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We experimentally demonstrate high degree of polarization of 13C nuclear spins weakly interacting with nitrogen-vacancy (NV) centers in diamond. We combine coherent microwave excitation pulses with optical illumination to provide controlled…

Quantum Physics · Physics 2019-10-25 Jiwon Yun , Kiho Kim , Dohun Kim

Color centers that enable nuclear-spin control without RF fields offer a powerful route towards simplified and scalable quantum devices. Such capabilities are especially valuable for quantum sensing and computing platforms that already find…

Molecular nanostructures may constitute the fabric of future quantum technologies, if their degrees of freedom can be fully harnessed. Ideally one might use nuclear spins as low-decoherence qubits and optical excitations for fast…

Among the possible types of magnetic dipole interactions in molecular systems, couplings between nuclear motion and the nuclear spin have probably received the least attention in molecular spectroscopy. Although very small in comparison to…

Chemical Physics · Physics 2026-04-22 Matthias Diez , Johannes K. Krondorfer , Albert Hirtenfelder , Andreas W. Hauser

Nuclear-spin qubits have long coherence time and are desirably applied into quantum information processing. However, the existing methods either fail to address single nucleus (such as nuclear magnetic resonance), or severely affect nuclear…

Quantum Physics · Physics 2021-11-30 Jian Leng , Fan Yang , Xiang-Bin Wang

In this article, we study control of electron-nuclear spin dynamics at magnetic field strengths where the Larmor frequency of the nucleus is comparable to the hyperfine coupling strength. The quantization axis for the nuclear spin differs…

Quantum Physics · Physics 2009-11-13 Navin Khaneja

We review and summarize recent theoretical and experimental work on electron spin dynamics in quantum dots and related nanostructures due to hyperfine interaction with surrounding nuclear spins. This topic is of particular interest with…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 John Schliemann , Alexander Khaetskii , Daniel Loss

We develop energy efficient, continuous microwave schemes to couple electron and nuclear spins, using phase or amplitude modulation to bridge their frequency difference. These controls have promising applications in biological systems,…

Quantum Physics · Physics 2019-01-14 J. Casanova , E. Torrontegui , M. B. Plenio , J. J. García-Ripoll , E. Solano

Nuclear spins in the solid state environment of diamond are highly coherent, but difficult to rapidly control due to the small nuclear gyromagnetic ratio. Here we demonstrate a more than 50-fold enhancement of the effective nuclear…

Mesoscale and Nanoscale Physics · Physics 2016-08-05 S. Sangtawesin , J. R. Petta

We review recent theoretical and experimental advances toward understanding the effects of nuclear spins in confined nanostructures. These systems, which include quantum dots, defect centers, and molecular magnets, are particularly…

Mesoscale and Nanoscale Physics · Physics 2009-09-15 W. A. Coish , J. Baugh

Coherent two-level systems, or qubits, based on electron spins in GaAs quantum dots are strongly coupled to the nuclear spins of the host lattice via the hyperfine interaction. Realizing nuclear spin control would likely improve electron…

Mesoscale and Nanoscale Physics · Physics 2010-06-15 D. J. Reilly , J. M. Taylor , J. R. Petta , C. M. Marcus , M. P. Hanson , A. C. Gossard

We present a quantum solution to the electron spin decoherence by a nuclear pair-correlation method for the electron-nuclear spin dynamics under a strong magnetic field and a temperature high for the nuclear spins but low for the electron.…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Wang Yao , Ren-Bao Liu , L. J. Sham

We study quantum control of the full hyperfine manifold in the ground-electronic state of alkali atoms based on applied radio frequency and microwave fields. Such interactions should allow essentially decoherence-free dynamics and the…

Quantum Physics · Physics 2009-11-13 Seth T. Merkel , Poul S. Jessen , Ivan H. Deutsch

We report magnetic resonance spectroscopy measurements of individual nuclear spins in a crystal coupled to a neighbouring paramagnetic center, detected using microwave fluorescence at millikelvin temperatures. We observe real-time quantum…

Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…

Quantum Physics · Physics 2022-11-11 Alexander A. Wood , Russell M. Goldblatt , Robert E. Scholten , Andy M. Martin

A coherent superposition of many nuclear spin states can be prepared and manipulated via the hyperfine interaction with the electronic spins by varying the Landau level filling factor through the gate voltage in appropriately designed…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 T. Maniv , Yu. A. Bychkov , I. D. Vagner

We propose a protocol that achieves arbitrary N-qubit interactions between nuclear spins and that can measure directly nuclear many-body correlators by appropriately making the nuclear spins interact with a nitrogen vacancy (NV) center…

Quantum Physics · Physics 2017-09-20 J. Casanova , Z. -Y. Wang , M. B. Plenio

The electron-nuclei (hyperfine) interaction is central to spin qubits in solid state systems. It can be a severe decoherence source but also allows dynamic access to the nuclear spin states. We study a double quantum dot exposed to an…

Mesoscale and Nanoscale Physics · Physics 2013-06-13 Gunnar Petersen , Eric A. Hoffmann , Dieter Schuh , Werner Wegscheider , Geza Giedke , Stefan Ludwig

We introduce a method for solving the problem of an externally controlled electron spin in a quantum dot interacting with host nuclei via the hyperfine interaction. Our method accounts for generalized (non-unitary) evolution effected by…

Mesoscale and Nanoscale Physics · Physics 2011-07-21 Edwin Barnes , Sophia E. Economou

Large-scale quantum computers must be built upon quantum bits that are both highly coherent and locally controllable. We demonstrate the quantum control of the electron and the nuclear spin of a single 31P atom in silicon, using a…