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The persistence length of a single, strongly charged, stiff polyelectrolyte chain is investigated theoretically. Path integral formulation is used to obtain the effective electrostatic interaction between the monomers. We find significant…

Soft Condensed Matter · Physics 2009-11-07 Gil Ariel , David Andelman

We study at- and out-of-equilibrium dynamics of a single homopolymer chain at low temperature using molecular dynamics simulations. The main quantities of interest are the average root mean square displacement of the monomers below the…

Soft Condensed Matter · Physics 2009-11-07 Nikolay V. Dokholyan , Estelle Pitard , Sergey V. Buldyrev , H. Eugene Stanley

We study the interplay of intrinsic-electronic and environmental factors on long-range charge transport across molecular chains with up to $N\sim 80$ monomers. We describe the molecular electronic structure of the chain with a tight-binding…

Mesoscale and Nanoscale Physics · Physics 2022-09-21 Francisco Lai Liang , Dvira Segal

Despite a mounting evidence that the same gradients which active colloids use for swimming, induce important cross-interactions (phoretic interaction), they are still ignored in most many-body descriptions, perhaps to avoid complexity and a…

Soft Condensed Matter · Physics 2019-02-20 B. Liebchen , H. Löwen

The dynamics of a heteropolymer chain in solution is studied in the limit of long chain length. Using functional integral representation we derive an effective equation of motion, in which the heterogeneity of the chain manifests itself as…

Condensed Matter · Physics 2009-10-28 Jiunn-Ren Roan , E. I. Shakhnovich

Cellular biology abound with filaments interacting through fluids, from intracellular microtubules, to rotating flagella and beating cilia. While previous work has demonstrated the complexity of capturing nonlocal hydrodynamic interactions…

Fluid Dynamics · Physics 2016-12-21 Yi Man , Lyndon Koens , Eric Lauga

A large-scale molecular dynamics simulation is performed on a glass-forming Lennard-Jones mixture to determine the nature of dynamical heterogeneities which arise in this model fragile liquid. We observe that the most mobile particles…

Disordered Systems and Neural Networks · Physics 2009-10-30 Claudio Donati , Jack F. Douglas , Walter Kob , Steven J. Plimpton , Peter H. Poole , Sharon C. Glotzer

The hydrodynamic interactions among bacterial cell bodies, flagella, and surrounding boundaries are essential for understanding bacterial motility in complex environments. In this study, we demonstrate that each slender flagellum can be…

Soft Condensed Matter · Physics 2025-01-07 Baopi Liu , Lu Chen , Ji Zhang

Minute amount of long chain flexible polymer dissolved in a turbulent flow can drastically change flow properties, such as reducing the drag and enhancing mixing. One fundamental riddle is how these polymer additives interact with the…

Fluid Dynamics · Physics 2021-02-02 Yi-Bao Zhang , Eberhard Bodenschatz , Haitao Xu , Heng-Dong Xi

The flow-driven transport of interacting micron-sized particles occurs in many soft matter systems spanning from the translocation of proteins to moving emulsions in microfluidic devices. Here we combine experiments and theory to…

Soft Condensed Matter · Physics 2022-11-16 Dominik Lips , Eric Cereceda-López , Antonio Ortiz-Ambriz , Pietro Tierno , Artem Ryabov , Philipp Maass

We study the propulsion of a one-dimensional (1D) polymer chain under sinusoidal external forces in the overdamped (low Reynolds number) regime. We show that, when hydrodynamical interactions are included, the polymer presents directional…

Soft Condensed Matter · Physics 2012-09-25 Daniel Santos-Oliván , Alessandro Fiasconaro , Fernando Falo

Generic interacting many-body quantum systems are believed to behave as classical fluids on long time and length scales. Due to rapid progress in growing exceptionally pure crystals, we are now able to experimentally observe this collective…

Strongly Correlated Electrons · Physics 2018-01-08 Andrew Lucas , Kin Chung Fong

We study the mobility of a charged colloidal particle in a constant homogeneous electric field by means of computer simulations. The simulation method combines a lattice Boltzmann scheme for the fluid with standard Langevin dynamics for the…

Soft Condensed Matter · Physics 2007-06-20 Vladimir Lobaskin , Burkhard Duenweg , Christian Holm

Several recent experiments suggest that rather generally the diffusion of enzymes may be augmented through their activity. We demonstrate that such swimming motility can emerge from the interplay between the enzyme energy landscape and the…

Soft Condensed Matter · Physics 2015-10-08 Xiaoyu Bai , Peter G. Wolynes

We present a hydrodynamic theory describing pair diffusion in systems with periodic boundary conditions, thereby generalizing earlier work on self-diffusion [D\"unweg and Kremer, J. Chem. Phys. 1993, 99, 6983-6997; Yeh and Hummer, J. Phys.…

Soft Condensed Matter · Physics 2023-05-03 Diddo Diddens , Andreas Heuer

We study the electrokinetics of a single polyelectrolyte chain in salt solution using hydrodynamic simulations. The salt-dependent chain mobility compares well with experimental DNA data. The mobility of condensed counterions exhibits a…

Soft Condensed Matter · Physics 2009-05-26 Sebastian Fischer , Ali Naji , Roland R. Netz

Over times shorter than that required for relaxation of enthalpy, a liquid can exhibit striking heterogeneities. The picture of these heterogeneities is complex with transient patches of rigidity, irregular yet persistent, intersected by…

Soft Condensed Matter · Physics 2010-09-30 Peter Harrowell

We report an extensive and systematic investigation of the multi-point and multi-time correlation functions to reveal the spatio-temporal structures of dynamic heterogeneities in glass-forming liquids. Molecular dynamics simulations are…

Soft Condensed Matter · Physics 2013-01-04 Kang Kim , Shinji Saito

We investigate ion and polymer dynamics in polymer electrolytes PPO-LiClO4 performing 2H and 7Li NMR line-shape analysis. Comparison of temperature dependent 7Li and 2H NMR spectra gives evidence for a coupling of ion and polymer dynamics.…

Materials Science · Physics 2009-11-11 M. Vogel , T. Thorbrugge

The recent discovery of electro-active polymers has shown great promises in the field of soft robotics, and was logically followed by experimental, numerical and theoretical developments. Most of these studies were concerned with systems…

Soft Condensed Matter · Physics 2020-12-07 Hadrien Bense , Benoît Roman , Bruno Andreotti