Related papers: Control of recollision wave packets for molecular …
Trains of ultrashort laser pulses separated by the time of rotational revival (typically, tens of picoseconds) have been exploited for creating ensembles of aligned molecules. In this work we introduce a chiral pulse train - a sequence of…
We apply theoretically open-loop quantum optimal control techniques to provide methods for the verification of various quantum coherent transport mechanisms in natural and artificial light-harvesting complexes under realistic experimental…
High-order harmonic generation (HHG), a robust tabletop source for producing attosecond pulses, has been extensively utilized in attosecond metrology. Traditionally, HHG driven by classical laser fields involves two typical quantum paths…
Genetic algorithms, as implemented in optimal control strategies, are currently successfully exploited in a wide range of problems in molecular physics. In this context, laser control of molecular alignment and orientation remains a very…
Two oppositely charged particles created within a microscopic space-time region can be separated, accelerated over a much larger distance, and brought to a recollision by a laser field. Consequently, new reactions become feasible, where the…
Non dispersive electronic Rydberg wave packets may be created in atoms illuminated by a microwave field of circular polarization. We discuss the spontaneous emission from such states and show that the elastic incoherent component (occuring…
XUV and X-ray Free Electron Lasers (FELs) produce short wavelength pulses with high intensity, ultrashort duration, well-defined polarization and transverse coherence, and have been utilised for many experiments previously possible at long…
We consider few-photon ionization of atomic lithium by linearly polarized femtosecond laser pulses, and demonstrate that asymmetries of the electron angular distribution can occur for initially polarized (2p, m=+1) target atoms. The…
In nonlinear Thomson scattering, a relativistic electron reflects and re-radiates the photons of a laser pulse, converting optical light to x rays or beyond. While this extreme frequency conversion offers a promising source for probing…
We theoretically investigate high-harmonic generation in hexagonal boron nitride with linearly polarized laser pulses. We show that imperfect recollisions between electron-hole pairs in the crystal give rise to an electron-hole-pair…
We apply the theory of high-order harmonic generation by low-frequency laser fields in the strong field approximation to the study of the spatial and temporal coherence properties of the harmonics. We discuss the role of dynamically induced…
We propose a semi-classical approach based on the Vlasov equation to describe the time-dependent electronic dynamics in a bulk simple metal under an ultrashort intense laser pulse. We include in the effective potential not only the ionic…
Laser control of molecular rotation is an area of active research. A number of recent studies has aimed at expanding the reach of rotational control to extreme, previously inaccessible rotational states, as well as controlling the…
We have constructed an automated learning apparatus to control quantum systems. By directing intense shaped ultrafast laser pulses into a variety of samples and using a measurement of the system as a feedback signal, we are able to reshape…
The finite-amplitude short coherent control pulse with small random errors in its direction is considered. We derive the conditions for it to approximate an ideal delta-shaped pulse up to an error in the second order of pulse duration.…
Introducing a spatial chirp into a pulse with a longitudinal vortex, such as a standard pulsed Laguerre-Gauss beam, results in a vortex pulse with an arbitrary orientation of the line phase singularity between longitudinal and transverse,…
A comprehensive theoretical approach to describe the electron-ion radiative recombination in the presence of intense, short laser pulses, which accounts for nondipole corrections is presented. It is based on the relativistic Coulomb-Volkov…
An all non-optical method for accurately determining the pulse parameters of individual few-cycle laser shots is presented. By analyzing the "left" and "right" asymmetry of high-energy photoelectrons along the polarization axis using the…
High-order harmonic generation (HHG), characterized by its highly nonlinear nature, often exhibits a complex spatio-temporal profile that poses challenges for practical applications. In this study, we unveil a method for manipulating the…
The coherent control of small quantum system is considered. For a two-level system coupled to an arbitrary bath we consider a pulse of finite duration. We derive the leading and the next-leading order corrections to the evolution operator…