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One of the most fundamental limitations of a muon-spin relaxation experiment can be the lack of knowledge of the implantation site of the muon and the uncertainty about the muon's perturbation of its host. Here we review some of the work…

A spin-polarized muon implanted into a fluoride forms a coupled F--$\mu$--F complex in which the muon spin and neighbouring fluorine nuclear spins become entangled. Here we apply radio-frequency (RF) excitation to this coupled system and…

Muon-spin relaxation (\mu SR) is a sensitive probe of magnetism, but its utility can be severely limited by the lack of knowledge of the muon implantation site and the extent to which the muon perturbs its host. We demonstrate…

Strongly Correlated Electrons · Physics 2013-03-19 J. S. Möller , D. Ceresoli , T. Lancaster , N. Marzari , S. J. Blundell

Entangled spin states are created by implanting muons into single crystal LiY0.95Ho0.05F4 to form a cluster of correlated, dipole-coupled local magnetic moments. The resulting states have well-defined energy levels allowing experimental…

The unitary evolution of a quantum system preserves its coherence, but interactions between the system and its environment result in decoherence, a process in which the quantum information stored in the system becomes degraded. A…

Strongly Correlated Electrons · Physics 2020-08-26 J. M. Wilkinson , S. J. Blundell

A positive muon is a spin-1/2 particle. Beams of muons with all their spins polarized can be prepared and subsequently implanted in various types of condensed matter. The subsequent precession and relaxation of their spins can then be used…

Strongly Correlated Electrons · Physics 2014-10-13 S. J. Blundell

We present a study of a microtwinned single crystal of LaMnO$_3$ by means of implanted muons. Two muon stopping sites are identified from the symmetry of the internal field in the ordered phase. The temperature dependence of these fields…

Condensed Matter · Physics 2019-05-15 M. Cestelli Guidi , G. Allodi , R. De Renzi , G. Guidi , M. Hennion , L. Pinsard , A. Amato

We present the results of a muon-spin relaxation (muSR) investigation into magnetic ordering in several families of layered quasi-two-dimensional molecular antiferromagnets based on transition metal ions such as S=1/2 Cu2+ bridged with…

Muons implanted into ionic fluorides often lead to a so-called F-mu-F state, in which the time evolution of the muon spin contains information about the geometry and nature of the muon site. Nuclei more distant from the muon than the two…

Statistical Mechanics · Physics 2022-01-05 J. M. Wilkinson , F. L. Pratt , T. Lancaster , P. J. Baker , S. J. Blundell

We present the results of muon-spin relaxation measurements of spin excitations in the one-dimensional quantum Heisenberg antiferromagnet Cu(pyz)(NO$_{3}$)$_{2}$. Using density-functional theory we propose muon sites and assess the degree…

Strongly Correlated Electrons · Physics 2015-05-20 F. Xiao , J. S. Möller , T. Lancaster , R. C. Williams , F. L. Pratt , S. J. Blundell , D. Ceresoli , A. M. Barton , J. L. Manson

We present the results of muon-spin relaxation measurements on ferromagnetic BiMnO3. Below T_C=98.0(1) K oscillations in the time-dependence of the muon polarization are observed, characteristic of a quasistatic magnetic field at a single…

Strongly Correlated Electrons · Physics 2007-11-14 T. Lancaster , S. J. Blundell , P. J. Baker , F. L. Pratt , W. Hayes , I. Yamada , M. Azuma , M. Takano

A new pyrochlore compound, NaCaNi$_2$F$_7$, was recently synthesized and has a single magnetic site with spin-1 Ni$^{2+}$. We present zero field (ZF) and longitudinal field (LF) muon spin rotation ($\mu$SR) measurements on this pyrochlore.…

Strongly Correlated Electrons · Physics 2018-09-26 Y. Cai , M. N. Wilson , A. M. Hallas , L. Liu , B. A. Frandsen , S. R. Dunsiger , J. W. Krizan , R. J. Cava , Y. J. Uemura , O. Rubel , G. M. Luke

Muon spin relaxation measurements are reported on samples of dimethylammonium metal formates containing magnetic divalent nickel, cobalt, manganese, and copper ions. These hybrid organic-inorganic perovskites exhibit weak ferromagnetism and…

Strongly Correlated Electrons · Physics 2015-05-19 P. J. Baker , T. Lancaster , I. Franke , W. Hayes , S. J. Blundell , F. L. Pratt , P. Jain , Z. -M. Wang , M. Kurmoo

Uranium beryllium-13 is a heavy fermion system whose anomalous behavior may be explained by its poorly understood internal magnetic structure. Here, uranium beryllium-13's magnetic distribution is probed via muon spin spectroscopy…

Materials Science · Physics 2018-07-11 Jack Li

We present new muon spectroscopy data on a Fe$_3$O$_4$ single crystal, revealing different spin precession patterns in five distinct temperature ranges. A careful analysis of the local field and its straightforward modeling obtains…

Strongly Correlated Electrons · Physics 2013-05-29 M. Bimbi , G. Allodi , R. De Renzi , C. Mazzoli , H. Berger

A model for magnetoresistance in positionally disordered organic materials is presented and solved using percolation theory. The model describes the effects of spin flips on hopping transport by considering the effect of spin dynamics on an…

Disordered Systems and Neural Networks · Physics 2012-05-02 N. J. Harmon , M. E. Flatté

Inspired by recent experimental studies of local magnetic moments interacting with a metallic quasicrystal, we study the low-temperature fate of spins placed in two-dimensional tilings. In the diluted local moment limit, we calculate the…

Strongly Correlated Electrons · Physics 2024-10-17 Ronaldo N. Araújo , Carlo C. Bellinati , Eric C. Andrade

We report muon spin relaxation measurements on two Ti3+ containing perovskites, LaTiO3 and YTiO3, which display long range magnetic order at low temperature. For both materials, oscillations in the time-dependence of the muon polarization…

Strongly Correlated Electrons · Physics 2009-11-13 P. J. Baker , T. Lancaster , S. J. Blundell , W. Hayes , F. L. Pratt , M. Itoh , S. Kuroiwa , J. Akimitsu

We report on the first example of quantum coherence between the spins of muons and quadrupolar nuclei. We observe this effect in vanadium intermetallic compounds which adopt the A15 crystal structure, and whose members include all…

We review examples of muon-spin relaxation measurements on molecule-based magnetic coordination polymers, classified by their magnetic dimensionality. These include the one-dimensional s=1/2 spin chain Cu(pyz)(NO3)2 and the two-dimensional…

Strongly Correlated Electrons · Physics 2014-01-17 T. Lancaster , S. J. Blundell , F. L. Pratt
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