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We have performed large-scale Lennard-Jones molecular dynamics simulations of homogeneous vapor-to-liquid nucleation, with $10^9$ atoms. This large number allows us to resolve extremely low nucleation rates, and also provides excellent…

Chemical Physics · Physics 2014-04-07 Raymond Angélil , Jürg Diemand , Kyoko K. Tanaka , Hidekazu Tanaka

This paper exposes a novel exploratory formalism, which end goal is the numerical simulation of the dynamics of a cloud of particles weakly or strongly coupled with a turbulent fluid. Giventhe large panel of expertise of the list of…

Analysis of PDEs · Mathematics 2019-10-21 Ludovic Goudenège , Adam Larat , Julie Llobell , Marc Massot , David Mercier , Olivier Thomine , Aymeric Vié

Recent results have shown that there is an acceleration in the spread of the size distribution of droplet populations in the region bordering the cloud and undersaturated ambient. We have analyzed the supersaturation balance in this region,…

Atmospheric and Oceanic Physics · Physics 2022-06-13 Ludovico Fossà , Shahbozbek Abdunabiev , Mina Golshan , Daniela Tordella

We discuss molecular cloud formation by large-scale supersonic compressions in the diffuse warm neutral medium (WNM). Initially, a shocked layer forms, and within it, a thin cold layer. An analytical model and high-resolution 1D simulations…

Strongly first-order phase transitions, i.e., those with a large order parameter, are characterized by a considerable supercooling and high velocities of phase transition fronts. A very strong phase transition may have important…

Cosmology and Nongalactic Astrophysics · Physics 2017-04-26 Ariel Megevand , Santiago Ramirez

We consider the dynamics of diffusing particles in one space dimension with annihilation on collision and nucleation (creation of particles) with constant probability per unit time and length. The cases of nucleation of single particles and…

Statistical Mechanics · Physics 2009-11-07 S. Habib , K. Lindenberg , G. Lythe , C. Molina-Paris

We present results from large-scale molecular dynamics (MD) simulations of homogeneous vapor-to-liquid nucleation. The simulations contain between one and eight billion Lennard-Jones (LJ) atoms, covering up to 1.2 {\mu}s (56 million…

Chemical Physics · Physics 2013-08-22 Jürg Diemand , Raymond Angélil , Kyoko K. Tanaka , Hidekazu Tanaka

Under continuous laser irradiation, noble metal nanoparticles immersed in water can quickly heat up, leading to the nucleation of so-called plasmonic bubbles. In this work, we want to further understand the bubble nucleation and growth…

The heterogeneous condensation of a Lennard-Jones vapor onto a nanoscale seed particle is studied using molecular dynamics simulations. Measuring the nucleation rate and the height of the free energy barrier using the mean first passage…

Soft Condensed Matter · Physics 2015-05-27 Levent Inci , Richard K. Bowles

Anomalous coarsening in far-from equilibrium one-dimensional systems is investigated by simulation and analytic techniques. The minimal hard core particle (exclusion) models contain mechanisms of aggregated particle diffusion, with rates…

Statistical Mechanics · Physics 2009-11-10 Fabio D. A. Aarao Reis , Robin B. Stinchcombe

Demixing of binary fluids subjected to slow temperature ramps shows repeated waves of nucleation which arise as a consequence of the competition between generation of supersaturation by the temperature ramp and relaxation of supersaturation…

Statistical Mechanics · Physics 2012-10-16 Izabella J. Benczik , Jürgen Vollmer

We have developed an original setup using microfluidic tools allowing one to produce continuously monodisperse microreactors ($\approx 100$ nL), and to control their temperatures as they flow in the microdevice. With a specific…

Soft Condensed Matter · Physics 2009-11-11 Philippe Laval , Jean-Baptiste Salmon , Mathieu Joanicot

We present high resolution ($1024^3$) simulations of super-/hyper-sonic isothermal hydrodynamic turbulence inside an interstellar molecular cloud (resolving scales of typically 20 -- 100 AU), including a multi-disperse population of dust…

Astrophysics of Galaxies · Physics 2018-12-19 Lars Mattsson , Akshay Bhatnagar , Fred A. Gent , Beatriz Villarroel

We theoretically investigate the nucleation of liquid droplets from vapor in the presence of a charged spherical particle. Due to field gradients, sufficiently close to the critical point of the vapor--gas system, the charge destabilizes…

Chemical Physics · Physics 2021-11-04 Roni Kroll , Yoav Tsori

Monolayer cluster growth in far-from-equilibrium systems is investigated by applying simulation and analytic techniques to minimal hard core particle (exclusion) models. The first model (I), for post-deposition coarsening dynamics, contains…

Statistical Mechanics · Physics 2009-11-10 F. D. A. Aarao Reis , R. B. Stinchcombe

We present results from direct, large-scale molecular dynamics (MD) simulations of homogeneous bubble (liquid-to-vapor) nucleation. The simulations contain half a billion Lennard-Jones (LJ) atoms and cover up to 56 million time-steps. The…

Chemical Physics · Physics 2015-06-23 Jürg Diemand , Raymond Angélil , Kyoko K. Tanaka , Hidekazu Tanaka

We consider the nucleation process associated with capillary condensation of a vapor in a hydrophobic cylindrical pore (capillary evaporation). The liquid-vapor transition is described within the framework of a simple lattice model. The…

Materials Science · Physics 2007-05-23 Anthony Saugey , Lyderic Bocquet , J. -L. Barrat

The understanding of the fusion probability is of particular importance to reveal the mechanism of producing superheavy elements. We present a microscopic study of the compound nucleus formation by combining time-dependent density…

Nuclear Theory · Physics 2022-07-27 Xiang-Xiang Sun , Lu Guo

The growth of homogeneously nucleated droplets in water vapor at the fixed temperatures T=273, 283, 293, 303, 313, 323, 333, 343, 353, 363 and 373 K (the pressure $p=1$ atm.) is investigated on the basis of the coarse-grained molecular…

Soft Condensed Matter · Physics 2012-12-06 Anatolii V. Mokshin , Bulat N. Galimzyanov

Turbulent mixing and entrainment at the boundary of a cloud is studied by means of direct numerical simulations that couple the Eulerian description of the turbulent velocity and water vapor fields with a Lagrangian ensemble of cloud water…

Fluid Dynamics · Physics 2013-10-14 Bipin Kumar , Joerg Schumacher , Raymond A. Shaw