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By analyzing ``exact'' theoretical results from solving the time-dependent Schr\"odinger equation of atoms in few-cycle laser pulses, we established the general conclusion that differential elastic scattering and photo-recombination cross…

Atomic Physics · Physics 2008-04-04 Toru Morishita , Anh-Thu Le , Zhangjin Chen , C. D. Lin

Compton scattering of short and ultra short (sub-cycle) laser pulses off mildly relativistic electrons is considered within a QED framework. The temporal shape of the pulse is essential for the differential cross section as a function of…

High Energy Physics - Phenomenology · Physics 2015-06-22 Alexander I. Titov , Burkhard Kampfer , Takuya Shibata , Atsushi Hosaka , Hideaki Takabe

Ultrafast imaging of molecular chirality is a key step towards the dream of imaging and interpreting electronic dynamics in complex and biologically relevant molecules. Here, we propose a new ultrafast chiral phenomenon exploiting recent…

A detailed analysis of the photon emission spectra of an electron scattered by a laser pulse containing only very few cycles of the carrying electromagnetic field is presented. The analysis is performed in the framework of strong-field…

High Energy Physics - Phenomenology · Physics 2011-03-21 F. Mackenroth , A. Di Piazza

The requirement of high space-time resolution and brightness is a great challenge for imaging atomic motion and making molecular movies. Important breakthroughs in ultrabright tabletop laser, x-ray and electron sources have enabled the…

Atomic Physics · Physics 2022-02-10 Ming Zhang , Zhenning Guo , Xiaoyu Mi , Zheng Li , Yunquan Liu

Imaging structures at the molecular level is a fast developing interdisciplinary research field that spans across the boundaries of physics and chemistry. High spatial resolution images of molecules can be obtained with photons or ultrafast…

Atomic Physics · Physics 2016-09-01 R. Puthumpally-Joseph , J. Viau-Trudel , M. Peters , T. T. Nguyen-Dang , O. Atabek , E. Charron

We theoretically study the inelastic electron-H($2s$) scattering in a linearly polarized laser field in the domain of high scattering energies and moderate field intensities. We investigate the angular distributions and the resonance…

Atomic Physics · Physics 2023-09-04 Gabriela Buica

We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show…

Atomic Physics · Physics 2012-10-02 Michel Peters , Tung Nguyen-Dang , Eric Charron , Arne Keller , Osman Atabek

Spatial distributions of electrons ionized and scattered from ultra-low pressure gases are proposed and experimentally demonstrated as a method to directly measure the intensity of an ultra-high intensity laser pulse. Analytic models…

Inverse Compton scattering (ICS) is a unique mechanism for producing fast pulses - picosecond and below - of bright X- to gamma-rays. These nominally narrow spectral bandwidth electromagnetic radiation pulses are efficiently produced in the…

We demonstrate how the technique of ultrafast resonant x-ray scattering can be applied to imaging dynamics of electronic wave packets in crystals. We study scattering patterns from crystals with electron dynamics in valence bands taking…

Optics · Physics 2018-12-11 Daria Popova-Gorelova , Robin Santra

The advent of ultrafast pulsed X-ray free-electron lasers with very high brightness has enabled the determination of transient molecular structures of small and medium-sized organic molecules in excited states and undergoing chemical…

Chemical Physics · Physics 2025-10-07 Peter M. Weber , Brian Stankus , Adam Kirrander

We consider solid surface scattering of molecules that were subject to strong non-resonant ultrashort laser pulses just before hitting the surface. The pulses modify the rotational states of the molecules, causing their field free…

Chemical Physics · Physics 2015-06-12 Yuri Khodorkovsky , J. R. Manson , Ilya Sh. Averbukh

Ultrashort laser pulses that last only a few optical cycles have been transformative tools for studying and manipulating light--matter interactions. Few-cycle pulses are typically produced from high-peak-power lasers, either directly from a…

Irradiation of solid surfaces with intense ultrashort laser pulses represents a unique way of depositing energy into materials. It allows to realize states of extreme electronic excitation and/or very high temperature and pressure, and to…

We investigated the two-dimensional electron momentum distributions of atomic negative ions in an intense laser field by solving the time-dependent Schrodinger equation (TDSE) and using the first- and 2nd-order strong-field approximations…

Atomic Physics · Physics 2009-11-13 XiaoXin Zhou , Zhangjin Chen , Toru Morishita , Anh-Thu Le , C. D. Lin

A comprehensive quantitative rescattering (QRS) theory for describing the production of high-energy photoelectrons generated by intense laser pulses is presented. According to the QRS, the momentum distributions of these electrons can be…

Atomic Physics · Physics 2009-11-13 Zhangjin Chen , Anh-Thu Le , Toru Morishita , C. D. Lin

Using a quantum wave packet simulation including the nuclear and electronic degrees of freedom, we investigate the femtosecond and picosecond energy- and angle-resolved photoelectron spectra of the E($^1\Sigma_g^+$) electronic state of…

Chemical Physics · Physics 2019-04-04 R. Chamakhi , R. Puthumpally-Joseph , M. Telmini , E. Charron

We experimentally observe the action of multiple light pulses on the transverse motion of a continuous beam of fullerenes. The light potential is generated by non-resonant ultra-short laser pulses in perpendicular spatial overlap with the…

Atomic and Molecular Clusters · Physics 2013-07-02 Paul Venn , Hendrik Ulbricht

Laser-induced electron diffraction is an evolving tabletop method, which aims to image ultrafast structural changes in gas-phase polyatomic molecules with sub-{\AA}ngstr\"om spatial and femtosecond temporal resolution. Here, we provide the…

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