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The structural and magnetic properties of two mixed-valence cobaltites with formal population of 0.30 Co$^{4+}$ ions per f.u., (Pr$_{1-y}$Y$_{y}$)$_{0.7}$Ca$_{0.3}$CoO$_3$ ($y=0$ and 0.15), have been studied down to very low temperatures by…

Materials Science · Physics 2015-06-17 K. Knizek , J. Hejtmanek , M. Marysko , P. Novak , E. Santava , Z. Jirak , T. Naito , H. Fujishiro , C. R. dela Cruz

Frustrated systems exhibit remarkable properties due to the high degeneracy of their ground states. Stabilised by competing interactions, a rich diversity of typically nanometre-sized phase structures appear in polymer and colloidal…

Nuclear magnetic resonance (NMR), electron paramagnetic resonance (EPR), magnetization measurements and electronic structure calculations in VOMoO4 are presented. It is found that VOMoO4 is a frustrated two-dimensional antiferromagnet on a…

Strongly Correlated Electrons · Physics 2009-11-07 P. Carretta , N. Papinutto , C. B. Azzoni , M. C. Mozzati , E. Pavarini , S. Gonthier , P. Millet

Oxide double perovskites wherein octahedra formed by both 3d elements and sp-based heavy elements give rise to unconventional magnetic ordering and correlated quantum phenomena crucial for futuristic applications. Here, by carrying out…

Strongly Correlated Electrons · Physics 2021-03-30 J. Khatua , T. Arh , Shashi B. Mishra , H. Luetkens , A. Zorko , B. Sana , M. S. Ramachandra Rao , B. R. K. Nanda , P. Khuntia

Hexagonal UNi_4B is magnetically frustrated, yet it orders antiferromagnetically at T_N = 20 K. However, one third of the U-spins remain paramagnetic below this temperature. In order to track these spins to lower temperature, we measured…

Strongly Correlated Electrons · Physics 2009-10-31 R. Movshovich , M. Jaime , S. Mentink , A. A. Menovsky , J. A. Mydosh

Frustrated lattices1-3, characterized by minor breakdown in local order in an otherwise periodic lattice, lead to simultaneous possibilities of several ground states which can trigger unique physical properties, in condensed matter systems.…

Mesoscale and Nanoscale Physics · Physics 2014-04-07 Satyendra Prakash Pal , P. Sen

We have studied the crystal and magnetic structures of the magnetoelectric materials RMn2O5 (R = Tb, Ho, Dy) using neutron diffraction as a function of temperature. All three materials display incommensurate antiferromagnetic ordering below…

Strongly Correlated Electrons · Physics 2009-11-11 G. R. Blake , L. C. Chapon , P. G. Radaelli , S. Park , N. Hur , S-W. Cheong , J. Rodriguez-Carvajal

Magneto-dielectric spectra of La0.95Ca0.05CoO3 covering the crossover of spin states reveals strong coupling of its spin and dipolar degrees of freedom. Signature of spin-state transition at 30K clearly manifests in magnetization, supported…

Materials Science · Physics 2016-02-29 Suchita Pandey , Jitender Kumar , A. M. Awasthi

In our study, we conduct magnetization and heat capacity measurements to investigate field induced magnetic phase transitions within the newly synthesized compound K2Ni2(SeO3)3, a spin-1 dimer system arranged on a triangular lattice. From…

Strongly Correlated Electrons · Physics 2024-05-30 Lei Yue , Ziyou Lu , Kun Yan , Le Wang , Shu Guo , Ruixin Guo , Peng Chen , Xiaobin Chen , Jia-Wei Mei

By performing heat capacity, magnetocaloric effect, torque magnetometry and force magnetometry measurements up to 33 T, we have mapped out the T-H phase diagram of the S = 1/2 spin dimer compound Ba3Cr2O8. We found evidence for…

Strongly Correlated Electrons · Physics 2009-04-03 A. A. Aczel , Y. Kohama , M. Jaime , L. Balicas , K. Ninios , H. B. Chan , H. A. Dabkowska , G. M. Luke

SrTi0.5Mn0.5O3 (STMO) is a chemically disordered perovskite having random distribution of Ti and Mn over 1b site. Striking discrepancies about the structural and magnetic properties of STMO demands detailed analysis which is addressed. To…

We report results of 11B NMR and susceptibility measurements on the quasi 2D frustrated dimer spin system SrCu2(BO3)2 under high pressure. At 2.4 GPa and in a magnetic field of 7 T, NMR lines split with decreasing temperature in two steps.…

Strongly Correlated Electrons · Physics 2009-11-13 Takeshi Waki , Koichi Arai , Masashi Takigawa , Yuta Saiga , Yoshiya Uwatoko , Hiroshi Kageyama , Yutaka Ueda

The antiferromagnetic - ferromagnetic phase transition in YBaCo2O5.50 and YBaCo2O5.44 cobaltites with different types of oxygen-ion ordering in the [YO0.5/0.44] layers has been studied by neutron powder diffraction. Using the magnetic…

Materials Science · Physics 2007-05-23 D. D. Khalyavin , D. N. Argyriou , U. Amann , A. A. Yaremchenko , V. V. Kharton

The synergistic interplay between spin correlations, spin-orbit coupling, and competing exchange interactions provides a promising route to realize exotic quantum states with nontrivial excitations in rare-earth based frustrated magnets.…

Strongly Correlated Electrons · Physics 2026-05-25 J. Khatua , D. Tay , T. Shiroka , M. Pregelj , K. Kargeti , S. K. Panda , G. B. G. Stenning , P. Manuel , M. D. Le , D. T. Adroja , P. Khuntia

Some frustrated pyrochlore antiferromagnets, such as Y2Mo2O7, show a spin-freezing transition and magnetic irreversibilities below a temperature Tf similar to what is observed nonlinear magnetization measurements on Y2Mo2O7 that provide…

Disordered Systems and Neural Networks · Physics 2009-10-28 M. J. P. Gingras , C. V. Stager , N. P. Raju , B. D. Gaulin , J. E. Greedan

We investigate magnetic properties of the $s$ = 1/2 compound K$_{2}$Cu$_{3}$(MoO$_{4}$)$_{4}$ by combining magnetic susceptibility, magnetization, specific heat, and electron spin resonance (ESR) with density functional calculations. Its…

We present the results of magnetic measurements on Nd6Co(1.67)Si3, a compound recently reported to crystallize in a hexagonal structure (space group P6_3/m) and to undergo long range magnetic ordering below 84 K. The results reveal that the…

Strongly Correlated Electrons · Physics 2009-11-13 Niharika Mohapatra , S. Narayana Jammalamadaka , Sitikantha D. Das , E. V. Sampathkumaran

Spin-state ordering - a periodic pattern of ions with different spin-state configurations along a crystal lattice - is a rare phenomenon, and its possible interrelation with other electronic degrees of freedom remains little explored. Here…

Strongly Correlated Electrons · Physics 2024-03-27 E. Granado , C. W. Galdino , B. D. Moreno , G. King , D. C. Freitas

The spin-nematic phase is an intriguing state of matter that lacks usual long-range dipolar order, yet it exhibits higher multipolar order. This makes its detection extremely difficult and controversial. Recently, nuclear magnetic resonance…

Strongly Correlated Electrons · Physics 2020-08-10 M. Pregelj , A. Zorko , D. Arčon , M. Klanjšek , O. Zaharko , S. Krämer , M. Horvatić , A. Prokofiev

Electric quadrupolar state in a frustrated quantum magnet $\rm Tb_{2+\it \delta}Ti_{2-\it \delta}O_7$ has been studied by means of ultrasonic and magnetostriction measurements. A single crystal showed elastic anomaly at about 0.4 K,…

Strongly Correlated Electrons · Physics 2022-03-23 Y. Nii , Y. Hirokane , S. Nakamura , S. Kimura , Y. Tomioka , T. Nojima , Y. Onose