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Related papers: Structure, bonding and magnetism in cobalt cluster…

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Noncollinear magnetic states in clusters are studied by using the single-band Hubbard Hamiltonian. The unrestricted Hartree-Fock (UHF) approximation is considered without imposing any symmetry constraints neither to the size or orientation…

Strongly Correlated Electrons · Physics 2009-10-31 Miguel A. Ojeda , J. Dorantes-Davila , G. M. Pastor

Organometallic clusters based on transition metal atoms are interesting because possible applications in spintronics and quantum information. In addition to the enhanced magnetism at the nanoscale, the organic ligands may provide a natural…

Chemical Physics · Physics 2017-06-12 J. W. González , T. Alonso-Lanza , F. Delgado , F. Aguilera-Granja , A. Ayuela

In this paper we propose a tight-binding molecular dynamics with parameters fitted to first-principles calculations on the smaller clusters and with an environment correction, to be a powerful technique for studying large transition/noble…

Atomic and Molecular Clusters · Physics 2009-11-10 Mukul Kabir , Abhijit Mookerjee , A. K. Bhattacharya

The evolution of the magnetic moment in iron clusters containing 20 to 400 atoms is investigated using first-principles numerical calculations based on density-functional theory and real-space pseudopotentials. Three families of clusters…

Materials Science · Physics 2009-11-11 Murilo L. Tiago , Yunkai Zhou , M. M. G. Alemany , Yousef Saad , James R. Chelikowsky

We have used the Stern-Gerlach deflection technique to study magnetism in chromium clusters of 20-133 atoms. Between 60 K and 100 K, we observe that these clusters have large magnetic moments and respond superparamagnetically to applied…

Atomic and Molecular Clusters · Physics 2009-11-13 F. W. Payne , Wei Jiang , L. A. Bloomfield

The size dependent electronic structure and separate spin and orbital magnetic moments of free Co$_n^+$ ($n = 4\;\textrm{-}\;9$) cluster ions have been investigated by x-ray absorption and x-ray magnetic circular dichroism spectroscopy in a…

Atomic and Molecular Clusters · Physics 2019-10-30 V Zamudio-Bayer , K Hirsch , A Langenberg , A Ławicki , A Terasaki , B von Issendorff , J T Lau

We have investigated structure and properties of small metal clusters using all-electron ab initio theoretical methods based on the Hartree-Fock approximation and density functional theory, perturbation theory and compared results of our…

Atomic and Molecular Clusters · Physics 2009-11-07 Ilia A. Solov'yov , Andrey V. Solov'yov , Walter Greiner

The objective of this paper is to help shedding some light on the nature and the properties of the cold structures formed via thermal instability in the magnetized atomic interstellar medium. To this end, we searched for clumps formed in…

Astrophysics of Galaxies · Physics 2020-12-23 Adriana Gazol , Marco Villagran

The cobalt and iron clusters CoN, FeN (20 < N < 150) measured in a cryogenic molecular beam are found to be bistable with magnetic moments per atom both {\mu}N/N 2{\mu}B in the ground states and {\mu}N */N {\mu}B in the metastable excited…

Strongly Correlated Electrons · Physics 2012-03-06 Xiaoshan Xu , Shuangye Yin , Ramiro Moro , Anthony Liang , John Bowlan , Walt A. de Heer

Magnetic properties of metals are investigated through electronic structure calculations based on the recently-proposed magnetic-field-containing relativistic tight-binding approximation (MFRTB) method [Phys. Rev. B \textbf{91}, 075122…

Strongly Correlated Electrons · Physics 2017-05-31 Masahiko Higuchi , Katsuhiko Higuchi

Electronic structures of 13-atom Rh clusters with three possible high-symmetry geometries are studied using the discrete-variational local-spin-density-functional method. The ground state is found to be the icosahedral structure, and a…

Condensed Matter · Physics 2007-05-23 Yang Jinlong , F. Toigo , Wang Kelin , Zhang Manhong

Global minimum structures of neutral (Fe2O3)n clusters with n = 1-5 were determined employing the genetic algorithm in combination with ab initio parameterized interatomic potentials and subsequent refinement at the density functional…

Materials Science · Physics 2024-05-30 Andreas Erlebach , Carolin Hühn , Richard Jana , Marek Sierka

In this present work, we report a structural and magnetic study of mixed Co58Pt42 clusters. MgO, Nb and Si matrix can be used to embed clusters, avoiding any magnetic interactions between particles. Transmission Electron Microscopy (TEM)…

In this work, results of {\it ab-initio} band structure calculations for $A_2BC$ Heusler compounds that have $A$ and $B$ sites occupied by transition metals and $C$ by a main group element are presented. This class of materials includes…

Materials Science · Physics 2009-11-11 Hem C. Kandpal , Gerhard H. Fecher , Claudia Felser

We report an unusual evolution of structure and magnetism in stoichiometric MnO clusters based on an extensive and unbiased search through the potential energy surface within density functional theory. The smaller clusters, containing up to…

Mesoscale and Nanoscale Physics · Physics 2011-11-11 Shreemoyee Ganguly , Mukul Kabir , Biplab Sanyal , Abhijit Mookerjee

We present a new approach to clustering, based on the physical properties of an inhomogeneous ferromagnet. No assumption is made regarding the underlying distribution of the data. We assign a Potts spin to each data point and introduce an…

Disordered Systems and Neural Networks · Physics 2008-02-03 Marcelo Blatt , Shai Wiseman , Eytan Domany

The theoretical formalism of the local density approximation (LDA) to density functional theory (DFT) has been used to study the electronic and geometric structures of SimCn (1<=m, n<=4;n<=m) clusters. An all electron 6-311++G** basis set…

Atomic and Molecular Clusters · Physics 2007-05-23 Prachi Pradhan , Asok K. Ray

Magnetic properties of Dy_N clusters in a molecular beam generated with a liquid helium cooled nozzle are investigated by Stern-Gerlach experiments. The cluster magnetizations \mu_z are measured as a function of magnetic field (B = 0 -…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 S. Pokrant

The structure, binding energy, magnetic moments and electronic structure of FemIrn clusters are investigated using state of the art density functional theory techniques. Fully unconstrained structural relaxations are undertaken by…

Mesoscale and Nanoscale Physics · Physics 2013-01-23 S. Assa Aravindh

Geometry, electronic structure, and magnetic properties of TMNan (TM=Cr-Ni; n = 4-7) clusters are studied within a gradient corrected density functional theory (DFT) framework. Two complementary approaches, the first adapted to all-electron…

Materials Science · Physics 2017-09-13 Kalpataru Pradhan , Prasenjit Sen , J. Ulises Reveles , Shiv N. Khanna