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Related papers: Spin ice behavior in Dy2Sn2-xSbxO7+x/2 and Dy2NbSc…

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We report the low-temperature magnetothermal properties and spin dynamics of a mixed pyrochlore, Dy2GaSbO7 through the coordination of measurements of dc magnetization, ac susceptibility, and heat capacity, and CF computation. In Dy2GaSbO7,…

Materials Science · Physics 2021-04-19 Saikat Nandi , Yatramohan Jana , Jahangir Alam , Pallab Bag , S. S. Islam , Ramesh Nath

We have studied the thermodynamics of the stuffed spin ice material, Dy2(DyxTi2-x)O7-x/2, in which additional Dy3+ replace Ti4+ in the pyrochlore Dy2Ti2O7. Heat capacity measurements indicate that these materials lose the spin ice zero…

Strongly Correlated Electrons · Physics 2008-04-26 B. G. Ueland , G. C. Lau , R. S. Freitas , J. Snyder , M. L. Dahlberg , B. D. Muegge , E. L. Duncan , R. J. Cava , P. Schiffer

Pyrochlore materials are characterized by their hallmark network of corner-sharing rare-earth tetrahedra, which can produce a wide array of complex magnetic ground states. Ferromagnetic Ising pyrochlores often obey the "two-in-two-out" spin…

We report systematic low temperature measurements of the DC magnetization, AC susceptibility, and heat capacity of dysprosium pyrogermanate (Dy2Ge2O7) single crystal and powder samples. Our results confirm that Dy2Ge2O7 is an anisotropic…

Strongly Correlated Electrons · Physics 2009-11-13 X. Ke , M. L. Dahlberg , E. Morosan , J. A. Fleitman , R. J. Cava , P. Schiffer

The recent identification of the dysprosium titanate compound $Dy_2 Ti_2 O_7$ as a ``Spin-Ice'', i.e. the spin analog of regular entropic ice of Pauling, has created considerable excitement. The ability to manipulate spins using magnetic…

Statistical Mechanics · Physics 2009-11-07 B. Sriram Shastry

Neutron scattering, a.c. magnetic susceptibility and specific heat studies have been carried out on polycrystalline Dy2Zr2O7. Unlike the pyrochlore spin ice Dy2Ti2O7, Dy2Zr2O7 crystallizes into the fluorite structure and the magnetic Dy3+…

Disordered Systems and Neural Networks · Physics 2019-07-01 J. G. A. Ramon , C. W. Wang , L. Ishida , P. L. Bernardo , M. M. Leite , F. M. Vichi , J. S. Gardner , R. S. Freitas

We report a study of the low temperature bulk magnetic properties of the spin ice compound Dy2Ti2O7 with particular attention to the (T < 4 K) spin freezing transition. While this transition is superficially similar to that in a spin glass,…

Materials Science · Physics 2007-05-23 J. Snyder , B. G. Ueland , J. S. Slusky , H. Karunadasa , R. J. Cava , P. Schiffer

We report magnetization and ac susceptibility of single crystals of the spin ice compound Dy2Ti2O7. Saturated moments at 1.8 K along the charasteristic axes [100] and [110] agree with the expected values for an effective ferromagnetic…

Strongly Correlated Electrons · Physics 2016-08-31 H. Fukazawa , R. G. Melko , R. Higashinaka , Y. Maeno , M. J. P. Gingras

Spin ice materials are the model systems that have a zero-point entropy as \textit{T} $\rightarrow$ 0 K, owing to the frozen disordered states. Here, we chemically alter the well-known spin ice Ho$_{2}$Ti$_{2}$O$_{7}$ by replacing Ti sites…

Strongly Correlated Electrons · Physics 2022-04-20 Sheetal , A. Elghandour , R. Klingeler , C. S. Yadav

The spin ice system Dy$_{2}$Ti$_{2}$O$_{7}$ exhibits strong frequency-dependent spin-freezing at $\sim$ 16 K temperature. Although it has been a matter of discussion for years, the origin of this unusual spin freezing is still unknown. The…

Strongly Correlated Electrons · Physics 2022-04-06 Sheetal , C. S. Yadav

The low temperature magnetic properties of pyrochlore compound Dy2Ti2O7 in magnetic fields applied along the [111] direction are reported. Below 1 K, a clear plateau has been observed in the magnetization process in the field range 2~9 kOe,…

Materials Science · Physics 2009-11-07 Kazuyuki Matsuhira , Zenji Hiroi , Takashi Tayama , Seishi Takagi , Toshiro Sakakibara

Magnetic pyrochlores with non-Kramers rare-earth ions provide a platform for exploring emergent gauge physics and quantum spin-ice behavior, yet the influence of structural disorder on their ground states remains insufficiently understood.…

The disordered pyrochlore oxide Dy$_{2}$Zr$_{2}$O$_{7}$ shows the signatures of field-induced spin freezing with remnant zero-point spin-ice entropy at 5 kOe magnetic field. We have performed zero-field and longitudinal field Muon spin…

Strongly Correlated Electrons · Physics 2023-03-28 Sheetal , Pabitra K. Biswas , K. Yokoyama , D. T. Adroja , C. S. Yadav

The pyrochlore oxides Dy$_{2}$Ti$_{2}$O$_{7}$ and Ho$_{2}$Ti$_{2}$O$_{7}$ are well studied spin ice systems and have shown the evidences of magnetic monopole excitations. Unlike these, Dy$_{2}$Zr$_{2}$O$_{7}$ is reported to crystallize in a…

Strongly Correlated Electrons · Physics 2020-08-26 Sheetal , Anzar Ali , Sarita Rajput , Yogesh Singh , Tulika Maitra , C. S. Yadav

Dy$_{2}$Zr$_{2}$O$_{7}$ a disordered pyrochlore system, exhibits the spin ice freezing under the application of magnetic field. Our studies suggest the stabilization of pyrochlore phase in Dy$_{2-x}$La$_{x}$Zr$_{2}$O$_{7}$ with the…

Strongly Correlated Electrons · Physics 2021-10-12 Sheetal , C. S. Yadav

We have studied the low temperature a.c. magnetic susceptibility of the diluted spin ice compound Dy(2-x)MxTi2O7, where the magnetic Dy ions on the frustrated pyrochlore lattice have been replaced with non-magnetic ions, M = Y or Lu. We…

Materials Science · Physics 2007-05-23 J. Snyder , B. G. Ueland , Ari Mizel , J. S. Slusky , H. Karunadasa , R. J. Cava , P. Schiffer

We use numerical linked cluster (NLC) expansions to compute the specific heat, C(T), and entropy, S(T), of a quantum spin ice model of Yb2Ti2O7 using anisotropic exchange interactions recently determined from inelastic neutron scattering…

Strongly Correlated Electrons · Physics 2012-10-11 R. Applegate , N. R. Hayre , R. R. P. Singh , T. Lin , A. G. R. Day , M. J. P. Gingras

We present an experimental determination of the isothermal magnetic susceptibility of the spin ice materials Dy2Ti2O7 and Ho2Ti2O7 in the temperature range 1.8-300 K. The use of spherical crystals has allowed the accurate correction for…

Strongly Correlated Electrons · Physics 2013-09-02 L. Bovo , L. D. C. Jaubert , P. C. W. Holdsworth , S. T. Bramwell

We report the specific heat and entropy of single crystals of the spin ice compound Dy2Ti2O7 at temperatures down to 0.35 K. We apply magnetic fields along the four characteristic directions: [100], [110], [111] and [112]. Because of Ising…

Strongly Correlated Electrons · Physics 2009-11-10 Ryuji Higashinaka , Hideto Fukazawa , Yoshiteru Maeno

We report the low temperature magnetic properties of the pyrochlore Pr$_2$Hf$_2$O$_7$. Polycrystalline and single-crystal samples are investigated using time-of-flight neutron spectroscopy and macroscopic measurements, respectively. The…

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