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Spin-phonon interaction plays an important role in 2D magnetic materials and motivates the development of next-generation spin- and charge-dependent microelectronic devices. Understanding the spin-phonon interaction by tuning the growth…

We report on polarized infrared reflectivity measurements of multiferroic, monoclinic MnWO4 between 10K and 295K. The full dielectric tensor and the frequency dependence of the orientation of the principal axes have been determined in the…

Strongly Correlated Electrons · Physics 2014-10-08 T. Möller , P. Becker , L. Bohaty , J. Hemberger , M. Grüninger

Magnetic and lattice excitations in the quantum antiferromagnet (C$_4$H$_{12}$N$_2$)Cu$_2$Cl$_6$ (PHCC) are studied across two pressure-induced phase transition at $P_c=4.3~\mathrm{kbar}$ and $P_1=13.4~\mathrm{kbar}$ using Raman…

Strongly Correlated Electrons · Physics 2020-03-17 Simon Bettler , Gediminas Simutis , Gérard Perren , Dominic Blosser , Severian Gvasaliya , Andrey Zheludev

The intermediate valence (IV) compound YbAl$_3$ exhibits nonintegral valence (Yb 4$f^{14-n_f}$ (5d6s)$^z$ where z = 2+n$_f$ = 2.75) in a moderately heavy (m* = 20-30me) ground state with a large Kondo temperature (T$_K$ ~ 500-600K). We have…

We have carried out temperature and pressure-dependent Raman and x-ray measurements on single crystals of Tb$_2$Ti$_2$O$_7$. We attribute the observed anomalous temperature dependence of phonons to phonon-phonon anharmonic interactions. The…

Tailored magnon-phonon hybrid systems, where high overtone bulk acoustic resonators couple resonantly to the magnonic mode of a ferromagnetic thin film, are considered optimal for the creation of acoustic phonons with a defined circular…

We investigated the magnetic and magnetoelastic properties of MnSc$_2$Se$_4$ single crystals at low temperature under a magnetic field directed along the crystallographic [111] axis. The magnetization data at low temperature show a linear…

Strongly Correlated Electrons · Physics 2024-10-29 J. Sourd , Y. Skourski , L. Prodan , V. Tsurkan , A. Miyata , J. Wosnitza , S. Zherlitsyn

We study the magnetically-induced phonon splitting in cubic ACr$_2$O$_4$ (A=Mg, Zn, Cd, Hg) spinels from first principles, and demonstrate that the sign of the splitting, which is experimentally observed to be opposite in CdCr$_2$O$_4$…

Materials Science · Physics 2016-05-04 Aleksander L. Wysocki , Turan Birol

AgCrSe$_2$ is an example of a super-ionic conductor that has recently attracted attention for its low thermal conductivity. Here we investigate the optical properties of AgCrSe$_2$ in the ordered phase between 14 K and 374 K using…

Materials Science · Physics 2022-09-01 Jim Groefsema , Xuanbo Feng , Corentin Morice , Yingkai. Huang , Erik van Heumen

Using a combination of first-principles and magnetization-dynamics calculations, we study the effect of the intense optical excitation of phonons on the magnetic behavior in insulating magnetic materials. Taking the prototypical…

Strongly Correlated Electrons · Physics 2018-06-13 M. Fechner , A. Sukhov , L. Chotorlishvili , C. Kenel , J. Berakdar , N. A. Spaldin

We present the Raman scattering results on layered 2D semiconducting ferromagnetic compound CrSiTe$_3$. Four Raman active modes, predicted by symmetry, have been observed and assigned. The experimental results are supported by DFT…

Materials Science · Physics 2018-10-16 A. Milosavljević , A. Šolajić , J. Pešić , Yu Liu , C. Petrovic , N. Lazarević , Z. V. Popović

The temperature dependence of phonon excitations and the presence of spin phonon coupling in polycrystalline Pr2NiMnO6 samples were studied using micro-Raman spectroscopy and magnetometry. Magnetic properties show a single…

Materials Science · Physics 2011-01-17 K. D. Truong , M. P. Singh , S. Jandl , P. Fournier

A first-principles-based method for computing phonons of magnetic random solid solutions including thermal magnetic fluctuations is developed. The method takes fluctuations of force constants (FCs) due to magnetic excitations as well as due…

Materials Science · Physics 2019-08-07 Yuji Ikeda , Fritz Körmann , Biswanath Dutta , Abel Carreras , Atsuto Seko , Jörg Neugebauer , Isao Tanaka

We report Raman spectra measurements on a MoS2 monolayer supported on SiO2 as a function of temperature. Unlike in previous studies, the positions of the two main Raman modes, E2g1 and A1g exhibited nonlinear temperature dependence.…

Mesoscale and Nanoscale Physics · Physics 2014-06-13 Andrzej Taube , Jarosław Judek , Cezariusz Jastrzębski , Anna Duzynska , Krzysztof Świtkowski , Mariusz Zdrojek

We report pressure-dependent reflection and transmission measurements on ZnCr$_2$Se$_4$, HgCr$_2$S$_4$, and CdCr$_2$O$_4$ single crystals at room temperature over a broad spectral range 200-24000 cm$^{-1}$. The pressure dependence of the…

Materials Science · Physics 2018-02-02 K. Rabia , L. Baldassarre , J. Deisenhofer , V. Tsurkan , C. A. Kuntscher

Reflection and transmission as a function of temperature have been measured on a single crystal of the magnetoelectric ferrimagnetic compound Cu$_{2}$OSeO$_{3}$ utilizing light spanning the far infrared to the visible portions of the…

Materials Science · Physics 2015-05-19 K. H. Miller , X. S. Xu , H. Berger , E. S. Knowles , D. J. Arenas , M. W. Meisel , D. B. Tanner

Cr2Ge2Te6 has been of interest for decades, as it is one of only a few naturally forming ferromagnetic semiconductors. Recently, this material has been revisited due to its potential as a 2 dimensional semiconducting ferromagnet and a…

Materials Science · Physics 2016-05-02 Yao Tian , Mason J. Gray , Huiwen Ji , R. J. Cava , Kenneth S. Burch

Lattice vibrations are highly sensitive to crystal symmetries and their changes across phase transitions. The latter can modify irreducible (co)representations and corresponding infrared and Raman selection rules of phonons. This concept is…

We present a systematic study of the structure and lattice dynamics at room temperature, and the phonon behavior at low temperatures in orthorhombic Gd$_{1-x}$Y$_{x}$MnO$_{3}$ manganites, with 0 $\leq$ x $\leq$ 0.4, using powder x-ray…

Strongly Correlated Electrons · Physics 2014-12-31 R. Vilarinho , E. C. Queirós , A. Almeida , P. B. Tavares , J. Agostinho Moreira

Polarized Raman scattering spectra of the K_xCo_{2-y}Se_2 single crystals reveal the presence of two phonon modes, assigned as of the A_{1g} and B_{1g} symmetry. Absence of additional modes excludes the possibility of vacancy ordering,…