Related papers: Efficiency of energy transfer in a light-harvestin…
It is known that ensembles of interacting oscillators or qubits can exhibit the phenomenon of quantum synchronization. In this work we consider a set of $N$ identical two-state systems that we call ``harmonic qubits'', because the kinetic…
The energy-transfer efficiency of the natural photosynthesis system seems to be perfectly optimized during the evolution for millions of years. However, how to enhance the efficiency in the artificial light-harvesting systems is still…
The coherence of light has been proposed as a quantum-mechanical control for enhancing light-harvesting efficiency. In particular, optical coherence can be manipulated by changing either the polarization state or spectral phase of the…
Quantum coherence, encoded in the off-diagonal elements of a system's density matrix, is a key resource in quantum thermodynamics, fundamentally limiting the maximum extractable work known as ergotropy. While previous experiments have…
We show that quantum coherence can increase the quantum efficiency of various thermodynamic systems. For example, we can enhance the quantum efficiency for a quantum dot photocell, a laser based solar cell and the photo-Carnot quantum heat…
The interplay between coherence and system-environment interactions is at the basis of a wide range of phenomena, from quantum information processing to charge and energy transfer in molecular systems, biomolecules, and photochemical…
Following the calculation of optimal energy transfer in thermal environment in our first paper (Wu et al., New J. Phys., 2010, 12, 105012), full quantum dynamics and leading-order `classical' hopping kinetics are compared in the seven-site…
We derive a unified quantum theory of coherent and incoherent energy transfer between two atoms (donor and acceptor) valid in arbitrary Markovian nanophotonic environments. Our theory predicts a fundamental bound $\eta_{max} =…
An asymptotic scaling theory is presented using the conceptual basis of trapping-free subspace (i.e., orthogonal subspace) to establish the generic mechanism of optimal efficiency of excitation energy transfer (EET) in light-harvesting…
Resonance energy transfer has become an indispensable experimental tool for single-molecule and single-cell biophysics. Its physical underpinnings, however, are subtle: It involves a discrete jump of excitation from one molecule to another,…
A genuine feature of projective quantum measurements is that they inevitably alter the mean energy of the observed system if the measured quantity does not commute with the Hamiltonian. Compared to the classical case, Jacobs proved that…
The resource theory of quantum thermodynamics has emerged as a powerful tool for exploring the out-of-equilibrium dynamics of microscopic and highly correlated systems. Recently, it has been employed in photoisomerization, a mechanism…
The theoretical and experimental study of energy transfer in photosynthesis has revealed an interesting transport regime, which lies at the borderline between classical transport dynamics and quantum-mechanical interference effects.…
Photosystem II (PSII) reaction center is a unique protein-chromophore complex that is capable of efficiently separating electronic charges across the membrane after photoexcitation. In the PSII reaction center, the primary energy- and…
We investigate how optical second-order cross correlations witness the quantum features of a prototype donor-acceptor light-harvesting unit. By considering a pair of detuned two-level emitters electronically coupled and incoherently driven…
It is shown that energy transfer in a homogeneous fully connected quantum network is assisted by a decohering interaction with environmental spins. Analytic expressions for the transfer probabilities are obtained for the zero temperature…
Photosynthesis powers life on our planet. The basic photosynthetic architecture comprises antenna complexes to harvest solar energy and reaction centers to convert the energy into a stable charge separated state. In oxygenic photosynthesis,…
Coherent hopping of excitation rely on quantum coherence over physically extended states. In this work, we consider simple models to examine the effect of symmetries of delocalized multi-excitation states on the dynamical timescales,…
Reversible entanglement transfer between light and matter is a crucial requisite for the ongoing developments of quantum information technologies. Quantum networks and their envisioned applications, e.g., secure communications beyond direct…
For more than 50 years we have known that photosynthetic systems harvest solar energy with almost unit {\it quantum efficiency}. However, recent experimental evidence of {\it quantum coherence} during the excitonic energy transport in…