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By implementing four-wave mixing (FWM) micro-spectroscopy we measure coherence and population dynamics of the exciton transitions in monolayers of MoSe$_2$. We reveal their dephasing times T$_2$ and radiative lifetime T$_1$ in a…

Pure dephasing of an exciton in a small quantum dot by optical and acoustic phonons is calculated using the ``independent boson model''. Considering the case of zero temperature the dephasing is shown to be only partial which manifests…

Condensed Matter · Physics 2009-11-07 E. Pazy

The full time-dependent four-wave mixing polarization in quantum dots is microscopically calculated, taking into account acoustic phonon-assisted transitions between different exciton states of the dot. It is shown that quite different…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 E. A. Muljarov , R. Zimmermann

We investigate theoretically acoustic phonon induced decoherence in quantum dots. We calculate the dephasing of fundamental (interband or intraband) optical transitions due to real and virtual transitions with higher energy levels. Up to…

Other Condensed Matter · Physics 2015-05-13 Thomas Grange

A microscopic theory of optical transitions in quantum dots with carrier-phonon interaction is developed. Virtual transitions into higher confined states with acoustic phonon assistance add a quadratic phonon coupling to the standard linear…

Condensed Matter · Physics 2009-11-10 E. A. Muljarov , R. Zimmermann

A new microscopic approach to the optical transitions in quantum dots and quantum dot molecules, which accounts for both diagonal and non-diagonal exciton-phonon interaction, is developed. The cumulant expansion of the linear polarization…

Other Condensed Matter · Physics 2015-06-25 E. A. Muljarov , T. Takagahara , R. Zimmermann

Optimized light-matter coupling in semiconductor nanostructures is a key to understand their optical properties and can be enabled by advanced fabrication techniques. Using in-situ electron beam lithography combined with a low-temperature…

We investigate the feasibility of minimum absorption and minimum broadening of pulse propagation in an inhomogeneously broadened semiconductor quantum dot medium. The phonon interaction is inevitable in studying any semiconductor quantum…

Quantum Physics · Physics 2023-06-19 Samit Kumar Hazra , P. K. Pathak , Tarak Nath Dey

The design of some optical devices such as semiconductor optical amplifiers for telecommunication applications requires polarization-insensitive optical emission at the long wavelengths (1300-1550 nm). Self-assembled InAs/GaAs quantum dots…

Materials Science · Physics 2015-05-20 Muhammad Usman , Susannah Heck , Edmund Clarke , Peter Spencer , Hoon Ryu , Ray Murray , Gerhard Klimeck

We experimentally and theoretically investigate dephasing of zero dimensional microcavity polaritons in electrically tunable single dot photonic crystal nanocavities. Such devices allow us to alter the dot-cavity detuning in-situ and to…

Other Condensed Matter · Physics 2009-12-21 A. Laucht , N. Hauke , J. M. Villas-Bôas , F. Hofbauer , M. Kaniber , G. Böhm , J. J. Finley

When an electron-hole pair is optically excited in a semiconductor quantum dot the host crystal lattice needs to adapt to the presence of the generated charge distribution. Therefore the coupled exciton-phonon system has to establish a new…

The dephasing mechanisms of p-shell and s-shell excitons in an InAs self-assembled quantum dot ensemble are examined using two-dimensional coherent spectroscopy (2DCS). 2DCS provides a comprehensive picture of how the energy level structure…

Mesoscale and Nanoscale Physics · Physics 2019-08-16 Takeshi Suzuki , Rohan Singh , Galan Moody , Marc Aßmann , Manfred Bayer , Arne Ludwig , Andreas D. Wieck , and Steven T. Cundiff

The decay time of the linear polarization degree of the luminescence in strongly confined semiconductor quantum dots with asymmetrical shape is calculated in the frame of second-order quasielastic interaction between quantum dot charge…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 E. Tsitsishvili , R. v. Baltz , H. Kalt

We provide a self-contained review of master equation approaches to modelling phonon effects in optically driven self-assembled quantum dots. Coupling of the (quasi) two-level excitonic system to phonons leads to dissipation and dephasing,…

Mesoscale and Nanoscale Physics · Physics 2016-06-14 Ahsan Nazir , Dara P. S. McCutcheon

The ultrafast scattering dynamics of intersubband polaritons in dispersive cavities embedding GaAs/AlGaAs quantum wells are studied directly within their band structure using a non-collinear pump-probe geometry with phase-stable…

Semiconductor quantum dots have emerged as an especially promising platform for the generation of polarization-entangled photon pairs. However, it was demonstrated recently that the two-photon excitation scheme employed in state-of-the-art…

Phonon-related decoherence effects in a quantum double-well two-level subsystem coupled to a solid are studied theoretically by the example of deformation phonons. Expressions for the reduced density matrix at T=0 are derived beyond the…

Other Condensed Matter · Physics 2009-11-13 L. A. Openov

We study theoretically the radiative recombination of excitons in double quantum dots in the presence of carrier-phonon coupling. We show that the phonon-induced pure dephasing effects and transitions between the exciton states strongly…

Mesoscale and Nanoscale Physics · Physics 2012-01-20 Pawel Karwat , Anna Sitek , Pawel Machnikowski

We study the electronic relaxation in a quantum dot within the polaron approach, by focusing on the {\it reversible} anharmonic decay of longitudinal optical (LO) phonons forming the polaron into longitudinal acoustic (LA) phonons. The…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 T. Stauber , M. I. Vasilevskiy

We compute the transient dynamics of phonons in contact with high energy "hot" charge carriers in 12 polar and non-polar semiconductors, using a first-principles Boltzmann transport framework. For most materials, we find that the decay in…

Mesoscale and Nanoscale Physics · Physics 2017-10-03 Sridhar Sadasivam , Maria K. Y. Chan , Pierre Darancet
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