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We report neutron scattering measurements of the spectrum of magnetic excitations in the stripe-ordered phase of La2-xSrxNiO4 (x=0.275 and 1/3). The propagating spin excitations follow a similar dispersion relation for the two compositions,…

Strongly Correlated Electrons · Physics 2009-11-10 A. T. Boothroyd , P. G. Freeman , D. Prabhakaran , H. Woo , K. Nakajima , J. M. Tranquada , K. Yamada , C. D. Frost

We study long wavelength magnetic excitations in lightly doped La_{2-x}Sr_{x}CuO_{4} (x < 0.03) detwinned crystals. The lowest energy magnetic anisotropy induced gap can be understood in terms of the antisymmetric spin interaction inside…

Strongly Correlated Electrons · Physics 2009-11-10 A. Gozar , B. S. Dennis , G. Blumberg , Seiki Komiya , Yoichi Ando

Including the orbital off-diagonal spin and charge condensates in the self consistent determination of magnetic order within a realistic three-orbital model for the $4d^4$ compound $\rm Ca_2 Ru O_4$, reveals a host of novel features…

Strongly Correlated Electrons · Physics 2021-07-05 Shubhajyoti Mohapatra , Avinash Singh

Inelastic neutron scattering (INS) experiments were performed to investigate the spin dynamics in magnetoelectric effect (ME) LiCoPO$_4$ single crystals. Weak dispersion was detected in the magnetic excitation spectra along the three…

Strongly Correlated Electrons · Physics 2013-08-14 Wei Tian , Jiying Li , Jeffrey W. Lynn , Jerel L. Zarestky , David Vaknin

Alkali superoxides differ from conventional transition metal magnets, exhibit magnetism from partially occupied oxygen molecular $\pi^*$-orbitals. Among them, CsO$_2$ stands out for its potential to exhibit novel quantum collective…

Strongly Correlated Electrons · Physics 2024-11-12 Ryota Ono , Ravi Kaushik , Sergey Artyukhin , Martin Jansen , Igor Solovyev , Russell A. Ewings

We present a neutron diffraction study of FeV2O4, which is rare in exhibiting spin and orbital degrees of freedom on both cation sublattices of the spinel structure. Our data confirm the existence of three structural phase transitions…

Strongly Correlated Electrons · Physics 2012-09-03 G. J. MacDougall , V. O. Garlea , A. A. Aczel , H. D. Zhou , S. E. Nagler

We report high-resolution neutron inelastic scattering experiments on the spin excitations of NaV2O5. Below Tc, two branches associated with distinct energy gaps are identified. From the dispersion and intensity of the spin excitation…

Strongly Correlated Electrons · Physics 2009-10-31 B. Grenier , O. Cepas , L. P. Regnault , J. E. Lorenzo , T. Ziman , J. P. Boucher , A. Hiess , T. Chatterji , J. Jegoudez , A. Revcolevschi

Correlated materials with competing spin-orbit and crystal-field interactions can host composite spin-orbital magnons that are highly susceptible to structural and electronic perturbations, enabling the control of magnetic dynamics beyond…

Evolution of composite spin-orbital order and coupled spin-orbital excitations is studied in a variety of $d^4$ systems with $n$=$4$ electrons in the $t_{2g}$ orbital sector using the generalised self-consistent + fluctuations approach for…

Strongly Correlated Electrons · Physics 2025-04-30 Shahid Ahmad , Harshvardhan Parmar , Shubhajyoti Mohapatra , Avinash Singh

We investigate interactions between spins of strongly correlated electrons subject to the spin-orbit interaction. Our main finding is that of a novel, spin-orbit mediated anisotropic spin-spin coupling of the van der Waals type. Unlike the…

Mesoscale and Nanoscale Physics · Physics 2008-04-23 Suhas Gangadharaiah , Jianmin Sun , Oleg A. Starykh

In this letter we report results from inelastic neutron scattering experiments on powder samples of vanadyl pyrophosphate, (VO)2P2O7. We see evidence for three magnetic excitations, at 3.5 meV, 6.0 meV and 14 meV. The intensity of the 3.5…

Condensed Matter · Physics 2009-10-28 A. W. Garrett , S. E. Nagler , T. Barnes , B. C. Sales

We performed inelastic neutron scattering experiments on single crystal samples of a linear magnetoelectric material Mn$_{3}$Ta$_{2}$O$_{8}$, which exhibits a collinear antiferromagnetic order, to reveal the spin dynamics. Numerous modes…

Strongly Correlated Electrons · Physics 2025-04-08 Hodaka Kikuchi , SHunsuke Hasegawa , Shinichiro Asai , Tao Hong , Kenta Kimura , Tsuyoshi Kimura , Shinichi Itoh , Takatsugu Masuda

NH4CuCl3 has two magnetization plateaus at one-quarter and three-quarters of the saturation magnetization, irrespective of the external field direction. Magnetic excitations in NH4CuCl3 have been investigated by means of neutron inelastic…

Strongly Correlated Electrons · Physics 2007-05-23 A. Oosawa , T. Ono , K. Kakurai , H. Tanaka

We report on the magnetic excitation spectrum of the coupled spin tetrahedral system Cu$_{2}$Te$_{2}$O$_{5}$Cl$_{2}$ using Raman scattering on single crystals. The transition to an ordered state at T$_{N}^{Cl}$=18.2 K evidenced from…

Strongly Correlated Electrons · Physics 2009-11-13 Kwang-Yong Choi , Hiroyuki Nojiri , Naresh S. Dalal , Helmuth Berger , Wolfram Brenig , Peter Lemmens

The mechanisms of magnetic and orbital interactions due to double exchange (DE) and superexchange (SE) in transition metal oxides with degenerate e_g orbitals are presented. Specifically, we study the effective spin-orbital models derived…

Strongly Correlated Electrons · Physics 2009-10-31 A. M. Oles , M. Cuoco , N. B. Perkins

We determined the magnetic structure of CuCr$_2$O$_4$ using neutron diffraction and irreducible representation analysis. The measurements identified a new phase between 155 K and 125 K as nearly collinear magnetic ordering in the Cr…

Strongly Correlated Electrons · Physics 2018-03-20 K. Tomiyasu , S. Lee , H. Ishibashi , Y. Takahashi , T. Kawamata , Y. Koike , T. Nojima , S. Torii , T. Kamiyama

Spin correlations in metallic and insulating phases of $V_2O_3$ and its derivatives are investigated using magnetic neutron scattering. Metallic samples have incommensurate spin correlations varying little with hole doping. Paramagnetic…

Strongly Correlated Electrons · Physics 2009-10-28 Wei Bao , C. Broholm , G. Aeppli , P. Dai , J. M. Honig , P. Metcalf

Effects of possible orbital order in magnetic properties of two-dimensional spin gap system for CaV$_4$O$_9$ are investigated theoretically. After analyzing experimental data, we show that single orbital models assumed in the literature are…

Strongly Correlated Electrons · Physics 2009-10-30 Nobuyuki Katoh , Masatoshi Imada

The temperature dependence and anisotropy of optical spectral weights associated with different multiplet transitions is determined by the spin and orbital correlations. To provide a systematic basis to exploit this close relationship…

Strongly Correlated Electrons · Physics 2007-05-23 Andrzej M. Oles , Giniyat Khaliullin , Peter Horsch , Louis Felix Feiner

Mixed spin chain compounds, ACuFe2(VO4)3 (A= Li,Na), reach magnetically ordered state at TN ~ 11 K (Li) or ~ 9 K (Na) and experience further transformation of magnetic order at T* ~ 7 K (Li) or ~ 5 K (Na), evidenced in magnetic…

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