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Attosecond laser pulses open the door to resolve microscopic electron dynamics in time. Experiments performed include the decay of a core hole, the time-resolved measurement of photo ionization and electron tunneling. The processes…

Atomic and Molecular Clusters · Physics 2011-11-09 Ionut Georgescu , Ulf Saalmann , Jan M. Rost

Studies of ultrafast dynamics along with femtosecond-pulse metrology rely on non-linear processes, induced solely by the exciting/probing pulses or the pulses to be characterized. Extension of these approaches to the extreme-ultraviolet…

Atomic Physics · Physics 2015-05-27 P. Tzallas , E. Skantzakis , L. A. A. Nikolopoulos , G. D. Tsakiris , D. Charalambidis

The effective transparency of rare-gas clusters, post-interaction with an extreme ultraviolet (XUV) pump pulse, is predicted by using an atomistic hybrid quantum-classical molecular dynamics model. We find there is an intensity range for…

Atomic and Molecular Clusters · Physics 2016-06-21 Rishi Pandit , Kasey Barrington , Thomas Teague , Zachary Hartwick , Nicolas Bigaouette , Lora Ramunno , Edward Ackad

Coherent light pulses of few to hundreds of femtoseconds (fs) duration have prolifically served the field of ultrafast phenomena. While fs pulses address mainly dynamics of nuclear motion in molecules or lattices in the gas, liquid or…

Chemical Physics · Physics 2013-04-26 P. A. Carpeggiani , P. Tzallas , A. Palacios , D. Gray , F. Martín , D. Charalambidis

The ionization dynamics of a Xenon cluster with 40 atoms is analyzed under a pum p probe scenario of laser pulses where an infrared laser pulse of 50 fs length follows with a well defined time delay a VUV pulse of the same length and peak…

Atomic and Molecular Clusters · Physics 2009-11-10 Ch. Siedschlag , J. M. Rost

A method to generate an intense isolated few-cycle attosecond XUV pulse is demonstrated using particle-in-cell simulations. When a tailored laser pulse with a sharp edge irradiates a foil target, a strong transverse net current can be…

Plasma Physics · Physics 2014-06-13 Zi-Yu Chen , Xiao-Ya Li , Li-Ming Chen , Yu-Tong Li , Wen-Jun Zhu

We investigate theoretically electron dynamics under a VUV attosecond pulse train which has a controlled phase delay with respect to an additional strong infrared laser field. Using the strong field approximation and the fact that the…

Atomic Physics · Physics 2015-05-13 P. Riviere , O. Uhden , U. Saalmann , J. M. Rost

We investigate the wavelength dependent ionization, heating, and expansion dynamics of medium-sized rare-gas clusters (Ar$_{923}$) under intense femtosecond short-wavelength free electron laser pulses by quasi-classical molecular dynamics…

Atomic and Molecular Clusters · Physics 2015-05-20 Mathias Arbeiter , Thomas Fennel

Extreme ultraviolet (XUV) attosecond pulses, generated by a process known as laser-induced electron recollision, are a key ingredient for attosecond metrology, providing a tool to precisely initiate and probe sub-femtosecond dynamics in the…

Atomic Physics · Physics 2016-02-24 Yunpei Deng , Zhinan Zeng , Zhengmao Jia , Pavel Komm , Yinhui Zheng , Xiaochun Ge , Ruxin Li , Gilad Marcus

An extreme ultraviolet (EUV) single attosecond pulse passing through a laser-dressed dense gas is studied theoretically. The weak EUV pulse pumps the helium gas from the ground state to the 2s2p(1P) autoionizing state, which is coupled to…

Atomic Physics · Physics 2013-01-18 Wei-Chun Chu , C. D. Lin

We report the generation and characterization of isolated attosecond XUV and VUV pulses generated simultaneously via HHG driven by few-cycle pulses using an in-line dual gas target system. One gas jet target was operated with Kr gas that…

Optics · Physics 2013-11-20 D. Fabris , W. A. Okell , D. Walke , T. Witting , J. P. Marangos , J. W. G. Tisch

Semi-classical molecular dynamics simulations of small rare gas clusters in short laser pulses of 100 nm wavelength were performed. For comparison, the cluster response to 800 nm laser pulses was investigated as well. The inner ionization…

Atomic and Molecular Clusters · Physics 2009-11-10 D. Bauer

The quantum-classical hybrid-description of rare-gas clusters interacting with intense light pulses which we have developed is described in detail. Much emphasis is put on the treatment of screening electrons in the cluster which set the…

Atomic and Molecular Clusters · Physics 2011-11-09 Ionut Georgescu , Ulf Saalmann , Jan M. Rost

Extreme-ultraviolet pulses can propagate through ionised solid-density targets, unlike optical pulses and, thus, have the potential to probe the interior of such plasmas on sub-femtosecond timescales. We present a synthetic diagnostic…

Plasma Physics · Physics 2022-04-27 Andréas Sundström , István Pusztai , Per Eng-Johnsson , Tünde Fülöp

Ultrafast phenomena on a femtosecond timescale are commonly examined by pump-probe experiments. This implies multiple measurements where the sample under investigation is pumped with a short light pulse and then probed with a second pulse…

A coherent vibrational wavepacket is launched and manipulated in the symmetric stretch (a$_1$) mode of CBr$_4$, by impulsive stimulated Raman scattering from non-resonant 400 nm laser pump pulses with various peak intensities on the order…

We present a new mechanism of attosecond extreme-ultraviolet (XUV) pulses generation from a relativistic laser-driven overdense plasma surfaces in the wavebreaking regime. Through particle-in-cell simulations and analysis, we demonstrate…

Plasma Physics · Physics 2016-08-18 Zi-Yu Chen , Mykyta Cherednychek , Alexander Pukhov

Natively, atomic and molecular processes develop in a sub-femtosecond time scale. In order to, for instance, track and capture the electron motion in that scale we need suitable `probes'. Attosecond pulses configure the most appropriate…

High-intensity extreme ultraviolet (XUV) pulses from a free-electron laser can be used to create a nanoplasma in clusters. In Ref. [Michiels et al. PCCP, 2020; 22: 7828-7834] we investigated the formation of excited states in an XUV-induced…

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