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Room-temperature ferromagnetism is observed in (110) oriented ZnO films containing 5 at % of Sc, Ti, V, Fe, Co or Ni, but not Cr, Mn or Cu ions. There are large moments, 1.9 and 0.5 muB/atom for Co- and Ti-substituted oxides, respectively.…

Materials Science · Physics 2009-11-10 M. Venkatesan , C. B. Fitzgerald , J. G. Lunney , J. M. D. Coey

Magnetometry, x-ray, and neutron scattering have been used to study the structural and magnetic properties of a TbMnO3 thin film grown on a [001] SrTiO3 substrate by pulsed laser deposition. Although bulk TbMnO3 is a low temperature…

Materials Science · Physics 2009-11-13 B. J. Kirby , D. Kan , A. Luykx , M. Murakami , D. Kundaliya , I. Takeuchi

We report the structural and magnetic properties of ZnO single crystals implanted at 623 K with up to 10 at. % of Ni. As revealed by X-ray diffraction, crystalline fcc-Ni nanoparticles were formed inside ZnO. The magnetic behavior…

Materials Science · Physics 2007-05-23 Shengqiang Zhou , K. Potzger , Gufei Zhang , F. Eichhorn , W. Skorupa , M. Helm , J. Fassbender

Unexpected ferromagnetism has been observed in carbon doped ZnO films grown by pulsed laser deposition [Phys. Rev. Lett. 99, 127201 (2007)]. In this letter, we introduce carbon into ZnO films by ion implantation. Room temperature…

The existence of high-temperature ferromagnetism in thin films and nanoparticles of oxides containing small quantities of magnetic dopants remains controversial. Some regard these materials as dilute magnetic semiconductors, while others…

Materials Science · Physics 2015-05-18 J. M. D. Coey , P. Stamenov , R. D. Gunning , M. Venkatesan , K. Paul

Magneto-optical properties of ZnO:Co and ZnO:Ni films were measured. Magnetization measurements show that some of the films are paramagnetic and others are ferromagnetic. Magnetic circular dichroism clarified that Zn1-xCoxO and Zn1-xNixO…

Materials Science · Physics 2007-05-23 K. Ando

We review pitfalls in recent efforts to make a conventional semiconductor, namely ZnO, ferromagnetic by means of doping with transition metal ions. Since the solubility of those elements is rather low, formation of secondary phases and the…

Materials Science · Physics 2009-08-06 Kay Potzger , Shengqiang Zhou

Magnetic 3d-ions doped into wide-gap oxides show signatures of room temperature ferromagnetism, although their concentration is two orders of magnitude smaller than that in conventional magnets. The prototype of these exceptional materials…

Materials Science · Physics 2009-11-13 C. D. Pemmaraju , R. Hanafin , T. Archer , H. B. Braun , S. Sanvito

Recently theoretical works predict that some semiconductors (e.g. ZnO) doped with magnetic ions are diluted magnetic semiconductors (DMS). In DMS magnetic ions substitute cation sites of the host semiconductor and are coupled by free…

Materials Science · Physics 2009-07-22 Shengqiang Zhou , K. Potzger , Qingyu Xu , G. Talut , M. Lorenz , W. Skorupa , M. Helm , J. Fassbender , M. Grundmann , H. Schmidt

We report room temperature ferromagnetism in as-implanted Eu doped ZnO (ZnO:Eu). To address the origin of ferromagnetism ab initio calculations of ZnO:Eu system are performed. Results show that the ferromagnetism is induced by ZnO point…

Materials Science · Physics 2010-06-22 M. H. N. Assadi , Y. B. Zhang , M. Ionescu , P. Photongkam , S. Li

Films of ZnO doped with magnetic ions, Mn and Co and, in some cases, with Al have been fabricated with a very wide range of carrier densities. Ferromagnetic behaviour is observed in both insulating and metallic films, but not when the…

Materials Science · Physics 2009-11-13 A. J. Behan , A. Mokhtari , H. J. Blythe , D. Score , X-H. Xu , J. R. Neal , A. M. Fox , G. A. Gehring

During the past years there has been renewed interest in the wide-bandgap II-VI semiconductor ZnO, triggered by promising prospects for spintronic applications. First, ferromagnetism was predicted for dilute magnetic doping. In…

Several experimental studies have referred to the grain boundary (GB) defect as the origin of the ferromagnetism in ZnO. However, the mechanism of this hypothesis has never been confirmed. Present study investigates the atomic structure and…

Materials Science · Physics 2016-01-20 S. Assa Aravindh , Udo Schwingenschloegl , Iman S. Roqan

We have investigated the magnetic properties of non-doped ZnO nanostructures by using {\it ab initio} total energy calculations. Contrary to many proposals that ferromagnetism in non-doped semiconductors should be induced by intrinsic point…

Materials Science · Physics 2009-04-28 A. L. Schoenhalz , J. T. Arantes , A. Fazzio , G. M. Dalpian

Room-temperature ferromagnetism has been observed in the nanoparticles (7 - 30 nm dia) of nonmagnetic oxides such as CeO2, Al2O3, ZnO, In2O3 and SnO2. The saturated magnetic moments in CeO_2 and Al_2O_3 nanoparticles are comparable to those…

Materials Science · Physics 2007-07-24 A. Sundaresan , R. Bhargavi , N. Rangarajan , U. Siddesh , C. N. R. Rao

Sol-gel derived thin films of Zn0.95Mn0.05O have been implanted with Ar9+ ions with doses viz. 5x10e14 ions/cm2 (low), 1x10e15 ions/cm2 (intermediate) and 1x10e16 ions/cm2 (high). Structural, morphological, optical and magnetic properties…

Here we present a study of magnetism in \CTO\ anatase films grown by pulsed laser deposition under a variety of oxygen partial pressures and deposition rates. Energy-dispersive spectrometry and transition electron microscopy analyses…

We report room temperature ferromagnetism in boron-doped ZnO both experimentally and theoretically. The single phase Zn1-xBxO films deposited under high oxygen pressure by pulsed-laser deposition show ferromagnetic behavior at room…

Materials Science · Physics 2015-05-18 X. G. Xu , H. L. Yang , Y. Wu , D. L. Zhang , S. Z. Wu , J. Miao , Y. Jiang

Thin films grown by pulsed-laser deposition from targets of Sn0.95Fe0.05O2 are transparent ferromagnets with Curie temperature and spontaneous magnetization of 610 K and 2.2 Am2kg-1, respectively. The 57Fe Mossbauer spectra show the iron is…

Condensed Matter · Physics 2009-11-10 J. M. D. Coey , A. P. Douvalis , C. B. Fitzgerald , M. Venkatesan

In view of the recent experimental reports of unexpected ferromagnetism in HfO$_{2}$ thin films, we carried out first principles investigations looking for magnetic order possibly brought about by the presence of small concentrations of…

Materials Science · Physics 2007-05-23 Chaitanya Das Pemmaraju , S. Sanvito
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