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We demonstrate a method to quantify and manipulate nuclear spin decoherence mechanisms that are active in zero to ultralow magnetic fields. These include: (i) non-adiabatic switching of spin quantization axis, due to residual background…

Chemical Physics · Physics 2022-06-28 Sven Bodenstedt , Morgan W. Mitchell , Michael C. D. Tayler

Magic-angle spinning (MAS) solid state nuclear magnetic resonance (NMR) spectroscopy is shown to be a promising technique for implementing quantum computing. The theory underlying the principles of quantum computing with nuclear spin…

In this work we experimentally study the efficiency of various dynamical decoupling sequences for suppressing decoherence of single as well as multiple quantum coherences on large spin-clusters. The system involves crystallites of a…

Quantum Physics · Physics 2011-10-10 Abhishek Shukla , T. S. Mahesh

Entanglement can improve the measurement precision of quantum sensors beyond the shot noise limit. Neutral atoms, the basis of some of the most precise and accurate optical clocks and interferometers, do not naturally exhibit all-to-all…

We present a study of the prospects for coherence preservation in solid-state spin qubits using dynamical decoupling protocols. Recent experiments have provided the first demonstrations of multipulse dynamical decoupling sequences in this…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 M. J. Biercuk , H. Bluhm

An exact general theory of heteronuclear decoupling is presented for spin-1/2 IS systems. RF irradiation applied to the I spins decouples the S spins by reversing the sign of antiphase magnetization. A one-to-one correspondence is…

Chemical Physics · Physics 2015-06-19 Thomas E. Skinner

Measuring the Hamiltonian of dipolar coupled spin systems is usually a difficult task due to the high complexity of their spectra. Currently, molecules with unknown geometrical structure and low symmetry are extremely tedious or impossible…

Quantum Physics · Physics 2013-12-10 Denis-Alexandre Trottier , Virginia Jauregui-Villanueva , Jingfu Zhang

Hyperpolarization of nuclear spins enhances nuclear magnetic resonance signals, which play a key role for imaging and spectroscopy in the natural and life sciences. This signal amplification unlocks previously inaccessible techniques, such…

We study multiple-spin coherence transfers in linear Ising spin chains with nearest neighbor couplings. These constitute a model for efficient information transfers in future quantum computing devices and for many multi-dimensional…

We present an efficient scheme which couples any designated pair of spins in heteronuclear spin systems. The scheme is based on the existence of Hadamard matrices. For a system of $n$ spins with pairwise coupling, the scheme concatenates…

Quantum Physics · Physics 2008-12-18 Debbie W. Leung , Isaac L. Chuang , Fumiko Yamaguchi , Yoshihisa Yamamoto

Dipolar coupled homonuclear spins present challenging, yet useful systems for quantum information processing. In such systems, eigenbasis of the system Hamiltonian is the appropriate computational basis and coherent control can be achieved…

Quantum Physics · Physics 2009-11-13 T. S. Mahesh , Dieter Suter

We describe a method for precise estimation of the polarization of a mesoscopic spin ensemble by using its coupling to a single two-level system. Our approach requires a minimal number of measurements on the two-level system for a given…

Quantum Physics · Physics 2009-11-11 G. Giedke , J. M. Taylor , D. D'Alessandro , M. D. Lukin , A. Imamoglu

Optically addressable molecular triplet spins provide a chemically tunable platform for quantum application, but their coherence is often limited by interactions with surrounding spin baths. Here we demonstrate controlled suppression of…

Dynamic nuclear polarization experiments use microwave irradiation to transfer the larger electron polarization to nuclear spins of interest, and thus enhance the NMR transitions above thermal equilibrium. How the polarization transfer from…

Chemical Physics · Physics 2026-01-12 Gian-Marco Camenisch , Nino Wili , Gunnar Jeschke , Matthias Ernst

Identifying weakly coupled nuclear spins around single electron spins is a key step of implementing quantum information processing using coupled electron-nuclei spin systems or sensing like single spin nuclear magnetic resonance detection…

Mesoscale and Nanoscale Physics · Physics 2015-01-08 Nan Zhao , Jörg Wrachtrup , Ren-Bao Liu

The majority of nuclei available for study in solid state Nuclear Magnetic Resonance have half-integer spin $I > 1/2 $, with corresponding electric quadrupole moment. As such, they may couple with a surrounding electric field gradient. This…

Materials Science · Physics 2009-05-19 William J. Brouwer , Michael C. Davis , Karl T. Mueller

Polarization transfers are crucial building blocks in magnetic resonance experiments, i.e., they can be used to polarize insensitive nuclei and correlate nuclear spins in multidimensional NMR spectroscopy. The polarization can be…

Chemical Physics · Physics 2022-08-24 Zhenfeng Pang , Sheetal Jain , Chen Yang , Xueqian Kong , Kong Ooi Tan

From condensed matter to quantum chromodynamics, multidimensional spins are a fundamental paradigm, with a pivotal role in combinatorial optimization and machine learning. Machines formed by coupled parametric oscillators can simulate spin…

Optics · Physics 2022-11-29 Marcello Calvanese Strinati , Claudio Conti

Nuclear magnetic resonance (NMR) spectroscopy is widely used in fields ranging from chemistry, material science to neuroscience. Nanoscale NMR spectroscopy using Nitrogen-vacancy (NV) centers in diamond has emerged as a promising platform…

The higher-order corrections for the SM-like Higgs boson mass and the trilinear Higgs self-couplings in the Next-to-Minimal Supersymmetric extension of the Standard Model (NMSSM) with Inverse Seesaw Mechanism are significant and highly…

High Energy Physics - Phenomenology · Physics 2025-06-04 Thi Nhung Dao , Martin Gabelmann , Margarete Mühlleitner