Related papers: Robust ultrafast currents in molecular wires throu…
Here we study incoherent transport through molecular wire treated as a linear chain of absorbers, where the phase-breaking processes are modeled by the use of imaginary point-like potentials. The calculations are performed within a…
The influence of an electron-vibrational coupling on the laser control of electron transport through a molecular wire that is attached to several electronic leads is investigated. These molecular vibrational modes induce an effective…
The ac Stark effect was used to induce resonant energy transfer between translationally cold Rydberg atoms. The Rb Rydberg atoms were obtained by laser excitation of cold atoms from a magneto-optical trap. Using two-photon microwave…
In the last decade, advancements in attosecond spectroscopy have allowed us to study electron motion dynamics in condensed matter. The access to these electron dynamics and, consequently, its control by an ultrafast light field paves the…
The appeal of lasers can be attributed to both their ubiquitous applications and their role as model systems for elucidating nonequilibrium and cooperative phenomena. Introducing novel concepts in lasers thus has a potential for both…
An ultrafast mechanism belonging to the family of interatomic Coulombic decay (ICD) phenomena is proposed. When two excited species are present, an ultrafast energy transfer can take place bringing one of them to its ground state and…
We present a scheme utilizing position-dependent ac Stark shifts for doing quantum logic with trapped ions. By a proper choice of direction, position and size, as well as power and frequency of a far-off-resonant Gaussian laser beam,…
We derive a master equation for the electron transport through molecular wires in the limit of strong Coulomb repulsion. This approach is applied to two typical situations: First, we study transport through an open conduction channel for…
We report an ultrafast and efficient way to create the maximum coherence between the two lower states in a -like atomic systems, driven by two nonlinearly chirped few-cycle pulses. The phenomenon of coherent population trapping and…
A laser cooling scheme for trapped ions is presented which is based on the fast dynamical Stark shift gate, described in [Jonathan etal, PRA 62, 042307]. Since this cooling method does not contain an off resonant carrier transition, low…
A circularly polarized laser pulse can induce persistent intra-molecular currents by either exciting or ionizing molecules. These two cases are identified as electron currents and hole currents, respectively, and up to now they have been…
We demonstrate a new, nonlinear optical effect of electric currents. First, a steady current is generated by applying a voltage on a doped GaAs crystal. We demonstrate that this current induces second-harmonic generation of a probe laser…
Novel perspectives of controlling molecular systems have recently arisen from the possibility of generating attosecond pulses in the ultraviolet regime and tailoring electron dynamics in its natural time scale. The cornerstone mechanism is…
Exciting electrons in solids with intense light pulses offers the possibility of generating new states of matter through nonthermal means and controlling their macroscopic properties on femto- to picosecond timescales. One way to manipulate…
In our work, we have engineered low capacitance single quantum dot photodiodes as sensor devices for the optoelectronic sampling of ultrafast electric signals. By the Stark effect, a time-dependent electric signal is converted into a…
Light offers a route to engineer new phases of matter far from equilibrium, including transient states suggestive of superconducting, charge-ordered, and excitonic ordering behavior. Yet it remains unclear how optical excitation can…
Electronic excitation energy transfer along a molecular wire depends on the relative orientation of the electronic transition dipole moments of neighboring chromophores. In porphycenes this orientation is changed upon double proton transfer…
An applied field can modulate optical signals by resonance shifting via the Stark effect. The optical Stark effect (OSE) uses ultrafast light in the transparency region of a material to shift resonances with speeds limited by the pulse…
Achieving coherent population transfer in the solid-state is challenging compared to atomic systems due to closely spaced electronic states and fast decoherence. Here, within an atomistic pseudopotential theory, we offer recipes for the…
Stark deceleration enables the production of cold and dense molecular beams with applications in trapping, collisional studies, and precision measurement. Improving the efficiency of Stark deceleration, and hence the achievable molecular…