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Coherent control of femtosecond two-photon absorption in the intermediate-field regime is analyzed in detail in the powerful frequency domain using an extended 4th-order perturbative description. The corresponding absorption is coherently…

Atomic Physics · Physics 2008-01-24 Lev Chuntonov , Leonid Rybak , Andrey Gandman , Zohar Amitay

We present and implement a new scheme for extended multi-channel selective femtosecond coherent control based on symmetry properties of the excitation channels. Here, an atomic non-resonant two-photon absorption channel is coherently…

Atomic Physics · Physics 2008-05-17 Andrey Gandman , Lev Chuntonov , Leonid Rybak , Zohar Amitay

We extend the powerful frequency-domain analysis of femtosecond two-photon absorption to the intermediate-field regime, which involves both two- and four-photon transitions. Consequently, we find a broad family of shaped pulses that enhance…

Atomic Physics · Physics 2008-02-20 Lev Chuntonov , Leonid Rybak , Andrey Gandman , Zohar Amitay

We demonstrate and study the enhancement of intermediate-field two-photon absorption by shaped femtosecond pulses having spectral phases of antisymmetric nature. The intermediate-field regime corresponds to pulse intensities, where the…

Atomic Physics · Physics 2015-05-14 Lev Chuntonov , Leonid Rybak , Andrey Gandman , Zohar Amitay

We present and implement a new scheme for independent control of both the final and the transient population utilizing the symmetry properties of the system. By proper pulse shaping, utilizing the invariance of the two-photon absorption to…

Atomic Physics · Physics 2009-10-20 Andrey Gandman , Leonid Rybak , Michal Bronstein , Naser Shakour , Zohar Amitay

Coherent control of the atomic two-photon absorption with shaped single-cycle pulses is examined theoretically in the weak-field regime. The control over the stabilized carrier-envelope phase (CEP) of the pulses is determined as a key…

Atomic Physics · Physics 2009-10-21 Lev Chuntonov , Avner Fleischer , Zohar Amitay

We introduce a new scheme for generating short-wavelength coherent broadband radiation with well-controlled spectral characteristics. It is based on shaping long-wavelength femtosecond pulse to coherently control atomic resonance-mediated…

Atomic Physics · Physics 2009-10-20 Leonid Rybak , Lev Chuntonov , Andrey Gandman , Naser Shakour , Zohar Amitay

We study the evolution of a V-type three-level system, whose two resonances are coherently excited and coupled by two ultrashort laser pump and probe pulses, separated by a varying time delay. We relate the quantum dynamics of the excited…

Atomic Physics · Physics 2015-04-02 Z. Liu , S. M. Cavaletto , C. Ott , K. Meyer , Y. Mi , Z. Harman , C. H. Keitel , T. Pfeifer

Dissipation of electromagnetic energy through absorption is a fundamental process that underpins phenomena ranging from photovoltaics to photography, analytical spectroscopy, photosynthesis, and human vision. Absorption is also a dynamic…

Optics · Physics 2022-09-13 Venkatram Nalla , Xu Fang , João Valente , Handong Sun , Nikolay I Zheludev

We present a theoretical study of three-photon electromagnetically induced absorption for a ladder-type three-level atomic system. A probe beam was tuned to the lower line and two counter-propagating, linearly polarized coupling beams were…

Atomic Physics · Physics 2015-08-03 Heung-Ryoul Noh , Han Seb Moon

The transient-absorption spectrum of a $V$-type three-level system is investigated, when this is periodically excited by a train of equally spaced, $\delta$-like pump pulses as, e.g., from an optical-frequency-comb laser. We show that, even…

Atomic Physics · Physics 2019-01-30 Juliane Haug , Stefano M. Cavaletto

The dynamics of a system interacting with an ultrashort pulse is known to depend on the phase content of said pulse. For linear absorption, phase control is possible over time-varying quantities, such as the population of metastable states,…

Chemical Physics · Physics 2019-10-31 Cyrille Lavigne , Paul Brumer

We investigate how the quantum control of a two-level system (TLS) coupled to photons can modify and tune the TLS's photon absorption spectrum. Tuning and controlling the emission and the absorption is of much interest e.g.\ for the…

Quantum Physics · Physics 2017-06-07 H. F. Fotso , V. V. Dobrovitski

The effect of quantum interference on the optical properties of a pumped-probe three-level V-type atomic system is investigated. The probe absorption, dispersion, group index and optical bistability beyond the two-photon resonance condition…

Quantum Physics · Physics 2015-06-04 S. M. Mousavi , L. Safari , M. Mahmoudi , M. Sahrai

We present a theoretical analysis of two-photon absorption of classical and squeezed light valid when one-photon absorption to an intermediate state is either resonant or far-detuned from resonance, and in both the low and high intensity…

Quantum Physics · Physics 2022-09-14 Christian Drago , John Sipe

We theoretically show that energy absorption in crystalline silicon can be controlled by two-color femtosecond double-pulse irradiation, in which two temporally separated pulses with different wavelengths interact sequentially with the…

Materials Science · Physics 2026-04-29 Eiyu S. Gushiken , Mizuki Tani , Hiroki Katow , Kenichi L. Ishikawa

The quantum dynamics of a system of Rb atoms, modeled by a V-type three-level system interacting with intense probe and pump pulses, are studied. The time-delay-dependent transient-absorption spectrum of an intense probe pulse is thus…

Atomic Physics · Physics 2018-02-14 Vadim Becquet , Stefano M. Cavaletto

Tho-photon absorption holds potential for many practical applications. We theoretically investigate the onset of this phenomenon in a semiconductor quantum dot -- metallic nanoshell composite subjected to a resonant CW excitation.…

Mesoscale and Nanoscale Physics · Physics 2021-01-08 Bintoro S. Nugroho , Alexander A. Iskandar , Victor A. Malyshev , Jasper Knoester

V-type three-level systems, where two excited states share a common ground state, serve as fundamental models for exploring coherent light-matter interactions in a range of quantum systems, from atomic gases to semiconductor nanostructures.…

Quantum Physics · Physics 2026-05-12 Rishabh Tripathi , Krishna K. Maurya , Rohan Singh

By combining genetic algorithm and a spatial light modulator we theoretically analyse how to improve a two-photon cascade absorption in atomic ensembles, inspecting the impact of various configurations and parameters in the optimized phase…

Atomic Physics · Physics 2026-02-24 L. B. A. Mélo , Daniel Felinto , Marcio H. G. de Miranda
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