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The magnetic properties of the double perovskite oxide $Sr_{2}$FeMo$O_{6}$ are analyzed using a mixed-spin Ising model with spins $\left( \frac{1}{2},\frac{5}{2}\right) $ in the presence of a random crystal field $\Delta$ and exchange…

Statistical Mechanics · Physics 2025-03-10 Said Khaireddine , Redouane Assad , Mohammed El Falaki , Rachid Ahl Lamara , Lalla Btissam Drissi

Realization of spin crossover (SCO) based applications requires studying of spin state switching characteristics of SCO complex molecules at nanostructured environments especially on-surface. Except for a very few cases, the SCO of a…

One of the key factors behind the rapid evolution of molecular spintronics is the efficient realization of spin manipulation of organic molecules with a magnetic center. The spin state of such molecules may depend crucially on the…

We consider polymers made of magnetic monomers (Ising or Heisenberg-like) in a good solvent. These polymers are modeled as self-avoiding walks on a cubic lattice, and the ferromagnetic interaction between the spins carried by the monomers…

Statistical Mechanics · Physics 2009-10-31 T. Garel , H. Orland , E. Orlandini

Spin-state transition, also known as spin crossover, plays a key role in diverse systems, including minerals and biological materials. In theory, the boundary range between the low- and high-spin states is expected to enrich the transition…

Despite a clear demonstration of bistability in spin-crossover (SCO) materials, the absence of long-range magnetic order and poor electrical conductivity limit their prospect in spintronic and nanoelectronic applications. Intending to…

The mechanism behind fast intersystem crossing in transition-metal complexes is shown to be a result of the dephasing of the photoexcited state to the phonon continuum of a different state with a significantly different transition…

Strongly Correlated Electrons · Physics 2010-02-11 Michel van Veenendaal , Jun Chang , A. J. Fedro

The dominant majority of the hundreds of available spin-crossover compounds, including the technologically most promising ones, are based on the Earth-abundant metal iron, making these switches particularly appealing in terms of sustainable…

Other Condensed Matter · Physics 2020-07-24 Latévi Max Lawson Daku , Mark Earl Casida

Octahedral Fe$^{2+}$ molecules are particularly interesting as they often exhibit a spin-crossover transition. In spite of the many efforts aimed at assessing the performances of density functional theory for such systems, an…

Materials Science · Physics 2015-06-05 A. Droghetti , D. Alfè , S. Sanvito

We present phase diagrams, free-energy landscapes, and order-parameter distributions for a model spin-crossover material with a two-step transition between the high-spin and low-spin states (a square-lattice Ising model with…

Materials Science · Physics 2017-12-01 Chor-Hoi Chan , Gregory Brown , Per Arne Rikvold

The X-ray absorption near-edge structure (XANES) of Mn in a spin-crossover compound, [Mn$^{\textrm{III}}$(taa)], was studied in pulsed high magnetic fields up to 37T. By applying magnetic fields to the low-temperature low-spin (LS) state,…

Strongly Correlated Electrons · Physics 2015-03-14 Jim Long Her , Yasuhiro H. Matsuda , Motohiro Nakano , Yasuhiro Niwa , Yasuhiro Inada

Mechanical stacking of two dissimilar materials often has surprising consequences for heterostructure behavior. In particular, a two-dimensional electron gas (2DEG) is formed in the heterostructure of the topological crystalline insulator…

Anti-ferromagnetic materials have the possibility to offer ultra fast, high data density spintronic devices. A significant challenge is the reliable detection of the state of the antiferromagnet, which can be achieved using exchange bias.…

Materials Science · Physics 2021-03-17 Sarah Jenkins , Roy. W. Chantrell , Richard. F. L. Evans

Spin crossover frameworks and molecular crystals display fascinating collective behaviours. This includes multi-step transitions with hysteresis and a wide variety of long-range ordered patterns of high-spin and low-spin metal centres. From…

Strongly Correlated Electrons · Physics 2020-11-25 Jace Cruddas , B. J. Powell

With the recent experimental verification that ferroelectric lattice distortions survive in the metallic phase of some materials, there is a desire to create devices that are both switchable and take advantage of the novel functionalities…

Mesoscale and Nanoscale Physics · Physics 2022-02-10 Kelsey S. Chapman , W. A. Atkinson

From general arguments, that are valid for spin models with sufficiently short-range interactions, we derive strong constraints on the excitation spectrum across a continuous phase transition at zero temperature between a magnetic and a…

Strongly Correlated Electrons · Physics 2009-11-11 Leonardo Spanu , Federico Becca , Sandro Sorella

We study a one-dimensional antiferromagnetic-elastic model with magnetic ions having spin $S=3/2$. By extensive DMRG computations and complementary analytical methods, we uncover a first-order transition from a homogeneous or…

Strongly Correlated Electrons · Physics 2025-09-15 C. J. Gazza , A. A. Aligia , A. O. Dobry , G. L. Rossini , D. C. Cabra

Conventional superexchange rules predict ferromagnetic exchange interaction between Ni(II) and M (M=Mo(V), W(V), Nb(IV)). Recent experiments show that in some systems this superexchange is antiferromagnetic. To understand this feature, in…

Strongly Correlated Electrons · Physics 2009-11-11 Rajamani Raghunathan , Jean-Pascal Sutter , Laurent Ducasse , Cedric Desplanches , S. Ramasesha

Structural, magnetic and electrical-transport properties of {\alpha}-LiFeO2, crystallizing in the rock salt structure with random distribution of Li and Fe ions, have been studied by synchrotron X-ray diffraction, 57Fe M\"ossbauer…

Strongly Correlated Electrons · Physics 2017-09-29 Samar Layek , Eran Greenberg , Weiming Xu , Gregory Kh. Rozenberg , Moshe P. Pasternak , Jean-Paul Itié , Dániel G. Merkel

Magnetic, dielectric, and magnetoelectric properties in a spin-state transition system are examined, motivated by the recent discovery of a multiferroic behavior in a cobalt oxide. We construct an effective model Hamiltonian based on the…

Strongly Correlated Electrons · Physics 2018-06-13 Makoto Naka , Eriko Mizoguchi , Joji Nasu , Sumio Ishihara