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We consider the nature of the fluid-solid phase transition in a polydisperse mixture of hard spheres. For a sufficiently polydisperse mixture crystallisation occurs with simultaneous fractionation. At the fluid-solid boundary, a broad fluid…

Condensed Matter · Physics 2007-05-23 P. Bartlett

Experiments and simulations are used to study the kinetics of crystal growth in a mixture of magnetic and nonmagnetic particles suspended in ferrofluid. The growth process is quantified using both a bond order parameter and a mean domain…

Soft Condensed Matter · Physics 2017-01-11 An T. Pham , Ryohei Seto , Johannes Schonke , Daniel Y. Joh , Ashutosh Chilkoti , Eliot Fried , Benjamin B. Yellen

We present a computer simulation study of a (6,12)-Lennard-Jones fluid confined to a slit pore, formed by two uniform planes. These interact via a (3,9)-Lennard-Jones potential with the fluid particles. When the fluid approaches the…

Soft Condensed Matter · Physics 2011-07-21 N. Gribova , A. Arnold , H. Maleki , T. Schilling , C. Holm

Below the melting temperature $T_m$ crystals are the stable phase of typical elemental or molecular systems. However, cooling down a liquid below $T_m$, crystallization is anything but inevitable. The liquid can be supercooled, eventually…

Disordered Systems and Neural Networks · Physics 2017-03-07 M. Zanatta , L. Cormier , L. Hennet , C. Petrillo , F. Sacchetti

We carry out molecular dynamics (MD) and Monte Carlo (MC) simulations to characterize nucleation in liquid clusters of 600 Lennard-Jones particles over a broad range of temperatures. We use the formalism of mean first-passage times to…

Materials Science · Physics 2016-10-05 Shahrazad M. A. Malek , Gregory P. Morrow , Ivan Saika-Voivod

We have carried out extensive equilibrium molecular dynamics (MD) simulations to investigate the Liquid-Vapor coexistence in partially miscible binary and ternary mixtures of Lennard-Jones (LJ) fluids. We have studied in detail the time…

Soft Condensed Matter · Physics 2009-11-10 Enrique Diaz-Herrera , Guillermo Ramirez-Santiago , Jose A. Moreno-Razo

Supercooled liquids are characterized by relaxation times that increase dramatically by cooling or compression. Many liquids have been shown to obey power-law density scaling, according to which the relaxation time is a function of density…

Soft Condensed Matter · Physics 2012-12-19 Lasse Bøhling , Trond S. Ingebrigtsen , A. Grzybowski , M. Paluch , Jeppe C. Dyre , Thomas B. Schrøder

We report the results of a numerical study on the initial formation stages of low-mass protostellar binary systems. We determine the separation of protostellar binaries formed as a function of the initial thermal state by varying the…

Solar and Stellar Astrophysics · Physics 2015-06-22 R. Riaz , S. Z. Farooqui , S. Vanaverbeke

It is demonstrated that the crossover between gas- and liquid-like regions on the phase diagram of the Lennard-Jones system occurs at a fixed value of the density divided by its value at the freezing point, $\rho/\rho_{\rm fr}\simeq 0.35$.…

Statistical Mechanics · Physics 2022-03-29 Sergey Khrapak

On the basis of microscopic statistical mechanics of simple liquids the orientational interaction between clusters consisting of a particle and its nearest neighbors is estimated. It is shown that there are ranges of density and temperature…

Disordered Systems and Neural Networks · Physics 2009-11-10 N. M. Chtchelkatchev , V. N. Ryzhov , T. I. Schelkacheva , E. E. Tareyeva

Depositions of amorphous Lennard-Jones clusters on a crystalline surface are numerically investigated. From the results of the molecular dynamics simulation, we found that the deposited clusters exhibit a transition from multilayered…

Mesoscale and Nanoscale Physics · Physics 2009-12-03 Kuniyasu Saitoh , Hisao Hayakawa

Differential thermal analysis has been conducted for the Al-Cu-Co alloys with the composition range of 15 at.% Co and 10 to 30 at.% Cu, and 25 at.% Co and 2.5 to 20 at.% Co. The features of the formation of solid phases have been studied…

Materials Science · Physics 2022-12-08 Larisa V. Kamaeva , Elena N. Tsiok , Nikolay M. Chtchelkatchev

The separation of isotopes of natural Krypton at the gas-liquid and liquid-solid phase interfaces was studied under nonequilibrium conditions using a cryogenic cell and mass spectrometry. Condensate formation during Kr cooling begins at an…

Materials Science · Physics 2024-07-17 A. R. Cholach , D. V. Yakovin , N. I. Latkin , I. A. Sidorov

We perform molecular dynamics (MD) simulations of the crystallization process in binary Lennard-Jones systems during heating and cooling to investigate atomic-scale crystallization kinetics in glass-forming materials. For the cooling…

Soft Condensed Matter · Physics 2015-06-23 Minglei Wang , Kai Zhang , Zhusong Li , Yanhui Liu , Jan Schroers , Mark D. Shattuck , Corey S. O'Hern

Properties of local minima as a function of density are studied in a binary Lennard-Jones system for kinetic equipartition temperatures $T=1.0$ (normal liquid), 0.5 (supercooled liquid), and 0.4 (glass), in reduced units. The number of…

Disordered Systems and Neural Networks · Physics 2009-11-07 Javier Hernandez-Rojas , David J. Wales

We use molecular dynamics simulations in 2d to study multi-component fluid in the limiting case where {\it all the particles are different} (APD). The particles are assumed to interact via Lennard-Jones (LJ) potentials, with identical size…

Soft Condensed Matter · Physics 2015-06-23 Lenin S. Shagolsem , Dino Osmanović , Orit Peleg , Yitzhak Rabin

Kinetics of phase separation in a three dimensional single-component Lennard-Jones fluid, that exhibits vapor-liquid transition, is studied via molecular dynamics simulations after quenching homogeneous systems, of different overall…

Statistical Mechanics · Physics 2018-03-09 Sutapa Roy , Subir K. Das

Multicanonical ensemble sampling simulations have been performed to calculate the phase diagram of a Lennard-Jones fluid embedded in a fractal random matrix generated through diffusion limited cluster aggregation. The study of the system at…

Statistical Mechanics · Physics 2015-06-25 V. De Grandis , P. Gallo , M. Rovere

Using a modified Lennard-Jones model for anisotropic particles, we present results of molecular dynamics simulation in two dimensions. In one-component systems, we find crystallization, a Berezinskii-Kosterlitz-Thouless phase, and a…

Soft Condensed Matter · Physics 2011-12-23 Kyohei Takae , Akira Onuki

We examine the changeover in the particle configurations and the dynamics in dense Lennard-Jones binary mixtures composed of small and large particles. By varying the composition at a low temperature, we realize crystal with defects,…

Soft Condensed Matter · Physics 2011-05-17 Hayato Shiba , Akira Onuki