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Resonant soft X-ray scattering was used to determine the presence of more subtle orderings not detected in standard structural analyses. By tuning to specific Co absorption edges, arrangements particular to the electronic states of those…

Strongly Correlated Electrons · Physics 2017-07-17 F. J. Rueckert , F. He , B. Poudel , B. Dabrowski , W. A. Hines , J. I. Budnick , B. O. Wells

We present a detailed study on the charge ordering (CO) transition in GdBaCo2O5 system by combining high resolution synchrotron powder/single crystal diffraction with electron paramagnetic resonance (EPR) experiments as a function of…

Strongly Correlated Electrons · Physics 2015-06-16 M. Allieta , M. Scavini , L. Lopresti , M. Coduri , L. Loconte , S. Cappelli , C. Oliva , P. Ghigna , P. Pattison , V. Scagnoli

The interplay of charge, spin, and lattice degrees of freedom in matter leads to various forms of ordered states through phase transitions. An important subclass of these phenomena of complex materials is charge ordering (CO), mainly driven…

Strongly Correlated Electrons · Physics 2018-08-15 Arvind Yogi , C. I. Sathish , Hasung Sim , Matthew J. Coak , Y. Noda , Je-Geun Park

We used resonant elastic x-ray scattering at the Cu $L_3$ and Dy $M_5$ edges to investigate charge order in thin films of underdoped DyBa$_2$Cu$_3$O$_{6+x}$ (DyBCO) epitaxially grown on NdGaO$_3$ (110) substrates. The films show an…

La doped SrFeO$_{3}$, La$_{1/3}$Sr$_{2/3}$FeO$_{3}$, exhibits a metal-to-insulator transition accompanied by both antiferromagnetic and charge ordering states along with the Fe-O bond disproportionation below a critical temperature near…

Strongly Correlated Electrons · Physics 2025-06-25 Nam Nguyen , Alex Taekyung Lee , Vijay Singh , Anh T. Ngo , Hyowon Park

Neutron diffraction measurements on multiferroic LuFe2O4 show changes in the antiferromagnetic (AFM) structure characterized by wavevector q = (1/3 1/3 1/2) as a function of electric field cooling procedures. The increase of intensity from…

Strongly Correlated Electrons · Physics 2011-11-09 A. M. Mulders , M. Bartkowiak , J. R. Hester , E. Pomjakushina , K. Conder

The kagome lattice is an intriguing and rich platform for discovering, tuning and understanding the diverse phases of quantum matter, which is a necessary premise for utilizing quantum materials in all areas of modern and future electronics…

We argue on the basis of symmetry selection rules and Raman scattering spectra that NaV$_2$O$_5$ undergoes a charge ordering phase transition at T$_c$=34 K. Such a transition is characterized by the redistribution of the charges at the…

Strongly Correlated Electrons · Physics 2009-10-31 M. J. Konstantinovic , Z. V. Popovic , A. N. Vasil'ev , M. Isobe , Y. Ueda

We report resonant X-ray scattering measurements on the orbitally-degenerate triangular metallic antiferromagnet 2H-AgNiO2 to probe the spontaneous transition to a triple-cell superstructure at temperatures below 365 K. We observe a strong…

Strongly Correlated Electrons · Physics 2015-05-19 G. L. Pascut , R. Coldea , P. G. Radaelli , A. Bombardi , G. Beutier , I. I. Mazin , M. D. Johannes , M. Jansen

The present resonant x-ray scattering from each of monoclinically-split single domains of NaV2O5 has critically enhanced contrast between V4+ and V5+ ions strong enough to lead to unambiguous conclusion of the charge-order pattern of its…

We have utilized neutron powder diffraction to probe the crystal structure of layered Na$_{x}$CoO$_{2}$ near the half doping composition of $x=$0.46 over the temperature range of 2 to 600K. Our measurements show evidence of a dynamic…

Strongly Correlated Electrons · Physics 2008-06-16 D. N. Argyriou , O. Prokhnenko , K. Kiefer , C. J. Milne

The Fe intercalated transition metal dichalcogenide (TMD), Fe$_{1/3}$NbS$_2$, exhibits remarkable resistance switching properties and highly tunable spin ordering phases due to magnetic defects. We conduct synchrotron X-ray scattering…

Using low-energy electron diffraction, we show that the room-temperature $(\sqrt{2}\times\sqrt{2})R45^\circ$ reconstruction of Fe$_3$O$_4$(100) reversibly disorders at $\sim$450 $^\circ$C. Short-range order persists above the transition,…

The crystal structure of Fe3O4 below the 122 K Verwey transition has been refined using high-resolution X-ray and neutron powder diffraction data. The refinements give direct evidence for charge ordering (CO) over four independent…

Strongly Correlated Electrons · Physics 2009-11-07 J. P. Wright , J. P. Attfield , P. G. Radaelli

Resonant soft x-ray scattering experiments with photon energies near the O K and the Cu L3 edge on the system La1.8-xEu0.2SrxCuO4 for 0.1 <= x <= 0.15 are presented. A phase diagram for stripe-like charge ordering is obtained together with…

Superconductivity · Physics 2015-05-20 Jörg Fink , Victor Soltwisch , Jochen Geck , Enrico Schierle , Eugen Weschke , Bernd Büchner

In the Fe-Mo based B-site ordered double-perovskite, A2FeMoO6.0, with iron in the mixed-valence II/III state, the valence value of Fe is not precisely fixed at 2.5 but may be fine-tuned by means of applying chemical pressure at the A-cation…

Strongly Correlated Electrons · Physics 2009-11-10 Y. Yasukawa , M. Karppinen , J. Linden , T. S. Chan , R. S. Liu , H. Yamauchi

Resonant soft X-ray scattering with photon energies near the O K and the Cu L3 edges was used to study charge ordering in the system La_{1.8-x}Eu_{0.2}Sr_xCuO_4 as a function of temperature for x = 0.125 and 0.15. From the superstructure…

Superconductivity · Physics 2012-01-13 J. Fink , E. Schierle , E. Weschke , J. Geck , D. Hawthorn , H. Wadati , H. -H. Hu , H. A. Durr , N. Wizent , B. Buchner , G. A. Sawatzky

Transition-metal perovskite oxides exhibit a wide range of extraordinary but imperfectly understood phenomena. Charge, spin, orbital, and lattice degrees of freedom all undergo order-disorder transitions in regimes not far from where the…

Strongly Correlated Electrons · Physics 2009-11-07 Ch. Renner , G. Aeppli , B-G. Kim , Yeong-Ah Soh , S. -W. Cheong

In this work we explore the overall structural behaviour of the [(CH3)2NH2][Mn(HCOO)3] multiferroic compound across the temperature range where its ferroelectric transition takes place by means of calorimetry, thermal expansion measurements…

X-ray and electron diffraction measurements on the metal-insulator (M-I) transition compound PrRu$_4$P$_{12}$ have revealed the emergence of a periodic ordering of charge density around the Pr atoms. It is found that the ordering is…

Strongly Correlated Electrons · Physics 2009-11-10 C. H. Lee , H. Matsuhata , H. Yamaguchi , C. Sekine , K. Kihou , T. Suzuki , T. Noro , I. Shirotani