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Non-equilibrium processes following the irradiation of atomic clusters with short pulses of vacuum ultraviolet radiation are modelled using kinetic Boltzmann equations. The dependence of the ionization dynamics on the cluster size is…

Plasma Physics · Physics 2009-11-13 B. Ziaja , H. Wabnitz , E. Weckert , T. Möller

We present a scheme for amplifying an extreme-ultraviolet (XUV) seed isolated attosecond pulse via stimulated Raman scattering of a pulse-train pump. At sufficient seed and pump intensity, the amplification is nonlinear, and the amplitude…

Plasma Physics · Physics 2022-10-24 Andréas Sundström , Mickael Grech , István Pusztai , Caterina Riconda

The interaction of intense laser pulses with plasma mirrors has demonstrated the ability to generate high-order harmonics, producing a bright source of extreme ultraviolet (XUV) radiation and attosecond pulses. Here, we report an unexpected…

A time resolved experiment to investigate the ultrafast dynamics following an ion impact onto a solid surface requires an ultrashort ion pump pulse in combination with a properly synchronized and time resolved probe. In order to realize…

Atomic Physics · Physics 2023-05-18 P. Kucharczyk , A. Golombek , M. Schleberger , A. Wucher , L. Breuer

Calculating the energy absorption of atomic clusters as a function of the laser pulse length $T$ we find a maximum for a critical $T^*$. We show that $T^*$ can be linked to an optimal cluster radius $R^*$. The existence of this radius can…

Atomic and Molecular Clusters · Physics 2009-11-07 Christian Siedschlag , Jan M. Rost

Standard optical pump-probe methods analyze a system's temporal response to a laser pulse within sub-femtoseconds to several nanoseconds, constrained by the optical delay line's length. While resistance is a sensitive detector in various…

Instrumentation and Detectors · Physics 2024-04-26 M. I. Blumenau , A. Yu. Kuntsevich

Linear off-resonant X-ray Raman techniques are capable of detecting the ultrafast electronic coherences generated when a photoexcited wave packet passes through a conical intersection. A hybrid femtosecond or attosecond probe pulse is…

Chemical Physics · Physics 2022-11-07 Lorenzo Restaino , Deependra Jadoun , Markus Kowalewski

We derive the analytical theory describing the process of sub-femtosecond pulse formation from a quasi-monochromatic seeding extreme ultraviolet (XUV) radiation, which propagates in active medium of a hydrogen-like plasma-based X-ray laser…

We demonstrate pump-probe techniques, namely the Doppler spectrometry and the reflectometry in detail, which directly capture the time-resolved ultrafast evolution of high intensity femtosecond laser-driven hot, dense plasma. These…

Practical aspects of the robust method we recently proposed for producing few-cycle attosecond pulses with arbitrary waveform in the extreme ultraviolet spectral range are studied numerically. It is based on the undulator radiation of…

Optics · Physics 2016-04-28 Z. Tibai , Gy. Tóth , Zs. Nagy-Csiha , J. A. Fülöp , G. Almási , J. Hebling

Attosecond science is based on steering of electrons with the electric field of well-controlled femtosecond laser pulses. It has led to, for example, the generation of XUV light pulses with a duration in the sub-100-attosecond regime, to…

Quantum Physics · Physics 2011-07-11 Michael Krüger , Markus Schenk , Peter Hommelhoff

Time-resolved investigations of ultrafast electronic and molecular dynamics were not possible until recently. The typical time scale of these processes is in the picosecond to attosecond realm. The tremendous technological progress in…

Atomic Physics · Physics 2013-05-14 Stefan Pabst

Superfluid He nanodroplets resonantly excited by extreme ultraviolet (XUV) pulses exhibit complex relaxation dynamics, including the formation of metastable excited He$^*$ atoms trapped in bubbles, the desorption of excited atoms from the…

We observe and control a molecular vibrational wave packet in an electronically excited state of the neutral hydrogen molecule. In an extreme-ultraviolet (XUV) transient-absorption experiment we launch a vibrational wave packet in the $D…

Tracking the coupled motion of electrons and nuclei on their intrinsic timescales is essential to understanding and controlling photochemical transformations. While attosecond techniques have provided unprecedented insight into electronic…

We have investigated the polarization of attosecond light bursts generated by nanobunches of electrons from relativistic few-cycle laser pulse interaction with the surface of overdense plasmas. Particle-in-cell simulation shows that the…

Optics · Physics 2016-01-27 Guangjin Ma , Wei Yu , M. Y. Yu , Baifei Shen , Laszlo Veisz

We study the temporal aspects of laser-assisted extreme ultraviolet (XUV) photoionization using attosecond pulses of harmonic radiation. The aim of this paper is to establish the general form of the phase of the relevant transition…

We investigate the evolution of extreme ultraviolet (XUV) spectral lineshapes in an optically-thick helium gas under near-infrared (IR) perturbation. In our experimental and theoretical work, we systematically vary the IR intensity,…

Atomic Physics · Physics 2016-03-09 Chen-Ting Liao , Seth Camp , Kenneth J. Schafer , Mette B. Gaarde , Arvinder Sandhu

Extreme ultraviolet (XUV) light sources allow for the probing of bound electron dynamics on attosecond scales, interrogation of high-energy-density matter, and access to novel regimes of strong-field quantum electrodynamics. Despite the…

The interaction of strong near-infrared (NIR) laser pulses with wide-bandgap dielectrics produces high harmonics in the extreme ultraviolet (XUV) wavelength range. These observations have opened up the possibility of attosecond metrology in…

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