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The influence of monomer-monomer interactions on the scaling exponents and shape characteristics of a single polymer chain in a selective solvent is investigated using Langevin dynamics simulations. By systematically increasing the…

Soft Condensed Matter · Physics 2025-04-01 K. Haydukivska

We analyzed extensively the dynamics of polymer chains in solutions simulated with dissipative particle dynamics (DPD), with a special focus on the potential influence of a low Schmidt number of a typical DPD fluid on the simulated polymer…

Soft Condensed Matter · Physics 2009-11-11 W. Jiang , J. Huang , Y. Wang , M. Laradji

Using non-equilibrium Brownian dynamics computer simulations, we have investigated the steady state statistics of a polymer chain under three different shear environments: i) linear shear flow in the bulk (no walls), ii) shear vorticity…

Soft Condensed Matter · Physics 2015-05-14 Gui-Li He , René Messina , Hartmut Löwen

The radius of gyration of a polymer chain immersed in a low molecular weight solvent is known to vary monotonically with the solvent quality. Here, we consider the behavior of a chain immersed in a high molecular weight solvent (polymer…

Soft Condensed Matter · Physics 2007-05-23 Cyprien Gay , Elie Raphael

We consider three different continuum polymer models, that all depend on a tunable parameter r that determines the strength of the excluded-volume interactions. In the first model chains are obtained by concatenating hard spherocylinders of…

Soft Condensed Matter · Physics 2017-10-25 Giuseppe D'Adamo , Andrea Pelissetto

We report adaptive resolution molecular dynamics simulations of a flexible linear polymer in solution. The solvent, i.e., a liquid of tetrahedral molecules, is represented within a certain radius from the polymer's center of mass with a…

Soft Condensed Matter · Physics 2007-05-23 Matej Praprotnik , Luigi Delle Site , Kurt Kremer

Self-consistent field approach is used to model a single end-tethered polymer chain on a substrate subject to various forces in three dimensions. Starting from a continuous Gaussian chain model, the following perturbations are considered:…

The scaling of the bond-bond correlation function $C(s)$ along linear polymer chains is investigated with respect to the curvilinear distance, $s$, along the flexible chain and the monomer density, $\rho$, via Monte Carlo and molecular…

Soft Condensed Matter · Physics 2009-11-10 J. P. Wittmer , H. Meyer , J. Baschnagel , A. Johner , S. Obukhov , L. Mattioni , M. Mueller , A. N. Semenov

The crossover region in the phase diagram of polymer solutions, in the regime above the overlap concentration, is explored by Brownian Dynamics simulations, to map out the universal crossover scaling functions for the gyration radius and…

Soft Condensed Matter · Physics 2020-07-03 Aashish Jain , B. Duenweg , J. Ravi Prakash

Through extensive molecular simulations we determine a phase diagram of attractive, flexible polymer chains in two and three dimensions. A surprisingly rich collection of distinct crystal morphologies appear, which can be finely tuned…

In a recent article on stretched polymers in a poor solvent by Grassberger and Hsu \cite{grassberger2002a-a} questions were raised as to the conclusions that can be drawn from currently proposed scaling theory for a single polymer in…

Statistical Mechanics · Physics 2007-05-23 A. L. Owczarek , T. Prellberg

The rheological behavior of polymer melts is strongly influenced by parameters such as chain length, chain stiffness, and architecture. In particular, shear thinning, characterized by a power-law decrease in shear viscosity with increasing…

Soft Condensed Matter · Physics 2026-03-17 Yuhi Sakamaki , Shota Goto , Kang Kim , Nobuyuki Matubayasi

We examine the phase transition of polymer adsorption as well as the underlying kinetics of polymer binding from dilute solutions on a structureless solid surface. The emphasis is put on the properties of regular multiblock copolymers,…

Soft Condensed Matter · Physics 2009-09-03 A. Milchev , V. Rostiashvili , S. Bhattacharya , T. Vilgis

The conformational behavior of a coarse-grained finite polymer chain near an attractive spherical surface was investigated by means of multicanonical Monte Carlo computer simulations. In a detailed analysis of canonical equilibrium data…

Soft Condensed Matter · Physics 2018-01-03 Handan Arkin , Wolfhard Janke

We study the behavior of self avoiding polymers in a background of vertically aligned rods that are either frozen into random positions or free to move horizontally. We find that in both cases the polymer chains are highly elongated, with…

Soft Condensed Matter · Physics 2009-11-10 J. M. Deutsch , M. Warkentin

The static and dynamic properties of dendrimers in semidilute solutions of linear chains of comparable size are investigated using Brownian dynamics simulations. The radius of gyration and diffusivity of a wide variety of low generation…

Soft Condensed Matter · Physics 2024-06-19 Silpa Mariya , Jeremy J. Barr , P. Sunthar , J. Ravi Prakash

Langevin dynamics simulations are performed to investigate ejection dynamics of spherically confined flexible polymers through a pore. By varying the chain length $N$ and the initial volume fraction $\phi_0$ of the monomers, two scaling…

Soft Condensed Matter · Physics 2020-01-29 Hao-Chun Huang , Pai-Yi Hsiao

We investigate the localization of a hydrophobic - polar (HP) - regular copolymer at a selective solvent-solvent interface with emphasis on the impact of block length $M$ on the copolymer behavior. The considerations are based on simple…

Soft Condensed Matter · Physics 2007-05-23 Andrea Corsi , Andrey Milchev , Vakhtang G. Rostiashvili , Thomas A. Vilgis

Monte Carlo computer simulations are used to study the conformational free energy of a folded polymer confined to a long cylindrical tube. The polymer is modeled as a hard-sphere chain. Its conformational free energy $F$ is measured as a…

Soft Condensed Matter · Physics 2018-02-07 James M. Polson , Aidan F. Tremblett , Zakary R. N. McLure

Dissipative particle dynamics is a widely used mesoscale technique for the simulation of hydrodynamics (as well as immersed particles) utilizing coarse-grained molecular dynamics. While the method is capable of describing any fluid, the…

Computational Physics · Physics 2019-10-22 Ryan C. Krafnick , Angel E. Garcia