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In this paper we employ two distinct approaches - all-electron \textit{ab initio} method and the spherical jellium background model- within time dependent density functional theory to calculate the long range dipole-dipole dispersion…

Atomic and Molecular Clusters · Physics 2008-01-10 Arup Banerjee , Manoj K. Harbola

In this paper we employ all-electron time dependent density functional theory (TDDFT) to calculate the long range dipole-dipole dispersion coefficient (van der Waals coefficient) $C_{6}$ of alkali-metal atoms Li, Na, K, alkali-metal atom…

Atomic and Molecular Clusters · Physics 2009-11-13 Arup Banerjee , Jochen Autschbach

In this paper we employ the hydrodynamic formulation of time-dependent density functional theory to obtain the van der Waal coefficients $C_{6}$ and $C_{8}$ of alkali-metal clusters of various sizes including very large clusters. Such…

Atomic and Molecular Clusters · Physics 2007-05-23 Arup Banerjee , Manoj K. Harbola

The van der Waals dispersion coefficients of a set of polycyclic aromatic hydrocarbons, ranging in size from the single-cycle benzene to circumovalene (C66H20), are calculated with a real-time propagation approach to time-dependent density…

Materials Science · Physics 2009-11-13 Miguel A. L. Marques , Alberto Castro , Giuliano Malloci , Giacomo Mulas , Silvana Botti

A local approximation for dynamic polarizability leads to a nonlocal functional for the long-range dispersion interaction energy via an imaginary-frequency integral. We analyze several local polarizability approximations and argue that the…

Chemical Physics · Physics 2015-03-17 Oleg A. Vydrov , Troy Van Voorhis

A simple and computationally efficient scheme to calculate approximate imaginary-frequency dependent polarizability, hence asymptotic van der Waals coefficient, within density functional theory is proposed. The dynamical dipolar…

Materials Science · Physics 2009-04-20 Huy-Viet Nguyen , Stefano de Gironcoli

By inferring the dynamic permittivity of different material media from the observations and calculating dynamic electric dipole polarizabilties of the Li through Cs alkali atoms, precise values of $C_3$ coefficients were estimated in Phys.…

Atomic Physics · Physics 2023-10-02 Harpreet Kaur , Vipul Badhan , Bindiya Arora , B. K. Sahoo

Long range electrostatic, induction and dispersion coefficients including terms of order $R^{-8}$ have been calculated by the sum over states method using time dependent density functional theory. We also computed electrostatic moments and…

Chemical Physics · Physics 2015-06-05 Jason N. Byrd , John A. Montgomery , Robin Côté

Using time-dependent density functional theory (tdDFT) with exchange kernels we calculate and test imaginary frequency-dependent dipole polarizabilities for all atoms and many ns in rows 1-6 of the periodic table. These are then integrated…

Computational Physics · Physics 2016-07-08 Tim Gould , Tomas Bucko

We report a new technique to determine the van der Waals coeffcients of lithium (Li) atoms based on the relativistic coupled-cluster theory. These quantities are determined using the imaginary parts of the scalar dipole and quadrupole…

Atomic Physics · Physics 2009-11-13 L. W. Wansbeek , B. K. Sahoo , R. G. E. Timmermans , B. P. Das , D. Mukherjee

We study the dispersion interaction of the van der Waals and Casimir-Polder (vdW-CP) type between a neutral atom and the surface of a metal by allowing for nonlocal electrodynamics, i.e. electron diffusion. We consider two models: (i) bulk…

Atomic Physics · Physics 2014-07-23 Elad Eizner , Baruch Horovitz , Carsten Henkel

The mounting interest in conducting thorough analyses and studies of long-range interactions stems from their wide-ranging applications in cold atomic physics, making it a compelling area for research. In this work, we have evaluated long…

Atomic Physics · Physics 2025-04-23 Harpreet Kaur , Jyoti , Neelam Shukla , Bindiya Arora

The fully retarded dispersion interaction between an atom and a cluster or between two clusters is calculated. Results obtained with two different methods are compared. One is to consider a cluster as a collection of many atoms and evaluate…

Atomic and Molecular Clusters · Physics 2009-11-11 Hye-Young Kim , Jorge O. Sofo , Darrell Velegol , Milton W. Cole

The van der Waals coefficients and the separation dependent retardation functions of the interactions between the atomically thin films of the multi-layered transition metal molybdenum disulfide (MoS$_2$) dichalcogenides with the alkali…

Materials Science · Physics 2020-08-12 Shankar Dutt , Sukhjit Singh , A. Mahajan , Bindiya Arora , B. K. Sahoo

The van der Waals density functional (vdW-DF) of Dion et al. [Phys. Rev. Lett. 92, 246401 (2004)] is a promising approach for including dispersion in approximate density functional theory exchange-correlation functionals. Indeed, an…

Materials Science · Physics 2013-01-30 Jiří Klimeš , David R. Bowler , Angelos Michaelides

A systematic study of the leading isotropic van der Waals coefficients for the alkali-metal atom + molecule and molecule + molecule systems is presented. Dipole moments and static and dynamic dipole polarizabilities are calculated employing…

Atomic Physics · Physics 2013-02-22 P. S. Zuchowski , M. Kosicki , M. Kodrycka , P. Soldan

The van der Waals (vdW) density functional (vdW-DF) method [ROPP 78, 066501 (2015)] describes dispersion or vdW binding by tracking the effects of an electrodynamic coupling among pairs of electrons and their associated exchange-correlation…

Strongly Correlated Electrons · Physics 2018-02-21 Yang Jiao , Elsebeth Schröder , Per Hyldgaard

London-van der Waals dispersion forces are a fundamental component of condensed matter systems, biological processes, and self-assembly. In this letter we propose a method to calculate the C6 coefficients that characterize dispersion forces…

Chemical Physics · Physics 2019-02-06 Micael J. T. Oliveira , Ksenia Komarova , Francoise Remacle , Matthieu J. Verstraete

Using the general expressions for level shifts obtained from the master equation for a small system interacting with a large one considered as a reservoir, we calculate the dispersive potentials between an atom and a wall in the dipole…

Quantum Physics · Physics 2009-11-13 T. N. C. Mendes , C. Farina

The van der Waals coefficients, from C_11 through to C_16 resulting from 2nd, 3rd and 4th order perturbation theory are estimated for the alkali (Li, Na, K and Rb) atoms. The dispersion coefficients are also computed for all possible…

Atomic Physics · Physics 2007-05-23 J. Mitroy , M. W. J. Bromley
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