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We propose a novel method that uses the oscillation of an atomic excited wave packet observed through a pump-probe technique to accurately determine the zero time delay between a pair of ultrashort laser pulses. This physically-based…

Optics · Physics 2009-11-13 Qun Zhang , John W. Hepburn

In a novel experiment that images the momentum distribution of individual, isolated 100-nm-scale plasmas, we make the first experimental observation of shock waves in nanoplasmas. We demonstrate that the introduction of a heating pulse…

Two XUV-photon double ionization of Ne, induced by an intense few-pulse attosecond train with a ~ 4 fs envelope duration is investigated experimentally and theoretically. The experiment is performed at ELI-ALPS utilizing the recently…

The dynamics of an x-ray-ionized two-component core-shell nanosystem is probed using doped helium (He) nanodroplets. First, a soft x-ray pump pulse selectively inner-shell ionizes the core cluster formed of heavier rare-gas atoms, causing…

function of the CEP, we observe a transition from a modulated to a continuous SHHG spectrum, indicating the transition from double to high-contrast isolated attosecond pulse emission. Single shot-acquisitions of XUV spectral continua…

We present experimental studies on the generation and detection of pulsed, relative-intensity squeezed light in a warm rubidium vapor. The noise correlations between a pulsed probe beam and its conjugate -generated through nearly-degenerate…

Rare gas or metal clusters are known to absorb laser energy very efficiently. Upon cluster expansion the Mie plasma frequency may become equal to the laser frequency. This linear resonance has been well studied both experimentally and…

Atomic and Molecular Clusters · Physics 2009-11-11 M. Kundu , D. Bauer

Abrupt time variations of the properties of optical materials have been at the center of intense research efforts in recent years, with the prospect of enabling extreme wave transformations and of leveraging time as a degree of freedom for…

We introduce and experimentally demonstrate a method, where the two intrinsic time scales of a molecule, the slow nuclear motion and the fast electronic motion, are simultaneously measured in a photo-electron photo-ion coincidence…

Strongly laser-driven semiconductor crystals offer substantial advantages for the study of many-body physics and ultrafast optoelectronics via the high harmonic generation process. While this phenomenon has been employed to investigate the…

The complex interaction dynamics of intense femtosecond (fs) pulses and their picosecond (ps)-long leading edge with nanostructured solids occur at both the nanometer and the femtosecond scales, making them extremely difficult to measure…

Plasma Physics · Physics 2024-03-19 Ankit Dulat , Sagar Dam , Sk Rakeeb , Amit D. Lad , Yash M. Ved , G. Ravindra Kumar

Electronic correlations occur on attosecond timescales, dictating how chemical bonds form, energy flows, and materials respond to light. Capturing such many-body processes requires light pulses of similar duration. The soft X-ray water…

The quantum dynamics of a system of Rb atoms, modeled by a V-type three-level system interacting with intense probe and pump pulses, are studied. The time-delay-dependent transient-absorption spectrum of an intense probe pulse is thus…

Atomic Physics · Physics 2018-02-14 Vadim Becquet , Stefano M. Cavaletto

We have used optically excited ultrashort electrical pulses to measure the magnetoplasmon resonance of a two-dimensional electron gas formed in an AlGaAs/GaAs heterostructure at frequencies up to 200 gigahertz. This is accomplished by…

Materials Science · Physics 2009-11-07 E. A. Shaner , S. A. Lyon

Nonlinear wave-mixing in solids with ultrafast x-rays can provide new insight into complex electronic dynamics of materials. Here, tabletop-based attosecond noncollinear four-wave mixing (FWM) spectroscopy using one extreme ultraviolet…

The ability to control absorption by modifying the polarization of light presents an exciting opportunity to experimentally determine the orbital alignment of absorption features. Here, attosecond extreme ultraviolet (XUV) transient…

Visualizing ultrafast dynamics at the atomic scale requires time-resolved pump-probe characterization with femtosecond temporal resolution. For single-shot ultrafast electron diffraction (UED) with fully relativistic electron bunch probes,…

A detection scheme for characterizing high-energy $\gamma$-ray pulses down to the zeptosecond timescale is proposed. In contrast to existing attosecond metrology techniques, our method is not limited by atomic shell physics and therefore…

Instrumentation and Detectors · Physics 2011-08-17 Andreas Ipp , jörg Evers , Christoph H. Keitel , Karen Z. Hatsagortsyan

The spectrum of laser-plasma generated X-rays is very important, it characterizes electron dynamics in plasma and is basic for applications. However, the accuracies and efficiencies of existing methods to diagnose the spectrum of…

Instrumentation and Detectors · Physics 2021-09-03 Jiaxing Wen , Minghai Yu , Yuchi Wu , Ming Zeng , Bo Zhang , Jirong Cang , Yuge Zhang , Ge Ma , Yue Yang , Wenbo Mo , Zongqing Zhao

Attosecond pulses provide unique opportunities for studies of time-resolved electron dynamics. However, focusing these pulses, typically ranging from the vacuum ultraviolet to the soft-X-ray region, remains challenging. Conventional…