineh , Raul A. Santos , Toby Cubitt

In a previous contribution (E. Canc\`es, A. Kirsch and S. Perrin--Roussel, arXiv:2406.03384), we have proven the existence of a solution to the Dynamical Mean-Field Theory (DMFT) equations under the Iterated Perturbation Theory (IPT-DMFT)…

Numerical Analysis · Mathematics 2025-05-28 E. Cancès , A. Kirsch , S. Perrin--Roussel

The Iterated Perturbation Theory (IPT) equations of the Dynamical Mean Field Theory (DMFT) for the half-filled Hubbard model, are solved on nearly real frequencies at various values of the Hubbard parameters $U$, to investigate the nature…

Strongly Correlated Electrons · Physics 2008-08-05 M. B. Fathi , S. A. Jafari

We present an efficient impurity solver for the dynamical mean-field theory (DMFT). It is based on the separation of bath degrees of freedom into the low energy and the high energy parts. The former is solved exactly using exact…

Strongly Correlated Electrons · Physics 2017-01-02 Hengyue Li , Ning-Hua Tong

Fixed-node diffusion Monte Carlo (DMC) is a stochastic algorithm for finding the lowest energy many-fermion wave function with the same nodal surface as a chosen trial function. It has proved itself among the most accurate methods available…

Condensed Matter · Physics 2009-10-31 W. M. C. Foulkes , Randolph Q. Hood , R. J. Needs

Approximating a probability distribution using a set of particles is a fundamental problem in machine learning and statistics, with applications including clustering and quantization. Formally, we seek a weighted mixture of Dirac measures…

Machine Learning · Statistics 2026-04-24 Ayoub Belhadji , Daniel Sharp , Youssef Marzouk