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Electron spin resonance (ESR), at 9, 94, and 190 GHz, and magnetization studies on polycrystalline, powder, and ultrafine powder samples of Ni(C3H10N2)2N3(ClO4) (NINAZ) have revealed several effects arising from the Haldane phase. Using the…

Two quasi-1-dimensional S=1 quantum antiferromagnetic materials, PbNi2V2O8 and SrNi2V2O8, are studied by inelastic neutron scattering on powder samples. While magnetic interactions in the two systems are found to be very similar, subtle…

Strongly Correlated Electrons · Physics 2009-10-31 A. Zheludev , T. Masuda , I. Tsukada , Y. Uchiyama , K. Uchinokura , P. Boni , S. -H. Lee

We report an inelastic neutron scattering study of antiferromagnetic spin dynamics in the Haldane chain compound Ni(C2H8N2)2NO2ClO4 (NENP) under external hydrostatic pressure P = 2.5 GPa. At ambient pressure, the magnetic excitations in…

Condensed Matter · Physics 2016-08-31 I. A. Zaliznyak , D. C. Dender , C. Broholm , Daniel H. Reich

The molecular coordination complex NiI$_2$(3,5-lut)$_4$ [where (3,5-lut) $=$ (3,5-lutidine) $=$ (C$_7$H$_9$N)] has been synthesized and characterized by several techniques including synchrotron X-ray diffraction, ESR, SQUID magnetometry,…

We report experimental results of the static magnetization, ESR and NMR spectroscopic measurements of the Ni-hybrid compound NiCl$_3$C$_6$H$_5$CH$_2$CH$_2$NH$_3$. In this material NiCl$_3$ octahedra are structurally arranged in chains along…

Strongly Correlated Electrons · Physics 2018-02-22 F. Lipps , A. H. Arkenbout , A. Polyakov , M. Günther , T. Salikhov , E. Vavilova , H. -H. Klauss , B. Büchner , T. M. Palstra , V. Kataev

Low-lying excited states as well as the ground state of the spin-1 antiferromagnetic Heisenberg chain with a spin-1/2 impurity are studied by means of a method of numerical diagonalization. The isotropic nearest-neighbor exchange coupling…

Condensed Matter · Physics 2009-10-28 Takashi Tonegawa , Makoto Kaburagi

Inelastic neutron scattering was used to probe edge states in a quantum spin liquid. The experiment was performed on finite length antiferromagnetic spin-1 chains in Y_2BaNi_{1-x}Mg_xO_5. At finite fields, there is a Zeeman resonance below…

Strongly Correlated Electrons · Physics 2009-11-07 M. Kenzelmann , G. Xu , I. A. Zaliznyak , C. Broholm , J. F. DiTusa , G. Aeppli , T. Ito , K. Oka , H. Takagi

We consider spin-1 Haldane chains with single-ion anisotropy, which exists in known Haldane chain materials. We develop a perturbation theory in terms of anisotropy, where magnon-magnon interaction is important even in the low temperature…

Statistical Mechanics · Physics 2011-11-22 Shunsuke C. Furuya , Takafumi Suzuki , Shintaro Takayoshi , Yoshitaka Maeda , Masaki Oshikawa

We present electron spin resonance experiments in the one-dimensional antiferromagnetic S=1 spin chains NENP and NINO in pulsed magnetic fields up to 50T. The measured field dependence of the quantum energy gap for B||b is analyzed using…

Strongly Correlated Electrons · Physics 2009-10-31 M. Sieling , U. Löw , B. Wolf , S. Schmidt , S. Zvyagin , B. Lüthi

This paper overviews the behavior of the end-chain spins of linear chain systems possessing a Haldane gap. The physical properties of the end-chain spins are described by reviewing the results obtained primarily with materials known as…

Condensed Matter · Physics 2007-05-23 Mark W. Meisel

The impurity-induced antiferromagnetic ordering of the doped Haldane magnet Pb(Ni{1-x}Mg{x})2V2O8 (0 < x <0.06) was studied by electron spin resonance (ESR) on ceramic samples in the frequency range 9-110 GHz. Below the N\'{e}el temperature…

Strongly Correlated Electrons · Physics 2009-11-07 A. I. Smirnov , V. N. Glazkov , H. -A. Krug von Nidda , A. Loidl , L. N. Demianets , A. Ya. Shapiro

We investigate magnetic and thermodynamic properties of a spin-1 Heisenberg diamond chain in a magnetic field using a combination of analytical and numerical methods including the variational approach, exact diagonalization, density-matrix…

Statistical Mechanics · Physics 2025-10-22 Azam Zoshki , Hamid Arian Zad , Katarina Karlova , Jozef Strecka

We performed single-crystal magnetic susceptibility and $^1$H NMR measurements on a quasi-1D, spin-1 antiferromagnet NiC$_2$O$_4$$\cdot$2NH$_3$, with temperature down to 100 mK and with field up to 26 T. With field applied along the chain…

Strongly Correlated Electrons · Physics 2025-06-02 Shuo Li , Zhanlong Wu , Yanhong Wang , Jun Luo , Kefan Du , Xiaoyu Xu , Ze Hu , Ying Chen , Jie Yang , Zhengxin Liu , Rong Yu , Yi Cui , Rui Zhou , Hongcheng Lu , Weiqiang Yu

We consider quasi one dimensional spin-1 Heisenberg chains with crystal field anisotropy in a uniform magnetic field. We determine the dynamical structure factor in various limits and obtain a fairly complete qualitative picture of how it…

Strongly Correlated Electrons · Physics 2009-11-10 Fabian H. L. Essler , Ian Affleck

Inelastic neutron scattering on deuterated single-crystal samples is used to study Haldane-gap excitations in the new S=1 one-dimensional quantum antiferromagnet NDMAP, that was recently recognized as an ideal model system for high-field…

Strongly Correlated Electrons · Physics 2009-10-31 A. Zheludev , Y. Chen , C. L. Broholm , Z. Honda , K. Katsumata

Impurity effect is systematically studied in doped Haldane material Pb(Ni$_{1-x}$$M_x$)$_2$V$_2$O$_8$ ($M$ = Mn, Co, Cu, and Mg) by use of DC and AC susceptibility, and heat capacity measurements. The occurrence of three-dimensional ordered…

Strongly Correlated Electrons · Physics 2007-05-23 S. Imai , T. Masuda , T. Matsuoka , K. Uchinokura

We report the results of elastic and inelastic neutron scattering experiments on the Haldane gap quantum antiferromagnet Ni(C5D14N2)2N3(PF6) performed at mK temperatures in a wide range of magnetic field applied parallel to the S = 1 spin…

Linear-chain nickelates with the composition (Nd_x Y_{1-x})_2 Ba Ni O_5 (x=1, x=0.75, x=0.5, and x=0.25) are studied in a series of neutron scattering experiments. Powder diffraction is used to determine the temperature dependence of the…

Strongly Correlated Electrons · Physics 2008-12-18 T. Yokoo , S. Raymond , A. Zheludev , S. Maslov , E. Ressouche , I. Zaliznyak , R. Erwin , M. Nakamura , J. Akimitsu

Magnetic susceptibility, high-field magnetization and inelastic neutron scattering experiments are used to study the magnetic properties of a new S=1 quasi-1-dimensional antiferromagnet PbNi2V2O8. Inter-chain interactions are shown to be…

Strongly Correlated Electrons · Physics 2009-10-31 Y. Uchiyama , Y. Sasago , I. Tsukada , K. Uchinokura , A. Zheludev , T. Hayashi , N. Miura , P. Böni

The NMR relaxation rates of (quasi-)one-dimensional spin gapped systems such as the $S=1/2$ spin ladder with a diagonal interaction and the Haldane-gap system are investigated at low temperatures in magnetic fields. We show that in the…

Strongly Correlated Electrons · Physics 2009-10-31 Nobuyasu Haga , Sei-ichiro Suga
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