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Related papers: Diffusion quantum Monte Carlo study of three-dimen…

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Three-dimensional (3D) excitonic complexes influence the optoelectronic properties of bulk semiconductors. More generally, correlated few-particle molecules and ions, held together by pairwise Coulomb potentials, play a fundamental role in…

Materials Science · Physics 2022-12-26 F Marsusi , E. Mostaani , N. D. Drummond

We present an algorithm for rigid body diffusion Monte Carlo with importance sampling, which is based on a rigorous short-time expansion of the Green's function for rotational motion in three dimensions. We show that this short-time…

Computational Physics · Physics 2009-11-07 Alexandra Viel , Mehul V. Patel , Parhat Niyaz , K. Birgitta Whaley

We present results of Diffusion Monte Carlo calculations for a system of solid ortho-D_2 at different densities, for pressure ranging from 0 up to 350MPa. We compare the equation of state obtained using two of the most used effective…

Other Condensed Matter · Physics 2009-11-11 Francesco Operetto , Francesco Pederiva

We present density-functional theory (DFT) and quantum Monte Carlo (QMC) calculations designed to resolve experimental and theoretical controversies over the optical properties of H-terminated C nanoparticles (diamondoids). The QMC results…

Materials Science · Physics 2008-01-03 N. D. Drummond , A. J. Williamson , R. J. Needs , G. Galli

Electrons can form an ordered solid crystal phase ascribed to the interplay between Coulomb repulsion and kinetic energy. Tuning these energy scales can drive a phase transition from electron solid to liquid, i.e. melting of Wigner crystal.…

We present a systematic and comprehensive study of finite-size effects in diffusion quantum Monte Carlo calculations of metals. Several previously introduced schemes for correcting finite-size errors are compared for accuracy and efficiency…

Materials Science · Physics 2016-08-23 Sam Azadi , Matthew Foulkes

We show that the liquid-to-crystal quantum phase transition in the Rokhsar--Kivelson dimer model on the two-dimensional triangular lattice occurs as a condensation of vortex-like excitations called ``visons''. This conclusion is drawn from…

Strongly Correlated Electrons · Physics 2007-10-25 Arnaud Ralko , Michel Ferrero , Federico Becca , Dmitri Ivanov , Frederic Mila

We modify the reweighting factor of the projector used in diffusion Monte Carlo to reduce the time-step error of the total energy. Further, we present a reweighting scheme that has the desirable feature that it is exactly size-consistent,…

Chemical Physics · Physics 2024-03-18 Tyler A. Anderson , Manolo C. Per , C. J. Umrigar

We apply diffusion quantum Monte Carlo (DMC) to a broad set of solids, benchmarking the method by comparing bulk structural properties (equilibrium volume and bulk modulus) to experiment and DFT based theories. The test set includes…

Materials Science · Physics 2015-06-17 Luke Shulenburger , Thomas R. Mattsson

The phase diagram of quantum electron bilayers in zero magnetic field is obtained using density functional theory. For large electron densities the system is in the liquid phase, while for smaller densities the liquid may freeze (Wigner…

Condensed Matter · Physics 2009-10-28 G. Goldoni , F. M. Peeters

The ground state energy and the lowest excitations of a two dimensional Wigner crystal in a perpendicular magnetic field with one and two electrons per cell is investigated. In case of two electrons per lattice site, the interaction of the…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 M. Taut

We study numerically the low temperature behavior of a one-dimensional Bose gas trapped in an optical lattice. For a sufficient number of particles and weak repulsive interactions, we find a clear regime of temperatures where density…

Statistical Mechanics · Physics 2013-05-29 C. Gils , L. Pollet , A. Vernier , F. Hebert , G. G. Batrouni , M. Troyer

A floating Wigner crystal differs from the standard one by a spatial averaging over positions of the Wigner-crystal lattice. It has the same internal structure as the fixed crystal, but contrary to it, takes into account rotational and/or…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 S. A. Mikhailov , K. Ziegler

The local environment and the energetic properties of one $^3$He atom solved in bulk superfluid $^4$He are studied by means of the diffusion Monte Carlo method. The chemical potential of the $^3$He impurity is calculated with a generalized…

Statistical Mechanics · Physics 2009-10-31 J. Boronat , J. Casulleras

A theoretical study is reported of the molecular-to-atomic transition in solid hydrogen at high pressure. We use the diffusion quantum Monte Carlo method to calculate the static lattice energies of the competing phases and a…

Materials Science · Physics 2014-04-23 Sam Azadi , Bartomeu Monserrat , W. M. C. Foulkes , R. J. Needs

Bosonic van der Waals clusters of sizes three, four and five are studied by diffusion quantum Monte-Carlo techniques. In particular we study the unbinding transition, the ultra-quantum limit where the ground state ceases to exist as a bound…

chem-ph · Physics 2019-08-15 M. Meierovich , A. Mushinski , M. P. Nightingale

The scattering from crystals can be divided into two parts: Bragg scattering and diffuse scattering. The analysis of Bragg diffraction data gives only information about the average structure of the crystal. The interpretation of diffuse…

Materials Science · Physics 2007-05-23 Th. Proffen , T. R. Welberry

Nobel metals that are deposited on a polymer surface exhibit surface diffusion and diffusion into the bulk. At the same time the metal atoms tend to form clusters because their cohesive energy is about two orders of magnitude higher than…

Plasma Physics · Physics 2011-12-30 L. Rosenthal , A. Filinov , M. Bonitz , V. Zaporojtchenko , F. Faupel

The quantum Monte Carlo methods represent a powerful and broadly applicable computational tool for finding very accurate solutions of the stationary Schroedinger equation for atoms, molecules, solids and a variety of model systems. The…

Computational Physics · Physics 2011-01-28 Jindrich Kolorenc , Lubos Mitas

The sampling of the configuration space in diffusion Monte Carlo (DMC) is done using walkers moving randomly. In a previous work on the Hubbard model [\href{https://doi.org/10.1103/PhysRevB.60.2299}{Assaraf et al.~Phys.~Rev.~B \textbf{60},…

Strongly Correlated Electrons · Physics 2023-01-19 Roland Assaraf , Emmanuel Giner , Vijay Gopal Chilkuri , Pierre-François Loos , Anthony Scemama , Michel Caffarel