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The rich information of electron energy-loss spectroscopy (EELS) comes from the complex inelastic scattering process whereby fast electrons transfer energy and momentum to atoms, exciting bound electrons from their ground states to higher…

We present an absolute extraction method of optical constants of metal from the measured reflection electron energy loss (REELS) spectra by using the recently developed reverse Monte Carlo (RMC) technique. The method is based on a direct…

Materials Science · Physics 2017-05-24 H. Xu , B. Da , J. Toth , K. Tokesi , Z. J. Ding

A simple procedure is developed to simultaneously eliminate multiple scattering contributions from two reflection electron energy loss spectra (REELS) measured at different energies or for different experimental geometrical configurations.…

Materials Science · Physics 2009-11-11 Wolfgang S. M. Werner

A consistent theory of electron energy-loss spectroscopy (EELS) includes two indispensable elements: (i) electronic response of the target system and (ii) quantum kinematics of probing electrons. While for the bulk materials and their…

Mesoscale and Nanoscale Physics · Physics 2017-12-12 Vladimir U. Nazarov , Vyacheslav M. Silkin , Eugene E. Krasovskii

A fully relativistic description of the electron energy loss and the induced radiation emission in arbitrary arrays of non-overlapping metallic cylinders is presented in terms of the multiple scattering method on the basis of vector…

Materials Science · Physics 2009-11-10 T. Ochiai , K. Ohtaka

Electron beam energies in Transmission Electron Microscopes (TEMs) reach the relativistic realm constituting Quantum Electrodynamics (QED) the appropriate framework for the study of electron matter interaction in TEMs. We focus on the…

Atomic Physics · Physics 2026-01-12 Ioannis Iatrakis , Valerii Brudanin

We study the electron-energy loss spectra of strongly correlated electronic systems doped away from half-filling using dynamical mean-field theory ($d=\infty$). The formalism can be used to study the loss spectra in the optical (${\bf…

Strongly Correlated Electrons · Physics 2009-10-31 Luis Craco , Mukul S. Laad

Recently it has been demonstrated that a careful treatment of both longitudinal and transverse matrix elements in electron energy loss spectra can explain the mystery of relativistic effects on the {\it magic angle}. Here we show that there…

Materials Science · Physics 2009-11-13 A. P. Sorini , J. J. Rehr , Z. H. Levine

Swift electrons passing near or through metallic structures have proven to be an excellent tool for studying plasmons and other types of confined optical modes involving collective charge oscillations in the materials hybridized with…

Low-loss electron energy loss spectroscopy (EELS) in the scanning transmission electron microscope (STEM) probes the valence electron density and relevant optoelectronic properties such as band gap energies and other band structure…

Materials Science · Physics 2018-11-20 Alberto Eljarrat , Christoph T. Koch

A procedure is developed to rigorously decompose experimental loss spectra of medium-energy electrons reflected from solid surfaces into contributions due to surface and volume electronic excitations. This can be achieved by analysis of two…

Materials Science · Physics 2009-11-11 Wolfgang S. M. Werner

We calculate electron energy loss spectra (EELS) for composite plasmonic structures based on silicene and germanene. A continued-fraction expression for the effective dielectric function is used to perform multiscale calculations of EELS…

Materials Science · Physics 2013-11-05 L. Rast , V. K. Tewary

Electron microscopy prevalently uses energy-dispersive x-ray spectroscopy (EDS) and electron energy loss spectroscopy (EELS) for elemental analysis. EDS and EELS energy resolutions are commonly between 30-100 eV or 0.01-1 eV, respectively.…

Inelastic scattering of electrons incident on a solid surface is determined by the two properties: (i) electronic response of the target system and (ii) the detailed quantum-mechanical motion of the projectile electron inside and in the…

Materials Science · Physics 2016-01-06 V. U. Nazarov , V. M. Silkin , E. E. Krasovskii

A simple method is proposed for inclusion of inelastic effects (electron absorption) in computations of low-energy electron reflectivity (LEER) spectra. The theoretical spectra are formulated by matching of electron wavefunctions obtained…

Mesoscale and Nanoscale Physics · Physics 2023-05-03 Qin Gao , P. C. Mende , M. Widom , R. M. Feenstra

In this paper convexity constraints are derived for a background model of electron energy loss spectra (EELS) that is linear in the fitting parameters. The model outperforms a power-law both on experimental and simulated backgrounds,…

Data Analysis, Statistics and Probability · Physics 2023-08-31 Wouter Van den Broek , Daen Jannis , Jo Verbeeck

The normalized differential mean free path for volume scattering and the differential surface excitation probability for medium energy electrons travelling in Fe, Pd and Pt are extracted from Reflection Electron Energy Loss Spectra (REELS).…

Materials Science · Physics 2009-11-11 Wolfgang S. M. Werner

The real-space Green's function code FEFF has been extensively developed and used for calculations of x-ray and related spectra, including x-ray absorption (XAS), x-ray emission (XES), inelastic x-ray scattering, and electron energy loss…

Materials Science · Physics 2021-06-28 J. J. Kas , F. D. Vila , J. J. Rehr , C. D. Pemmaraju , T. S. Tan

A general theory for the core-level electron excitation of anisotropic systems using angular integrated electron energy-loss spectroscopy has been derived. We show that it is possible to define a magic angle condition at which the specimen…

Materials Science · Physics 2007-05-23 Y. K. Sun , J. Yuan

A technique to measure the band gap of dielectric materials with high refractive index by means of energy electron loss spectroscopy (EELS) is presented. The technique relies on the use of a circular (Bessel) aperture and suppresses…

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