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We investigated the origin of the energy splitting observed in the resonant x-ray scattering (RXS) in manganites. Using thin film samples with controlled lattice parameters and orbital states at a fixed orbital filling, we estimated that…

Strongly Correlated Electrons · Physics 2009-11-10 M. Nakamura , M. Izumi , N. Ogawa , H. Ohsumi , Y. Wakabayashi , K. Miyano

X-ray echo spectroscopy, a counterpart of neutron spin-echo, is being introduced here to overcome limitations in spectral resolution and weak signals of the traditional inelastic x-ray scattering (IXS) probes. An image of a point-like x-ray…

Optics · Physics 2016-02-26 Yuri Shvyd'ko

Resonant x-ray scattering (RXS) experiment has been performed for the (3 0 1.5) superlattice reflection in the antiferroquadrupolar and antiferromagnetic phase of DyB2C2. Azimuthal-angle dependence of the resonance enhanced intensities for…

Strongly Correlated Electrons · Physics 2009-11-10 Takeshi Matsumura , Daisuke Okuyama , Nobuyuki Oumi , Kazuma Hirota , Hironori Nakao , Youichi Murakami , Yusuke Wakabayashi

The detection of inelastically scattered soft X-rays with high energy resolution usually requires large grating spectrometers. Recently, photoelectron spectrometry for analysis of X-rays (PAX) has been rediscovered for modern spectroscopy…

Resonant soft X-ray scattering with photon energies near the O K and the Cu L3 edges was used to study charge ordering in the system La_{1.8-x}Eu_{0.2}Sr_xCuO_4 as a function of temperature for x = 0.125 and 0.15. From the superstructure…

Superconductivity · Physics 2012-01-13 J. Fink , E. Schierle , E. Weschke , J. Geck , D. Hawthorn , H. Wadati , H. -H. Hu , H. A. Durr , N. Wizent , B. Buchner , G. A. Sawatzky

The electronic structure of CuIr$_2$S$_4$ has been investigated using various bulk-sensitive x-ray spectroscopic methods near the Ir $L_3$-edge: resonant inelastic x-ray scattering (RIXS), x-ray absorption spectroscopy in the partial…

Strongly Correlated Electrons · Physics 2012-06-18 H. Gretarsson , Jungho Kim , D. Casa , T. Gog , K. R. Choi , S. W. Cheong , Young-June Kim

Although orbital degrees of freedom are a factor of fundamental importance in strongly correlated transition metal compounds, orbital correlations and dynamics remain very difficult to access, in particular by neutron scattering. Via a…

Strongly Correlated Electrons · Physics 2015-03-20 Pasquale Marra , Krzysztof Wohlfeld , Jeroen van den Brink

This paper reviews non-resonant, meV-resolution inelastic x-ray scattering (IXS), as applied to the measurement of atomic dynamics of crystalline materials. It is designed to be an introductory, though in-depth, look at the field for those…

Materials Science · Physics 2020-08-26 Alfred Q. R. Baron

We present a theoretical investigation of the origin of Raman-like and fluorescencelike (FL) features of resonant inelastic x-ray scattering (RIXS) spectra. Using a combination of local-density approximation + dynamical mean-field theory…

Strongly Correlated Electrons · Physics 2018-09-26 Atsushi Hariki , Mathias Winder , Jan Kuneš

Excitons in a complex organic molecular crystal were studied by inelastic x-ray scattering (IXS) for the first time. The dynamic dielectric response function is measured over a large momentum transfer region, from which an exciton…

Other Condensed Matter · Physics 2007-05-23 K. Yang , L. P. Chen , Y. Q. Cai , N. Hiraoka , S. Li , J. F. Zhao , D. W. Shen , H. F. Song , H. Tian , L. H. Bai , Z. H. Chen , Z. G. Shuai , D. L. Feng

The recent discovery of spin-triplet superconductivity emerging from a non-magnetic parent state in UTe$_2$ has stimulated great interest in the underlying mechanism of Cooper pairing. Experimental characterization of short-range electronic…

X-ray absorption spectroscopy (XAS) is a powerful experimental technique to probe the local order in materials with core electron excitations. Experimental interpretation requires supporting theoretical calculations. For water, these…

Computational Physics · Physics 2022-05-17 Fujie Tang , Zhenglu Li , Chunyi Zhang , Steven G. Louie , Roberto Car , Diana Y. Qiu , Xifan Wu

We present a theory of the resonant inelastic x-ray scattering (RIXS) to study electronic excitations in orbital ordered manganites. The charge and orbital excitations of the Mn 3d electron are caused by the Coulomb interactions in the…

Strongly Correlated Electrons · Physics 2009-10-31 H. Kondo , S. Ishihara , S. Maekawa

We report a new theoretical method for X-ray absorption spectroscopy (XAS) in condensed matter which is based on the multi-channel multiple scattering theory of Natoli et al. and the eigen-channel R-matrix method. While the highly flexible…

Materials Science · Physics 2009-11-10 Peter Krüger , Calogero R. Natoli

Resonant angle scanned x-ray photoelectron diffraction (RXPD) allows the determination of the atomic and magnetic structure of surfaces and interfaces. For the case of magnetized nickel the resonant L2 excitation with circularly polarized…

Other Condensed Matter · Physics 2015-05-27 M. Morscher , F. Nolting , T. Brugger , T. Greber

We examine x-ray scattering from an isolated organic molecule from the linear to nonlinear absorptiveregime. In the nonlinear regime, we explore the importance of both the elastic and inelastic channelsand observe the onset of nonlinear…

Chemical Physics · Physics 2021-06-09 Phay J. Ho , Adam E. A. Fouda , Kai Li , Gilles Doumy , Linda Young

We provide a semiquantitative explanation of a recent experiment on the resonant inelastic x-ray scattering (RIXS) in insulating cuprate La2CuO4 (Y.J. Kim et al., Phys. Rev. Lett. 89, 177003 (2002).). We show theoretically that there are…

Strongly Correlated Electrons · Physics 2009-11-10 Takuji Nomura , Jun-ichi Igarashi

A prevailing description of the stripe phase in underdoped cuprate superconductors is that the charge carriers (holes) phase segregate on a microscopic scale into hole rich and hole poor regions. We report resonant elastic x-ray scattering…

Superconductivity · Physics 2013-01-08 A. J. Achkar , F. He , R. Sutarto , J. Geck , H. Zhang , Y. -J. Kim , D. G. Hawthorn

Resonant inelastic x-ray scattering (RIXS) has become a powerful tool in the study of the electronic structure of condensed matter. Although the linewidths of many RIXS features are narrow, the experimental broadening can often hamper the…

Strongly Correlated Electrons · Physics 2012-02-13 J. Laverock , A. R. H. Preston , D. Newby , K. E. Smith , S. B. Dugdale

Resonant inelastic x-ray scattering (RIXS) is a spectroscopic technique which has been widely used to study various elementary excitations in correlated and other condensed matter systems. For strongly correlated materials, besides boosting…

Strongly Correlated Electrons · Physics 2012-12-27 C. J. Jia , C. -C. Chen , A. P. Sorini , B. Moritz , T. P. Devereaux
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