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Photoreduction of CO$_2$ is an important alternative approach aimed to reduce the CO$_2$ atmospheric content which is responsible of the global warming. The development of an efficient photocatalyst can strongly improve the efficiency and…

Materials Science · Physics 2025-04-29 Onofrio Tau , Giacomo Giorgi , Riccardo Rurali

The turn-over frequency of the catalytic oxidation of CO at RuO2(110) was calculated as function of temperature and partial pressures using ab initio statistical mechanics. The underlying energetics of the gas-phase molecules, dissociation,…

Materials Science · Physics 2009-11-10 Karsten Reuter , Daan Frenkel , Matthias Scheffler

In a previous paper (arXiv:1309.2204, JHEP 1311 (2013) 087), we present a holographic s+p superconductor model with a scalar triplet charged under an SU(2) gauge field in the bulk. We also study the competition and coexistence of the s-wave…

High Energy Physics - Theory · Physics 2017-12-27 Zhang-Yu Nie , Rong-Gen Cai , Xin Gao , Li Li , Hui Zeng

We investigate transport effects in in situ studies of defined model catalysts using a multi-scale modeling approach integrating first-principles kinetic Monte Carlo simulations into a fluid dynamical treatment. We specifically address two…

Materials Science · Physics 2013-07-25 Sebastian Matera , Karsten Reuter

We study the deformation of a Fermi surface (FS) near charge-ordering (CO) transition. By applying a fluctuation-exchange approximation to the two-dimensional extended Hubbard model, we show that the FS is largely modified by strong charge…

Materials Science · Physics 2011-11-28 Kazuyoshi Yoshimi , Takeo Kato , Hideaki Maebashi

In regions where stars form, variations in density and temperature can cause gas to freeze-out onto dust grains forming ice mantles, which influences the chemical composition of a cloud. The aim of this paper is to understand in detail the…

Solar and Stellar Astrophysics · Physics 2017-11-08 S. Cazaux , R. Martin-Domenech , Y. J. Chen , G. M. Munoz Caro , C. Gonzalez Diaz

We found that a surface state induced by hydrogenation on the surface of SrTiO$_{3}$(001) (STO) did not obey the rigid band model, which was confirmed by in situ electrical resistivity measurements in ultrahigh vacuum. With exposure of…

Mesoscale and Nanoscale Physics · Physics 2020-03-04 Y. Takeuchi , R. Hobara , R. Akiyama , A. Takayama , S. Ichinokura , R. Yukawa , I. Matsuda , S. Hasegawa

In models of Pt 111 and Pt 100 surfaces in water, motions of molecules in the first hydration layer are spatially and temporally correlated. To interpret these collective motions, we apply quantitative measures of dynamic heterogeneity that…

Materials Science · Physics 2015-06-15 Adam P. Willard , David T. Limmer , Paul A. Madden , David Chandler

Electronic phase behavior in correlated-electron systems is a fundamental problem of condensed matter physics. We argue here that the change in the phase behavior near the surface and interface, i.e., {\em electronic reconstruction}, is the…

Strongly Correlated Electrons · Physics 2015-06-25 Satoshi Okamoto , Andrew J. Millis

We study the orbital behavior at the neighborhood of complex unstable periodic orbits in a 3D autonomous Hamiltonian system of galactic type. At a transition of a family of periodic orbits from stability to complex instability (also known…

Chaotic Dynamics · Physics 2017-01-09 M. Katsanikas , P. A. Patsis , G. Contopoulos

The behavior of a polyelectrolyte adsorbed on a charged surface of high-dielectric constant is studied by both Monte-Carlo simulation and analytical methods. It is found that in a low ionic strength medium, the transition is first-order…

Soft Condensed Matter · Physics 2007-05-23 Chi-Ho Cheng , Pik-Yin Lai

The band inversion in topological phase matters bring exotic physical properties such as the emergence of a topologically protected surface states. They strongly influence the surface electronic structures of the investigated materials and…

The vibrational properties of carbon monoxide adsorbed to the copper (100) surface are explored within density functional theory. Atoms of the substrate and adsorbate are treated on an equal footing in order to examine the effect of…

mtrl-th · Physics 2009-10-30 Steven P. Lewis , Andrew M. Rappe

Recently the oxygen-reconstructed tantalum surface Ta(001)-p(3$\times$3)-O has experienced considerable attention due its use as a potential platform for Majorana physics in adatom chains. Experimental studies using scanning tunneling…

Mesoscale and Nanoscale Physics · Physics 2019-10-02 R. Mozara , A. Kamlapure , M. Valentyuk , L. Cornils , A. I. Lichtenstein , J. Wiebe , R. Wiesendanger

A high-dimensional potential energy surface (PES) for CO interaction with the Au(111) surface is developed using a machine-learning algorithm. Including both molecular and surface coordinates, this PES enables the simulation of the recent…

Chemical Physics · Physics 2019-12-04 Meng Huang , Xueyao Zhou , Yaolong Zhang , Linsen Zhou , Maite Alducin , Bin Jiang , Hua Guo

Well-ordered organic molecular layers on oxide surfaces are key for organic electronics. Using a combination of scanning tunneling microscopy (STM) and non-contact atomic force microscopy (nc-AFM) we probe the structures of copper…

We study a spacetime obtained from the semi-classical backreaction computed via the Thermofield dynamics approach in the Poincare patch of de Sitter spacetime. The resulting bulk equation takes the Whittaker form and we examine two distinct…

High Energy Physics - Theory · Physics 2026-04-16 Antonis Kalogirou

We study the adsorption-desorption of fluid molecules on a solid substrate by introducing a schematic model in which the adsorption/desorption transition probabilities are given by irreversible kinetic constraints with a tunable violation…

Statistical Mechanics · Physics 2019-11-27 Mauro Sellitto

Detailed semi-empirical interaction potential calculations are performed to determine the potential energy surface experienced by the molecules CO, HCN, H2O and H2CO, when adsorbed on the basal plane (0001) of graphite at low temperature.…

Chemical Physics · Physics 2015-05-13 Azzedine Lakhlifi , John P. Killingbeck

We explore the effect of boundary curvature on the instability of reactive pulses in the catalytic oxidation of CO on microdesigned Pt catalysts. Using ring-shaped domains of various radii, we find that the pulses disappear (decollate from…

Pattern Formation and Solitons · Physics 2009-11-11 L. Qiao , I. G. Kevrekidis , C. Punckt , H. H. Rotermund
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