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Related papers: Phonon anharmonicities in graphite and graphene

200 papers

We present a first-principles study of the electron-phonon (e-ph) interactions and their contributions to the linewidths for the optical phonon modes at $\Gamma$ and K in one to three-layer graphene. It is found that due to the interlayer…

Materials Science · Physics 2009-03-31 Jia-An Yan , W. Y. Ruan , M. Y. Chou

We have investigated the anisotropic thermal expansion of graphite using ab-initio calculation of lattice dynamics and anharmonicity of the phonons, which reveal that the negative thermal expansion (NTE) in the a-b plane below 600 K and…

Materials Science · Physics 2021-05-05 Ranjan Mittal , Mayanak K. Gupta , Baltej Singh , S. K. Mishra , Samrath L. Chaplot

Radio-frequency compressed ultrafast electron diffraction has been used to probe the coherent and incoherent coupling of impulsive electronic excitation at 1.55 eV (800 nm) to optical and acoustic phonon modes directly from the perspective…

Materials Science · Physics 2015-06-23 Robert P. Chatelain , Vance R. Morrison , Bart L. M. Klarenaar , Bradley J. Siwick

Understanding thermal transport in 2D materials and especially in graphene is a key challenge for the design of heat management and energy conversion devices. The high sensitivity of measured transport properties to structural defects,…

Materials Science · Physics 2020-06-24 G. Bouzerar , S. Thébaud , S. Pecorario , Ch. Adessi

The anharmonic behavior of phonons and intrinsic thermal conductivity associated with the Umklapp scattering in monolayer MoS2 sheet are investigated via first-principles calculations within the framework of density functional perturbation…

Materials Science · Physics 2015-06-18 Yongqing Cai , Jinghua Lan , Gang Zhang , Yong-Wei Zhang

Anharmonic decay of coherent optical phonons in semimetal Sb has been investigated by using a femtosecond pump-probe technique. The coherent $A_{1g}$ mode is observed in time domain in a wide temperature range of 7 - 290 K. The decay rate…

Materials Science · Physics 2015-01-12 Muneaki Hase , Kiminori Ushida , Masahiro Kitajima

We derive the frequency shifts and the broadening of $\Gamma$ point longitudinal optical (LO) and transverse optical (TO) phonon modes, due to electron-phonon interaction, in graphene under uniaxial strain as a function of the electron…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Mohamed Assili , Sonia Haddad

The equilibrium optical phonons of graphene are well characterized in terms of anharmonicity and electron-phonon interactions, however their non-equilibrium properties in the presence of hot charge carriers are still not fully explored.…

Mesoscale and Nanoscale Physics · Physics 2018-02-15 C. Ferrante , A. Virga , L. Benfatto , M. Martinati , D. De Fazio , U. Sassi , C. Fasolato , A. K. Ott , P. Postorino , D. Yoon , G. Cerullo , F. Mauri , A. C. Ferrari , T. Scopigno

We present a phenomenological force-constant model developed for the description of lattice dynamics of sp2 hybridized carbon networks. Within this model approach, we introduce a new set of parameters to calculate the phonon dispersion of…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 J. Zimmermann , P. Pavone , G. Cuniberti

The electronic and vibrational properties of 2D materials are dramatically altered by the formation of a moir\'e superlattice. The lowest-energy phonon modes of the superlattice are two acoustic branches (called phasons) that describe the…

We examine the intrinsic energy dissipation steps in electrically biased graphene channels. By combining in-situ measurements of the spontaneous optical emission with a Raman spectroscopy study of the graphene sample under conditions of…

Mesoscale and Nanoscale Physics · Physics 2015-03-13 Stéphane Berciaud , Melinda Y. Han , Louis E. Brus , Philip Kim , Tony F. Heinz

All-carbon heterostructures have been produced recently via focused ion beam patterning of single layer graphene. Amorphized graphene is similar to a graphene sheet in which some hexagons are replaced by a combination of pentagonal,…

Materials Science · Physics 2017-04-07 B Mortazavi , Z Fan , LFC Pereira , A Harju , T Rabczuk

We have performed low temperature scanning tunnelling spectroscopy (STS) measurements on graphene epitaxially grown on Ru(0001). An inelastic feature, related to the excitation of a vibrational breathing mode of the graphene lattice, was…

We investigate the effect of strain and isotopic disorder on thermal transport in suspended graphene by equilibrium molecular dynamics simulations. We show that the thermal conductivity of unstrained graphene, calculated from the…

Materials Science · Physics 2013-08-08 Luiz Felipe C. Pereira , Davide Donadio

Recent advances in strain engineering at the nanoscale have shown the feasibility to modulate the properties of graphene. Although the electron-phonon (e-ph) coupling and Kohn anomalies in graphene define the phonon branches contributing to…

Mesoscale and Nanoscale Physics · Physics 2016-08-02 M. E. Cifuentes-Quintal , O. de la Peña-Seaman , R. Heid , R. de Coss , K. -P. Bohnen

The anharmonicity of the acoustic phonon dispersion of graphene has been studied by the harmonic linear response (HLR) approach at finite temperature. This is a non-perturbative method based on the linear response of the system to applied…

Materials Science · Physics 2020-08-20 R. Ramirez , C. P. Herrero

Allotropes of carbon, such as diamond and graphene, are among the best conductors of heat. We monitored the evolution of thermal conductivity in thin graphite as a function of temperature and thickness and found an intimate link between…

Materials Science · Physics 2020-03-25 Yo Machida , Nayuta Matsumoto , Takayuki Isono , Kamran Behnia

The dominant phonon wavevectors $q^{*}$ probed by the 2D Raman mode of graphene are highly anisotropic and rotate with the orientation of the polarizer:analyzer direction relative to the lattice. The corresponding electronic transitions…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Rohit Narula , Nicola Bonini , Nicola Marzari , Stephanie Reich

Time-domain femtosecond laser spectroscopic measurements of the ultrafast lattice dynamics in 2H-MoTe2 bulk crystals were carried out to understand the carrier-phonon interactions that govern electronic transport properties. An unusually…

Anharmonic lattice vibrations govern the thermal dynamics in materials and present how the atoms interact and how they conduct heat. An indepth understanding of the microscopic mechanism of phonon anharmonicity in condensed systems is…

Materials Science · Physics 2021-12-30 Bin Wei , Qiyang Sun , Chen Li , Jiawang Hong