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The effects of Ag15+ (120 MeV) swift heavy ion irradiation on the structural and morphological properties of epitaxial La0.25Pr0.375Ca0.375MnO3 (LPCMO) thin films was investigated by x-ray scattering and atomic force microscopy (AFM)…

Materials Science · Physics 2023-06-06 Harsh Bhatt , Yogesh Kumar , R. B. Tokas , A. P. Singh , Fouran Singh , Surendra Singh

Using finite-temperature phonon calculations and the Lyddane-Sachs-Teller relations, we calculate ab initio the static dielectric constants of 78 semiconducting oxides and fluorides with cubic perovskite structures at 1000 K. We first…

Materials Science · Physics 2020-11-26 Ambroise van Roekeghem , Jesús Carrete , Stefano Curtarolo , Natalio Mingo

The experimental data on the thermal properties of the nanostructured perovskite ferroelectrics are presented and analysed. The ability of the modified 3w method for specific heat measurements is discussed and illustrated by the thermal…

Materials Science · Physics 2007-05-23 B. Strukov , S. Davitadze , V. Lemanov , S. Shulman , Y. Uesu , S. Asanuma

The perovskite ruthenate has attracted considerable interest due to reports of possible non-Fermi-liquid behavior and its proximity to a magnetic quantum critical point, yet its ground state and electronic structure remain enigmatic. Here…

Strongly Correlated Electrons · Physics 2019-02-12 Yang Liu , Hari P. Nair , Jacob P. Ruf , Darrell G. Schlom , Kyle M. Shen

A previously unreported ferroelectric phase has been revealed on a highly homogeneous sample of Pb(Zr0.52Ti0.48)O3 by high-resolution synchrotron x-ray powder diffraction measurements. At ambient temperature the sample has tetragonal…

Materials Science · Physics 2009-10-31 B. Noheda , D. E. Cox , G. Shirane , J. A. Gonzalo , L. E. Cross , S-E. Park , .

SrMoO4 was studied under compression up to 25 GPa by angle-dispersive x-ray diffraction. A phase transition was observed from the scheelite-structured ambient phase to a monoclinic fergusonite phase at 12.2(9) GPa with cell parameters a =…

Materials Science · Physics 2008-02-04 Daniel Errandonea , Ravhi S. Kumar , Xinghua Ma , Chaoyang Tu

Using density functional theory (DFT) within the local density approximation (LDA), we calculate the physical and electronic properties of PbTiO3 (PTO) and a series of hypothetical compounds PbTiO3-xSx x = 0.2, 0.25, 0.33, 0.5, 1, 2, and 3…

It is demonstrated that for classical perovskites such as BaTiO3, SrTiO3 and PbTiO3 electrostrictive strain induced by an electric field may not obey traditionally considered "extension along the field, contraction perpendicular to it"…

Materials Science · Physics 2015-06-05 Alexander Kvasov , Alexander K. Tagantsev

Organic-inorganic halide perovskites (OIHPs) are promising optoelectronic materials, but their instability under radiation environments restricts their durability and practical applications. Here we employ electron and synchrotron X-ray…

BaTiO$_3$ (BTO) is a prototypical perovskite ferroelectric, whose dielectric permittivity and loss spectra -- which are strongly temperature and frequency dependent -- include contributions from inhomogeneous polarization patterns, with…

Materials Science · Physics 2024-07-31 Ashok Gurung , Mohammad Fatin Ishtiyaq , S. Pamir Alpay , John Mangeri , Serge Nakhmanson

Perovskite oxides form an eclectic class of materials owing to their structural flexibility in accommodating cations of different sizes and valences. They host well known point and planar defects, but so far no line defect has been…

We have fabricated PbTiO$_{3}$/SrRuO$_{3}$ superlattices with ultra-thin SrRuO$_{3}$ layers. Due to the superlattice geometry, the samples show a large anisotropy in their electrical resistivity, which can be controlled by changing the…

Materials Science · Physics 2015-06-03 S. J. Callori , J. Gabel , D. Su , J. Sinsheimer , M. V. Fernandez-Serra , M. Dawber

Recently, a new orthorhombic phase has been discovered in the ferroelectric system Pb(Zn1/3Nb2/3)O3-xPbTiO3 (PZN-xPT) for x= 9%, and for x= 8% after the application of an electric field. In the present work, synchrotron x-ray measurements…

Materials Science · Physics 2009-11-07 D. La-Orauttapong , B. Noheda , Z. -G. Ye , P. M. Gehring , J. Toulouse , D. E. Cox , G. Shirane

For the ferroelectric perovskite compounds BaTiO3 and PbTiO3, we have studied the effects of external electric fields on the structural properties of the (001) surfaces. The field-induced changes in the surface interlayer spacings and…

Materials Science · Physics 2009-10-31 B. Meyer , David Vanderbilt

Perovskite SrRuO3, a prototypical conductive ferromagnetic oxide, exhibits a kink in its band dispersion signalling the unusual electron dynamics therein. However, the origin of this kink remains elusive. By taking advantage of the combo of…

Strongly Correlated Electrons · Physics 2016-03-11 H. F. Yang , Z. T. Liu , C. C. Fan , Q. Yao , P. Xiang , K. L. Zhang , M. Y. Li , H. Li , J. S. Liu , D. W. Shen , M. H. Jiang

Oxides with perovskite-based structures have been known as essential materials for fascinating phenomena such as high-temperature and unconventional superconductivity. Discoveries of these oxide superconductors have driven the science…

The synthesis of SrRuO3 under high-pressure oxygen produces a nonstoichiometric form with randomly distributed vacancies on the Ru-sites, along with a significantly reduced ferromagnetic ordering temperature. In order to gain additional…

The atomic-scale synthesis of artificial oxide heterostructures offers new opportunities to create novel states that do not occur in nature. The main challenge related to synthesizing these structures is obtaining atomically sharp…

We present a thorough dielectric investigation of the hexagonal perovskites La1.2Sr2.7IrO7.33 and La1.2Sr2.7RuO7.33 in a broad frequency and temperature range, supplemented by additional infrared measurements. The occurrence of giant…

Strongly Correlated Electrons · Physics 2016-08-16 P. Lunkenheimer , T. Götzfried , R. Fichtl , S. Weber , T. Rudolf , A. Loidl , A. Reller , S. G. Ebbinghaus

We use a 30-nm x-ray beam to study the spatially resolved properties of a SmNiO$_3$-based nanodevice that is doped with protons. The x-ray absorption spectra supported by density-functional theory (DFT) simulations show partial reduction of…

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