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We consider resonant transport through a molecular quantum dot coupled to a local vibration mode. Applying the non-equilibrium Green function technique in the polaron representation, we develop a non-perturbative scheme to calculate the…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Alex Zazunov , Thierry Martin

We evaluate the shifts imparted to vibrational and rotational levels of a linear molecule by a nonresonant laser field at intensities of up to 10^12 W/cm^2. Both types of shift are found to be either positive or negative, depending on the…

Chemical Physics · Physics 2015-03-14 Mikhail Lemeshko , Bretislav Friedrich

We develop a classical mapping approach suitable to describe vibrationally coupled charge transport in molecular junctions based on the Cartesian mapping for many-electron systems [J. Chem. Phys. 137, 154107 (2012)]. To properly describe…

Strongly Correlated Electrons · Physics 2015-06-18 Bin Li , Eli. Y. Wilner , Michael Thoss , Eran Rabani , William H. Miller

We study theoretically the transport properties of a molecular two level system with large electron-vibron coupling in the Coulomb blockade regime. We show that when the electron-vibron coupling induces polaron states, the current-voltage…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Gregers A. Kaat , Karsten Flensberg

A recent experiment reports a non-local spin-signal that shows oscillatory behavior as a function of gate voltage when the contacts are magnetized along the direction of current flow, but not when they are magnetized perpendicular to the…

Mesoscale and Nanoscale Physics · Physics 2011-12-05 A. N. M. Zainuddin , S. Hong , L. Siddiqui , S. Datta

We calculate the non-linear tunneling current through a molecule with two electron-accepting orbitals which interact with an intramolecular vibration. We investigate the interplay between Coulomb blockade and non-equilibrium…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Katja C. Nowack , Maarten R. Wegewijs

We extend the theory of weakly coupled oscillators to incorporate slowly varying inputs and parameters. We employ a combination of regular perturbation and an adiabatic approximation to derive equations for the phase-difference between a…

Dynamical Systems · Mathematics 2016-03-09 Youngmin Park , Bard Ermentrout

We study the negative correction to the quantized value $2e^2/h$ of the conductance of a quantum point contact due to the backscattering of electrons by acoustic phonons. The correction shows activated temperature dependence and also gives…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Georg Seelig , K. A. Matveev

A model of a superconducting tunnel junction coupled to a mechanical oscillator is studied at zero temperature in the case of linear coupling between the oscillator and tunneling electrons. It is found that the Josephson current flowing…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Jian-Xin Zhu , Z. Nussinov , A. V. Balatsky

Shuttle-like mechanism of electron transport through a single level vibrating quantum dot is considered in the regime of strong electromechanical coupling. It is shown that the increment of shuttle instability is a nonmonotonic function of…

Mesoscale and Nanoscale Physics · Physics 2013-02-07 Gleb A. Skorobagatko , Ilya V. Krive , Robert I. Shekhter

The capability to excite, probe, and manipulate vibrational modes is essential for understanding and controlling chemical reactions at the molecular level. Recent advancements in tip-enhanced Raman spectroscopies have enabled the probing of…

We theoretically investigate the transport properties of a molecule embedded in one arm of a mesoscopic Aharonov-Bohm interferometer. Due to the presence of phonons the molecule level position ($\epsilon_d$) and the electron-electron…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Jong Soo Lim , Rosa Lopez , Gloria Platero , Pascal Simon

We study the response of a weakly damped vibrational mode of a nanostring resonator to a moderately strong resonant driving force. Because of the geometry of the experiment, the studied flexural vibrations lack inversion symmetry. As we…

Mesoscale and Nanoscale Physics · Physics 2021-11-01 J. S. Ochs , G. Rastelli , M. Seitner , M. I. Dykman , E. M. Weig

The thermoelectric properties of a molecular junction model, appropriate for large molecules such as fullerenes, are studied within a non-equilibrium adiabatic approach in the linear regime at room temperature. A self-consistent calculation…

Mesoscale and Nanoscale Physics · Physics 2014-09-26 C. A. Perroni , D. Ninno , V. Cataudella

The treatment of the previous paper is extended to molecular wires. Specifically, the effect of electron-vibrational interactions on the electronic transport induced by femtosecond $\omega+2\omega$ laser fields along unbiased molecular…

Quantum Physics · Physics 2009-11-13 Ignacio Franco , Moshe Shapiro , Paul Brumer

The analysis of nonlinear spectroscopy, widely used to study the dynamics and structures of condensed-phase matter, typically employs a perturbative approach noticing the weak interaction between the laser and the matter of interest.…

Optics · Physics 2022-06-23 Xue Zhang , Hui Dong

Vibrational dynamics in conventional molecules usually takes place on a timescale of picoseconds or shorter. A striking exception are ultralong-range Rydberg molecules, for which dynamics is dramatically slowed down as a consequence of the…

The model of coupled oscillators plays an important role in modern physics. It is used for description of various processes: from vibrations atoms in solid states to electromagnetic oscillations in slow-wave structures. The model with…

Accelerator Physics · Physics 2018-04-12 M. I. Ayzatsky , K. Yu. Kramarenko

We investigate on the same footing the time-dependent electronic transport properties and vibrational dynamics of a molecular junction. We show that fluctuations of both the molecular vibron displacement and the electronic current across…

Mesoscale and Nanoscale Physics · Physics 2019-03-27 Rémi Avriller , R Souto , A. Martin-Rodero , A Yeyati

A time-dependent approach is used to explore inelastic effects during electron transport through few-level systems. We study a tight-binding chain with one and two sites connected to vibrations. This simple but transparent model gives…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 S. Monturet , N. Lorente