Related papers: Multiple Quantum NMR Dynamics in Dipolar Ordered S…
Efficient simulations of quantum evolutions of spin-1/2 systems are relevant for ensemble quantum computation as well as in typical NMR experiments. We propose an efficient method to calculate the dynamics of an observable provided that the…
The simulation of nuclear magnetic resonance (NMR) experiments is a notoriously difficult task, if many spins participate in the dynamics. The recently established dynamic mean-field theory for high-temperature spin systems (spinDMFT)…
We theoretically study the nuclear spin dynamics driven by electron transport and hyperfine interaction in an electrically-defined double quantum dot (DQD) in the Pauli-blockade regime. We derive a master-equation-based framework and show…
The identification of spin-nematic states is challenging due to the absence of Bragg peaks. However, the study of dynamical physical quantities provides a promising avenue for characterizing these states. In this study, we investigate the…
We report the first experimental demonstration of quantum delayed-choice experiment via nuclear magnetic resonance techniques. An ensemble of molecules each with two spin-1/2 nuclei are used as target and the ancilla qubits to perform the…
The full design of relevant systems for quantum applications, ranging from quantum simulation to sensing, is presented using a combination of atomistic methods. A prototypical system features a two-dimensional ordered distribution of spins…
Nuclear spins and paramagnetic centers in a solid randomly group to form clusters featuring nearly-degenerate, hybrid states whose dynamics are central to processes involving nuclear spin-lattice relaxation and diffusion. Their…
We study repeated (noncontinuous) measurements on the electron spin in a quantum dot and find that the measurement technique may lead to a different met$ or mechanism to realize nuclear spin polarization. While it may be used in any case,…
Pulsed Dynamic Nuclear Polarization (DNP) is currently receiving substantial interest as a means to enhance the sensitivity of nuclear magnetic resonance (NMR) and magnetic resonance imaging (MRI) by orders of magnitude. It has also…
An open quantum system refers to a system, which is in turn coupled to an environment that can describe time irreversible dynamics through which the system evolves toward the thermal equilibrium state. We present a quantum mechanically…
Coupled electron-nuclear spins represent a promising quantum system, where the optically induced electron spin polarization can be dynamically transferred to nuclear spins via the hyperfine interaction. Most experiments on dynamic nuclear…
A dipolar recoupling technique is introduced as a new approach to quantum gate operation in solid-state NMR under magic angle spinning. The default-off property of inter-qubit interaction provides a simple way to controlled operation…
Researchers have used NMR to measure multi-phase fluid saturation and distribution inside porous media of natural rock. However, the NMR signal amplitude suffers reduction with the increase of temperature. The main reason is the Transverse…
We employ NMR techniques to investigate the nature of Mn spins in the I-II-V diluted magnetic semiconductor Li(Zn1-xMnx)P (x = 0.1, Curie temperature Tc = 25 K). We successfully identify the 7Li NMR signals arising from the Li sites…
We investigate quantum features and non-classical nature of two-spin-$1/2$ NMR systems at thermal equilibrium under external magnetic fields. More specifically, using suitable quantifiers, we analyze quantum coherence, mixedness, and…
Classical simulations of high-temperature nuclear spin dynamics in solids are known to accurately predict relaxation for spin 1/2 lattices with a large number of interacting neighbors. Once the number of interacting neighbors becomes four…
The NMR technique allows one to create a non-equilibrium local polarization and to detect its later evolution. By a change of the sign of the effective dipolar Hamiltonian, the apparently diffusive dynamics is reverted, generating a…
The central spin decoherence problem has been researched for over 50 years in the context of both nuclear magnetic resonance and electron spin resonance. Until recently, theoretical models have employed phenomenological stochastic…
Multirate characterization of spin responses in nuclear magnetic resonance (NMR) is a promising approach to fingerprinting complex molecules in the presence of multiple relaxation mechanisms. Here we present experimental and theoretical…
We demonstrate time reversal of nuclear spin dynamics in highly magnetized dilute liquid 3He-4He mixtures through effective inversion of long-range dipolar interactions. These experiments, which involve using magic sandwich NMR pulse…