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Silicon photonics lacks a second-order nonlinear optical response in general because the typical constituent materials are centro-symmetric and lack inversion symmetry, which prohibits second-order nonlinear processes such as second…

Optics · Physics 2022-07-21 Xiyuan Lu , Gregory Moille , Ashutosh Rao , Daron Westly , Kartik Srinivasan

We study the second-harmonic generation in left-handed metamaterials with a quadratic nonlinear response. We demonstrate a novel type of the exact phase matching between the backward propagating wave of the fundamental frequency and the…

Optics · Physics 2009-11-11 Ilya V. Shadrivov , Alexander A. Zharov , Yuri S. Kivshar

In this paper we explore the capabilities of MoS2 and WS2 2D monolayers to produce radiation in the terahertz range by generation of high-order harmonics. This phenomenon, which is a result of the non-linear response of the electronic…

Applied Physics · Physics 2024-02-13 Jose Manuel Iglesias , Elena Pascual , Maria J. Martin , Raul Rengel

Second-harmonic generation is of paramount importance in several fields of science and technology, including frequency conversion, self-referencing of frequency combs, nonlinear spectroscopy and pulse characterization. Advanced…

Mid-infrared nanophotonics can be realized using sub-diffractional light localization and field enhancement with surface phonon polaritons in polar dielectric materials. We experimentally demonstrate second harmonic generation due to the…

The reversible phase transition induced by femtosecond laser excitation of Gallium has been studied by measuring the dielectric function at 775 nm with ~ 200 fs temporal resolution. The real and imaginary parts of the transient dielectric…

Optics · Physics 2009-11-10 O. P. Uteza , E. G. Gamaly , A. V. Rode , M. Samoc , B. Luther-Davies

Nonlinear frequency conversion plays a crucial role in advancing the functionality of next-generation optical systems. Portable metrology references and quantum networks will demand highly efficient second-order nonlinear devices, and the…

Dynamical control of the nonlinear optical properties of solids -- with light itself -- will be essential for future ultrafast photonic technologies. Previously, methods to modulate nonlinear processes including second-harmonic generation…

Control over the spatial coherence, wavefront, and focusability of emitted light relies on understanding the intrinsic phase of the emission process, and vice versa, measuring phase can reveal insights about microscopic generation…

By combining analytical and numerical approaches, we study resonantly enhanced second-harmonic generation (SHG) by individual high-index dielectric nanoparticles made of centrosymmetric materials. Considering both bulk and surface…

Optics · Physics 2018-01-08 Daria Smirnova , Alexander I. Smirnov , Yuri S. Kivshar

Remarkable optical and electrical properties of two-dimensional (2D) materials, such as graphene and transition-metal dichalcogenide (TMDC) monolayers, offer vast technological potential for novel and improved optoelectronic nanodevices,…

Optics · Physics 2016-07-22 Martin Weismann , Nicolae C. Panoiu

We present a study of the second-order nonlinear optical properties of metal-based metamaterials. A hydrodynamic model for electronic response is used, in which nonlinear surface contributions are expressed in terms of the bulk…

Second and third harmonic generation in the opaque region of a GaAs wafer is experimentally observed both in transmission and reflection. These harmonic components can propagate through an opaque material as long as the pump is tuned to a…

Optics · Physics 2019-05-13 L. Rodriguez , J. Trull , M. Scalora , R. Vilaseca , C. Cojocaru

We study the linear- and nonlinear-optical lineshapes of metal nanoparticles (theory) and metallic photonic crystal slabs (experiment and theory). For metal nanoparticle ensembles, we show analytically and numerically that femtosecond…

Materials Science · Physics 2007-05-23 M. W. Klein , T. Tritschler , M. Wegener , S. Linden

Nonlinear second harmonic optical activity of graphene covering a gold photon sieve was determined for different polarizations. The photon sieve consists of a subwavelength gold nanohole array placed on glass. It combines the benefits of…

Mesoscale and Nanoscale Physics · Physics 2016-01-14 Michael Lobet , Michael Sarrazin , Francesca Cecchet , Nicolas Reckinger , Alexandru Vlad , Jean-François Colomer , Dan Lis

Monolayer transition metal dichalcogenides, coupled to metal plasmonic nanocavities, have recently emerged as new platforms for strong light-matter interactions. These systems are expected to have nonlinear optical properties that will…

We demonstrate second harmonic generation (SHG) in an $x$-cut congruent lithium niobate (LN) whispering gallery mode resonator. We first show theoretically that independent control of the coupling of the pump and signal modes is optimal for…

Two-dimensional materials constitute an exciting platform for nonlinear optics with large nonlinearities that are tunable by gating. Hence, gate-tunable harmonic generation and intensity-dependent refraction have been observed in e.g.…

Mesoscale and Nanoscale Physics · Physics 2019-05-15 F. Hipolito , Darko Dimitrovski , T. G. Pedersen

Strong field-confinement, long-lifetime resonances, and slow-light effects suggest that meta surfaces are a promising tool for nonlinear optical applications. These nanostructured devices have been utilized for relatively high efficiency…

We derive a low-energy theory for edge states in transition metal dichalcogenide monolayers for a two-band $\bm{kp}$-Hamiltonian in case of uncoupled valleys. In the absence of spin-orbit interaction at the edge, these states possess a…

Mesoscale and Nanoscale Physics · Physics 2016-09-29 V. V. Enaldiev
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