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Based on high-order harmonic generation (HHG) spectra obtained from solving the time-dependent Schrodinger equation for atoms, we established quantitatively that the HHG yield can be expressed as the product of a returning electron wave…

Atomic Physics · Physics 2008-08-14 Anh-Thu Le , Toru Morishita , C. D. Lin

We show that high-order harmonics generated from molecules by intense laser pulses can be expressed as the product of a returning electron wave packet and the photo-recombination cross section (PRCS) where the electron wave packet can be…

Atomic Physics · Physics 2008-04-04 Anh-Thu Le , R. Della Picca , P. D. Fainstein , D. A. Telnov , M. Lein , C. D. Lin

We present a quantum optical generalization of the quantum-matter Lewenstein model of high-harmonic generation (HHG) in gases that contains two channels corresponding to the inter- and intraband HHG in solids. Both channels can be presented…

Atomic Physics · Physics 2025-08-21 Adam Thorpe , Neda Boroumand , Graeme Bart , Lu Wang , Giulio Vampa , Thomas Brabec

High-order harmonic generation (HHG) results from strong-field laser matter interaction and it is one of the main processes that are used to extract electron structural and dynamical information about the atomic or molecular targets with…

We investigate high-order harmonic generation in inhomogeneous media for reduced dimensionality models. We perform a phase-space analysis, in which we identify specific features caused by the field inhomogeneity. We compute high-order…

Atomic Physics · Physics 2016-05-25 C. Zagoya , M. Bonner , H. Chomet , E. Slade , C. Figueira de Morisson Faria

The Quantitative Rescattering Theory (QRS) for high-order harmonic generation (HHG) by intense laser pulses is presented. According to the QRS, HHG spectra can be expressed as a product of a returning electron wave packet and the…

Atomic Physics · Physics 2009-08-05 Anh-Thu Le , R. R. Lucchese , S. Tonzani , T. Morishita , C. D. Lin

We investigated the high-order harmonic generation (HHG) process of diatomic molecular ion $\mathrm{H}_2^+$ in non-Born-Oppenheimer approximations. The corresponding three-dimensional time-dependent Schr\"odinger equation is solved with…

Atomic Physics · Physics 2017-02-28 Mu-Zi Li , Guang-Rui Jia , Xue-Bin Bian

We present a generic approach for treating the effect of nuclear motion in the high-order harmonic generation from polyatomic molecules. Our procedure relies on a separation of nuclear and electron dynamics where we account for the…

Atomic Physics · Physics 2010-04-21 C. B. Madsen , M. Abu-samha , L. B. Madsen

High-order harmonic responses from three $C_{20}$ isomers: fullerene, ring, and bowl, are calculated within the modified Lewenstein model for molecular systems. Spectra for all three structures exhibit intense modulations of the harmonic…

Quantum Physics · Physics 2022-03-31 F. Cajiao - Vélez , A. Jaron

The generation of harmonics by atoms or ions in a two-color, coplanar field configuration with commensurate frequencies is investigated through both, an analytical calculation based on the Lewenstein model and the numerical ab initio…

Atomic Physics · Physics 2009-11-07 F. Ceccherini , D. Bauer , F. Cornolti

We investigate the orientation dependence of molecular high-order harmonic generation (HHG) both numerically and analytically. We show that the molecular recollision electronic wave packets (REWPs) in the HHG are closely related to the…

Atomic Physics · Physics 2009-11-13 Yanjun. Chen , Yan. Li , Shiping. Yang , Jie. Liu

High harmonic generation (HHG) from gas phase atoms (or molecules) has opened up a new frontier in ultrafast optics, where attosecond time resolution and Angstrom spatial resolution are accessible. The fundamental physical pictures of HHG…

Optics · Physics 2023-04-26 Liang Li , Pengfei Lan , Xiaosong Zhu , Peixiang Lu

We study high-order harmonic generation (HHG) resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneities of the local electric field and the confinement of the electron motion…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , Srdjan S. Acimovic , T. Shaaran , J. Biegert , R. Quidant , M. Lewenstein

High-order harmonic generation (HHG) is combined with resonant x-ray excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process. To describe this setting, I develop a…

Atomic Physics · Physics 2015-10-15 Christian Buth

We report a detailed study of high-order harmonic generation (HHG) in helium. When comparing predictions from a single-active-electron model with those from all-electron simulations, such as ATTOMESA and R-matrix with time-dependence, which…

Atomic Physics · Physics 2024-03-06 A. T. Bondy , S. Saha , J. C. del Valle , A. Harth , N. Douguet , K. R. Hamilton , K. Bartschat

We present theoretical studies of high-order harmonic generation (HHG) produced by non-homogeneous fields as resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneity of the…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , J. Biegert , R. Quidant , M. Lewenstein

High harmonic generation (HHG) provides a flexible framework for the development of coherent light sources in the extreme-ultraviolet and soft x-ray regimes. However it suffers from low conversion efficiencies as the control of the HHG…

Optics · Physics 2014-09-16 Alberto Castro , Angel Rubio , E. K. U. Gross

High-order harmonic generation (HHG) is investigated for H$_2^+$ and its isotopomers under seven- and ten-cycle trapezoidal laser pulses at 800 nm wavelength and $I$=4$\times 10^{14}$ W$/$cm$^2$ intensity. We solved numerically…

Atomic Physics · Physics 2016-03-03 H. Ahmadi , M. Vafaee , A. Maghari

We investigate high-order harmonic generation (HHG) in graphene with a quantum master equation approach. The simulations reproduce the observed enhancement in HHG in graphene under elliptically polarized light [N. Yoshikawa et al, Science…

Materials Science · Physics 2021-02-03 Shunsuke A. Sato , Hideki Hirori , Yasuyuki Sanari , Yoshihiko Kanemitsu , Angel Rubio

We study high-order harmonic generation (HHG) in model atoms driven by plasmonic-enhanced fields. These fields result from the illumination of plasmonic nanostructures by few-cycle laser pulses. We demonstrate that the spatial inhomogeneous…

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